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We report temperature-dependent Raman spectra of CeFeAsO0.9F0.1 from 4 K to 300 K in spectral range of 60 to 1800 cm-1 and interpret them using estimates of phonon frequencies obtained from first-principles density functional calculations.…

Spin-phonon interactions in 2D magnetic materials are crucial in advancing next-generation spintronic devices. Therefore, identifying new materials with significant spin-phonon interactions is of great importance. In this context, MnSe,…

Materials Science · Physics 2025-02-27 Suman Kalyan Pradhan , Arnab Bera , Soham Das , Yongli Yu , Jicheng Wang , Rui Wu

A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "non-engineered" microscopic model (or in any…

Strongly Correlated Electrons · Physics 2025-10-01 Xun Cai , Zhaoyu Han , Zi-Xiang Li , Steven A. Kivelson , Hong Yao

We report an inelastic neutron scattering investigation of phonons with energies up to 159 meV in the conventional superconductor YNi$_2$B$_2$C. Using the SWEEP mode, a newly developed time-of-flight technique involving the continuous…

Low temperature optical spectroscopy in applied magnetic fields provides clear evidence of magnetoelastic coupling in the spin ice material Ho$_2$Ti$_2$O$_7$. In far-IR reflectometry measurements, we observe field dependent features around…

A spin and phonon excitations spectrum are studied using quantum Monte Carlo method in antiferromagnetic chain with spins $S=1/2$ coupled nonadiabaticity with acoustic phonons . It is found the critical coupling exists to open gap in the…

Soft Condensed Matter · Physics 2007-05-23 S. S. Aplesnin

Triangular lattice of rare-earth ions with interacting effective spin-$1/2$ local moments is an ideal platform to explore the physics of quantum spin liquids (QSLs) in the presence of strong spin-orbit coupling, crystal electric fields, and…

Electronic structure near Fermi level of Pr2CoFeO6 (at 300 K) was investigated by X-ray photoemission spectroscopy (XPS) technique. All three cations, i.e., Pr, Co and Fe were found to be trivalent in nature. XPS analysis also suggested the…

Strongly Correlated Electrons · Physics 2019-05-22 Arkadeb Pal , Surajit Ghosh , Amish G. Joshi , P. K. Gupta , P. Prakash , Amitabh Das , A. K. Ghosh , Sandip Chatterjee

The selective excitation of coherent phonons provides unique capabilities to control fundamental properties of quantum materials on ultrafast time scales. For instance, in the presence of strong electron-phonon coupling, the electronic band…

Materials Science · Physics 2020-06-02 P. Hein , S. Jauernik , H. Erk , L. Yang , Y. Qi , Y. Sun , C. Felser , M. Bauer

We calculate the crystal-field splitting, ground-state Kramers doublet and intersite exchange interactions within the ground-state doublet manifold using an ab initio Hubbard-I based approach for a representative set of Ce and Yb…

Strongly Correlated Electrons · Physics 2026-02-06 Leonid V. Pourovskii , Rafael D. Soares , Alexander Wietek

The existence of CEF states and the magnetism in conducting compounds NdAl2, UPd2Al3 and YbRh2Si2 is discussed. We point out that in metallic compounds localized crystal-field states coexist with conduction electrons. These compounds are…

Strongly Correlated Electrons · Physics 2008-10-08 R. J. Radwanski Z. Ropka

Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…

Unconventional topological quasiparticles have recently garnered significant attention in the realm of condensed matter physics. Here, based on first-principles calculations and symmetry analysis, we reveal the coexistence of multiple types…

Materials Science · Physics 2023-09-21 Xin-Yue Kang , Jin-Yang Li , Si Li

To unravel the interplay between the strong electronic correlation and itinerant-localized dual nature in atypical f electron systems, we employed the density functional theory in combination with the single-site dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2021-02-08 Haiyan Lu , Qin Liu

The electronic structure and electron-phonon coupling in Y2C3 is investigated using density functional calculations. We find that the Fermi level falls in a manifold of mixed character derived from Y d states and antibonding states…

Superconductivity · Physics 2009-11-10 D. J. Singh , I. I. Mazin

We study the ground state properties, the electronic excitations and lattice dynamics in spin-liquid candidate TbInO$_3$. By employing polarization resolved Raman spectroscopy we define the inter- and intra-multiplet excitations, and…

Strongly Correlated Electrons · Physics 2021-08-11 Mai Ye , Xianghan Xu , Xiangyue Wang , Jaewook Kim , Sang-Wook Cheong , Girsh Blumberg

The crystalline electric field (CEF) is investigated in Pr$_3$Pt$_{23}$Si$_{11}$ and Nd$_3$Pt$_{23}$Si$_{11}$ by neutron spectroscopy (NS). At low temperature, the number of observed CEF excitations is consistent with the orthorhombic…

Strongly Correlated Electrons · Physics 2016-12-13 R. M. Galéra , C. Opagiste , M. Amara , J. C. Toussaint , M. B. Lepetit , S. Rols

Rare-earth chalcogenide compounds $\mathrm{ARECh_2}$ (A = alkali or monovalent metal, RE = rare earth, Ch = O, S, Se, Te) are a large family of quantum spin liquid (QSL) candidate materials. $\mathrm{NaYbS_2}$ is a representative member of…

Strongly Correlated Electrons · Physics 2024-09-25 Weizhen Zhuo , Zheng Zhang , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Qingming Zhang

Hybridization between the localized f-electrons and the delocalized conduction electrons together with the crystal electric field (CEF) play a determinant role in governing the many-body ground state of a correlated-electron system. Here,…

We present a rigorous photonic mode model to describe the strong coupling between a monolayer of $\rm MoSe_2$ and a single gold nanoparticle. The onset of strong coupling is quantified by computing the three-dimensional hybrid quasinormal…