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Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

The delafossite family of compounds with a triangular lattice of rare earth ions has been recently proposed as a candidate host for quantum spin liquid (QSL) states. To realize QSLs, the crystal-electric-field (CEF) ground state of the rare…

Strongly Correlated Electrons · Physics 2020-07-20 Shang Gao , Fan Xiao , Kazuya Kamazawa , Kazuhiko Ikeuchi , Daniel Biner , Karl Krämer , Christian Rüegg , Taka-hisa Arima

On the basis of the point charge model, we formulate the crystalline electronic field (CEF) Hamiltonian $H_{\rm CEF}$ in the rare-earth based quasicrystal (QC) and approximant crystal (AC) with ligand ions located at pseudo 5-fold…

Strongly Correlated Electrons · Physics 2022-03-22 Shinji Watanabe , Mina Kawamoto

Drawing inspiration from the recent breakthroughs in the \ce{Na_{2}BaCo(PO_{4})_{2}} quantum magnet, renowned for its spin supersolidity phase and its potential for revolutionary cooling applications, our study delves into the intricate…

We report inelastic light scattering experiments on superconductor Ce0.6Y0.4FeAsO0.8F0.2 from 4K to 300K covering the superconducting transition temperature Tc ~ 48.6K. A strong evidence of the superconductivity induced phonon…

Materials Science · Physics 2015-06-17 Pradeep Kumar , D. V. S. Muthu , J. Prakash , A. K. Ganguli , A. K. Sood

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

Materials Science · Physics 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch

We study a simple electron-phonon model on square and triangular versions of the Lieb-lattice using an asymptotically exact strong coupling analysis. At zero temperature and electron density $n = 1$ (one electron per unit cell), for various…

Strongly Correlated Electrons · Physics 2023-05-05 Zhaoyu Han , Steven A. Kivelson

The optical properties of the superconducting single crystal Rb$_{0.8}$Fe$_{1.68}$Se$_2$ with $T_{c}$ $\simeq$ 31 K have been measured over a wide frequency range in the $ab$ plane. We found that the optical conductivity is dominated by a…

Superconductivity · Physics 2015-06-19 B. Xu , Y. M. Dai , J. Han , K. Wang , R. Yang , Y. X. Yang , W. Zhang , H. Xiao , X. G. Qiu

In this paper, we performed thermodynamic and electron spin resonance (ESR) measurements to study low-energy magnetic excitations, which were significantly affected by crystalline electric field (CEF) excitations due to relatively small…

Strongly Correlated Electrons · Physics 2021-08-24 Weiwei Liu , Zheng Zhang , Dayu Yan , Jianshu Li , Zhitao Zhang , Jianting Ji , Feng Jin , Youguo Shi , Qingming Zhang

The crystalline electric field (CEF) of Ce3+ in trigonal symmetry has recently become of some relevance, for instance, in the search of frustrated magnetic systems. Fortunately, it is one of the CEF case in which a manageable analytic…

Strongly Correlated Electrons · Physics 2018-11-21 Jacintha Banda , Binod K. Rai , Helge Rosner , Emilia Morosan , Christoph Geibel , Manuel Brando

A triangular lattice selenide series of rare earth (RE), CsRESe2, were synthesized as large single crystals using a flux growth method. This series stabilized in either trigonal (R-3m) or hexagonal (P63/mmc) crystal systems. Physical…

The lack of the theory of the crystalline electric field (CEF) in rare-earth based quasicrystal (QC) and approximant crystal (AC) has prevented us from understanding the electronic states. Recent success of the formulation of the CEF theory…

Strongly Correlated Electrons · Physics 2023-07-24 Shinji Watanabe , Tatsuya Iwasaki

We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

Electron Spin Resonance (ESR) can microscopically probe both conduction electrons (ce) and local moment (LM) spin systems in different materials. A ce spin resonance (CESR) is observed in metallic systems based on light elements or with…

Strongly Correlated Electrons · Physics 2009-08-04 L. M. Holanda , J. M. Vargas , C. Rettori , S. Nakatsuji , K. Kuga , Z. Fisk , S. B. Oseroff , P. G. Pagliuso

[Fe(phen)2(NCS)2] is a prototype transition metal complex material, which undergoes a phase transition between low-spin (LS) and high-spin (HS) phases, induced by temperature, pressure or light. Vibrational modes play a key role for…

Recently reported van der Waals layered honeycomb rare-earth chalcohalides REChX (RE = rare earth, Ch = chalcogen, and X = halogen) are considered to be promising Kitaev spin liquid (KSL) candidates. The high-quality single crystals of…

Strongly Correlated Electrons · Physics 2024-10-28 Yanzhen Cai , Wei Ren , Xijing Dai , Jing Kang , Weizhen Zhuo , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Zheng Zhang , Qingming Zhang

The interactions between elementary excitations such as phonons, plasmons, magnons, or particle-hole pairs, drive emergent functionalities and electronic instabilities such as multiferroic behaviour, anomalous thermoelectric properties,…

Quantum spin liquid (QSL), a state characterized by exotic low energy fractionalized excitations and statistics is still elusive experimentally and may be gauged via indirect experimental signatures. Remnant of QSL phase may reflect in the…

Strongly Correlated Electrons · Physics 2023-03-29 Vivek Kumar , Deepu Kumar , Birender Singh , Yuliia Shemerliuk , Mahdi Behnami , Bernd Buchner , Saicharan Aswartham , Pradeep Kumar

We report neutron inelastic scattering measurements on the normal and superconducting states of single-crystalline Cs0.8Fe1.9Se2. Consistent with previous measurements on Rb(x)Fe(2-y)Se2, we observe two distinct spin excitation signals: (i)…

We investigate the magnetic and crystal electric field (CEF) states of the Kondo lattice system CeCuGa3 by muon spin relaxation (muSR), neutron diffraction, and inelastic neutron scattering (INS) measurements. A noncentrosymmetric…

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