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A growing list of Ce-based magnets have shown an extra and heretofore unexplained crystal electric field (CEF) mode at high energies. We describe a process whereby an optical phonon can produce a split CEF mode well above the phonon energy.…

Strongly Correlated Electrons · Physics 2025-07-15 Allen O. Scheie , Sabrina J. Li , Stephen D. Wilson , Daniel A. Rehn

We investigate magnetically tunable Feshbach resonances in ultracold collisions between ground-state Yb and Cs atoms, using coupled-channel calculations based on an interaction potential recently determined from photoassociation…

The quasiparticle relaxation dynamics of the iron-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ ($T_c$ $\sim$ 29 K) were investigated using ultrafast optical spectroscopy. A pseudogap ($\Delta_{PG}$ $\approx$ 3.3 meV) was observed to open…

Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…

Strongly Correlated Electrons · Physics 2021-11-16 Jie Xing , Liurukara D. Sanjeewa , Andrew F. May , Athena S. Sefat

Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…

The delafossite structure of NaYbS2 contains a planar spin-1/2 triangular lattice of Yb3+ ions and features a possible realisation of a quantum spin-liquid state. We investigated the Yb3+ spin dynamics by Electron Spin Resonance (ESR) in…

Strongly Correlated Electrons · Physics 2019-03-11 Jörg Sichelschmidt , Philipp Schlender , Burkhard Schmidt , Michael Baenitz , Thomas Doert

We have measured polarized Raman scattering spectra of the Fe$_{1-x}$Co$_{x}$Sb$_{2}$ and Fe$_{1-x}$Cr$_{x}$Sb$_{2}$ (0$\leq x\leq $0.5) single crystals in the temperature range between 15 K and 300 K. The highest energy $B_{1g}$ symmetry…

Strongly Correlated Electrons · Physics 2016-09-20 N. Lazarević , Z. V. Popović , Rongwei Hu , C. Petrovic

The Kondo semiconductor $Yb B_{12}$ exhibits a spin and charge gap of approximately 15 meV. Close to the gap energy narrow dispersive collective excitations were identified by previous inelastic neutron scattering experiments. We present a…

Strongly Correlated Electrons · Physics 2009-03-10 Alireza Akbari , Peter Thalmeier , Peter Fulde

A primary goal at the interface of theoretical and experimental quantum magnetism is the investigation of exotic spin states, most notably quantum spin liquids (QSLs). Magnetic rare-earth ions go beyond the straightforward paradigm of…

Strongly Correlated Electrons · Physics 2022-01-11 Christopher A. Pocs , Peter E. Siegfried , Jie Xing , Athena S. Sefat , Michael Hermele , Bruce Normand , Minhyea Lee

The origin of quasi-one-dimensional (q1D) ferromagnetic (FM) excitations in the candidate spin-triplet superconductor CeSb$_2$ has remained unclear. Here we report an electronic mechanism for emergent q1D magnetism in the…

In low-temperature resonant Raman experiments on MoSe$_2$-WSe$_2$ heterobilayers, we identify a hybrid interlayer shear mode (HSM) with an energy, close to the interlayer shear mode (SM) of the heterobilayers, but with a much broader,…

We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

CaBi$_2$ is a recently discovered type-I superconductor with $T_c=2$~K and a layered crystal structure. In this work electronic structure, lattice dynamics and electron-phonon interaction are studied, with a special attention paid to the…

Superconductivity · Physics 2019-04-02 Sylwia Gołąb , Bartłomiej Wiendlocha

To get an insight into a new type of quantum critical phenomena recently discovered in the quasicrystal Yb$_{15}$Al$_{34}$Au$_{51}$ and approximant crystal (AC) Yb$_{14}$Al$_{35}$Au$_{51}$ under pressure, we discuss the property of the…

Strongly Correlated Electrons · Physics 2018-04-16 Shinji Watanabe , Kazumasa Miyake

We use inelastic neutron scattering to study the crystalline electric field (CEF) excitations of Ce$^{3+}$ in CeFeAsO$_{1-x}$F$_{x}$($x=0,0.16$). For nonsuperconducting CeFeAsO, the Ce CEF levels have three magnetic doublets in the…

We report an ultrafast optical spectroscopy study on the coherent phonon dynamics in the topological semimetal CeBi and its nonmagnetic isostructural compound LaBi, revealing profound insights into their electronic and magnetic…

Strongly Correlated Electrons · Physics 2025-07-15 Xu-Chen Nie , Chen Zhang , Qi-Yi Wu , Hao Liu , Jie Pang , You-Guo Shi , Zhi-An Xu , Yan-Feng Guo , Ya-Hua Yuan , H. Y. Liu , Yu-Xia Duan , Jian-Qiao Meng

We describe a coherent control technique for coupling electron spin states associated with semiconductor double-dot molecule to a microwave stripline resonator on a chip. We identify a novel regime of operation in which strong interaction…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. M. Taylor , M. D. Lukin

Local charge, spin, or orbital degrees of freedom with intersite interactions are oftentimes sufficient to construct most quantum orders. This is conventionally true for f-electron systems, where the extent of the f-electrons and their…

Long-range entanglement in quantum spin liquids (QSLs) lead to novel low energy excitations with fractionalised quantum numbers and (in 2D) statistics. Experimental detection and manipulation of these excitations present a challenge…

Strongly Correlated Electrons · Physics 2021-11-22 Srishti Pal , Arnab Seth , Piyush Sakrikar , Anzar Ali , Subhro Bhattacharjee , D. V. S. Muthu , Yogesh Singh , A. K. Sood

The rare earth intermetallic system \textit{R}Al\textit{X} (\textit{R} = rare earth elements, \textit{X} = Si and Ge) is known to be a promising candidate of magnetic Weyl semimetal. Due to the complex interactions between the rare earth…