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We construct a microscopic model based on superexchange theory for a moir\'e bilayer in chromium trihalides (Cr$X_3$, $X=$Br, I). In particular, we derive analytically the interlayer Heisenberg exchange and the interlayer…

Mesoscale and Nanoscale Physics · Physics 2023-06-27 Kok Wee Song

Aiming to clarify the mechanisms governing the interlayer magnetic coupling, we have investigated the stacking energy and interlayer magnetism of bilayer CrBr$_3$ systemically. The magnetic ground states of bilayer CrBr$_3$ with different…

Mesoscale and Nanoscale Physics · Physics 2020-11-06 Jun-Shan Si , Hongxing Li , Bin-Guang He , Zi-Peng Cheng , Wei-Bing Zhang

Two-dimensional (2D) ferromagnets with high Curie temperature have long been the pursuit for electronic and spintronic applications. CrI3 is a rising star of intrinsic 2D ferromagnets, however, it suffers from weak exchange coupling. Here…

Materials Science · Physics 2020-09-22 Yu Guo , Nanshu Liu , Yanyan Zhao , Xue Jiang , Si Zhou , Jijun Zhao

The manipulation of the antiferromagnetic interlayer coupling in the epitaxial Fe/Cr/Fe(001) trilayer system by moderate 5 keV He ion beam irradiation has been investigated experimentally. It is shown that even for irradiation with very low…

Single layers of transition-metal thiophosphates (2D-TMPS$_{3}$) van der Waals magnets are an ideal platform for studying antiferromagnetic interactions in two dimensions. However, the magnetic coupling mechanism between two or more…

Materials Science · Physics 2024-10-18 Andrea León , Beatriz Costa , Thomas Heine , Thomas Brumme

Two-dimensional van der Waals magnetic materials are intriguing for applications in the future spintronics devices, so it is crucial to explore strategy to control the magnetic properties. Here, we carried out first-principles calculations…

Materials Science · Physics 2021-07-20 Chong Xu , Qianjun Wang , Bin Xu , Jun Hu

A recent theoretical study reported large effects of perpendicular electric fields on the atomic structure of a monolayer CrI3, which could be related to the microscopic origin of the technologically promising and experimentally observed…

Materials Science · Physics 2019-07-24 S. Ghosh , N. Stojic , N. Binggeli

The challenge of controlling magnetism using electric fields raises fundamental questions and addresses technological needs such as low-dissipation magnetic memory. The recently reported two-dimensional (2D) magnets provide a new system for…

Atomically thin films of layered chromium triiodide (CrI$_3$) have recently been regarded as suitable candidates to a wide spectrum of technologically relevant applications, mainly owing to the opportunity they offer to achieve a reversible…

Strongly Correlated Electrons · Physics 2020-05-01 Michele Pizzochero , Oleg V. Yazyev

The bilayer of CrI3 is a prototypical van der Waals 2D antiferromagnetic material with magnetoelectric effect. It is not generally known, however, that for symmetry reasons the flexomagnetic effect, i.e., the strain gradient-induced…

Materials Science · Physics 2023-07-12 Lei Qiao , Jan Sladek , Vladimir Sladek , Alexey S. Kaminskiy , Alexander P. Pyatakov , Wei Ren

A key element to tailor the properties of magnetic multilayers is the coupling between the individual magnetic layers. In case of skyrmion hosting multilayers, coupling of skyrmions across the magnetic layers is highly desirable. Here the…

We predict that antiferromagnetic bilayers formed from van der Waals (vdW) materials, like bilayer CrI$_3$, have a strong magnetoelectric response that can be detected by measuring the gate voltage dependence of Faraday or Kerr rotation…

Mesoscale and Nanoscale Physics · Physics 2021-03-15 Chao Lei , Bheema Lingam Chittari , Kentaro Nomura , Nepal Banerjee , Jeil Jung , Allan H. MacDonald

Chromium trihalides, CrX$_3$ (with X = Cl, Br, I), are a family of layered magnetic materials that can be easily exfoliated to provide ferromagnetic monolayers. When two layers are stacked together to form a bilayer the interlayer exchange…

Materials Science · Physics 2020-12-30 Marco Gibertini

Two-dimensional CrI3 has attracted much attention as it is reported to be a ferromagnetic semiconductor with the Curie temperature around 45K. By performing first-principles calculations, we find that the magnetic ground state of CrI3 is…

Computational Physics · Physics 2019-01-09 Zewen Wu , Jin Yu , Shengjun Yuan

Twisting in bilayers introduces structural chirality with two enantiomers, i.e., left- and right-hand bilayers, depending on the oriented twist angle. The interplay between this global chirality and additional degrees of freedom, such as…

Mesoscale and Nanoscale Physics · Physics 2022-11-14 Kunihiro Yananose , Paolo G. Radaelli , Mario Cuoco , Jaejun Yu , Alessandro Stroppa

The ability to control magnetic interactions at the nanoscale is crucial for the development of next-generation spintronic devices and functional magnetic materials. In this work, we investigate theoretically, by means of many-body…

Mesoscale and Nanoscale Physics · Physics 2025-09-18 Tomas T. Osterholt , D. O. Oriekhov , Lumen Eek , Cristiane Morais Smith , Rembert A. Duine

Twisted graphene bilayers develop highly localised states around AA-stacked regions for small twist angles. We show that interaction effects may induce either an antiferromagnetic (AF) and a ferromagnetic (F) polarization of said regions,…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 Luis A. Gonzalez-Arraga , J. L. Lado , Francisco Guinea , Pablo San-Jose

Strong ferromagnetic interlayer exchange couplings $J$ in perpendicularly magnetized systems are becoming increasingly desirable for applications. We study whether ferromagnetic interlayer exchange couplings can be measured by a combination…

Materials Science · Physics 2016-04-22 Thibaut Devolder

We study a model thin film containing diluted bilayer structure with the RKKY long-range interaction. The magnetic subsystem is composed of two magnetically doped layers, separated by an undoped nonmagnetic spacer and placed inside a wider…

Materials Science · Physics 2015-05-13 Karol Szałowski , Tadeusz Balcerzak

We investigate the magnetic structures in a bilayer magnetic system with the locally inverted interlayer coupling region using Monte Carlo simulation. Stabilization of multiple magnetic structures including the magnetic skyrmion is possible…

Mesoscale and Nanoscale Physics · Physics 2020-02-26 Chanki Lee , Hee Young Kwon , Nam Jun Kim , Han Gyu Yoon , Chiho Song , Doo Bong Lee , Jun Woo Choi , Young-Woo Son , Changyeon Won