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Recent work with laser-cooled molecules in attractive optical traps has shown that the differential AC Stark shifts arising from the trap light itself can become problematic, limiting collisional shielding efficiencies, rotational coherence…

Atomic Physics · Physics 2022-06-08 Yukai Lu , Connor M. Holland , Lawrence W. Cheuk

Building a refrigerator based on the conversion of heat into optical energy is an ongoing engineering challenge. Under well-defined conditions, spontaneous anti-Stokes fluorescence of a dopant material in a host matrix is capable of…

Optics · Physics 2009-11-13 Peter Muys

In red-detuned magneto-optical traps (MOTs) of molecules, sub-Doppler heating competes with Doppler cooling, resulting in high temperature and low density. A solution is offered by the blue-detuned MOT where sub-Doppler cooling dominates…

Atomic Physics · Physics 2026-01-30 Qinshu Lyu , M. R. Tarbutt

Laser cooling typically requires one or more repump lasers to clear dark states and enable recycling transitions. Here, we have achieved cooling of Be+ ions using a single laser beam, facilitated by one-dimensional heating through…

Atomic Physics · Physics 2024-06-21 Yue Xiao , Yongxu Peng , Linfeng Chen , Chunhui Li , Zongao Song , Xin Wang , Tao Wang , Yurun Xie , Bin Zhao , Tiangang Yang

We consider optical properties of a gas of molecules that are brought to fast unidirectional spinning by a pulsed laser field. It is shown that a circularly polarized probe light passing through the medium inverts its polarization…

Optics · Physics 2015-06-17 Uri Steinitz , Yehiam Prior , Ilya Sh. Averbukh

We propose an alternative method to laser cooling. Our approach utilizes the extreme brightness of a supersonic atomic beam, and the adiabatic atomic coilgun to slow atoms in the beam or to bring them to rest. We show how internal-state…

The equations of motion for the molecular rotation are derived for vibrationally cold dimers that are polarized by off-resonant laser light. It is shown that, by eliminating electronic and vibrational degrees of freedom, a quantum master…

Quantum Physics · Physics 2009-11-10 A. Adelswaerd , S. Wallentowitz , W. Vogel

A lightsail can be accelerated to ultra-high speed by the radiation pressure of a laser having an intensity of the order of GW/m$^2$, which though presents a critical challenge in the thermal management of lightsails. In this letter, we…

Optics · Physics 2022-06-14 Weiliang Jin , Wei Li , Chinmay Khandekar , Meir Orenstein , Shanhui Fan

Laser cooling of atomic motion enables a wide variety of technological and scientific explorations using cold atoms. Here we focus on the effect of laser cooling on the photons instead of on the atoms. Specifically, we show that…

Quantum Physics · Physics 2018-09-24 Chiao-Hsuan Wang , M. J. Gullans , J. V. Porto , William D. Phillips , Jacob M. Taylor

Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple…

We investigate sub-Doppler laser cooling of bosonic potassium isotopes, whose small hyperfine splitting has so far prevented cooling below the Doppler temperature. We find instead that the combination of a dark optical molasses scheme that…

Atomic Physics · Physics 2023-07-20 M. Landini , S. Roy , L. Carcagni' , D. Trypogeorgos , M. Fattori , M. Inguscio , G. Modugno

We propose a highly efficient and fast method of translational cooling for high-angular-momentum atoms. Optical pumping and stimulated transitions, combined with magnetic forces, can be used to compress phase-space density, and the…

Atomic Physics · Physics 2023-10-03 Logan E. Hillberry , Dmitry Budker , Simon M. Rochester , Mark G. Raizen

We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path…

In this paper laser cooling of atoms with a narrow-line optical transition, i.e. in regimes of quantum nature of laser-light interactions resulting in a significant recoil effect, is studied. It is demonstrated that a minimum laser cooling…

Atomic Physics · Physics 2019-03-06 O. N. Prudnikov , R. Ya Il'enkov , A. V. Taichenachev , V. I. Yudin

A proposal for cooling the translational motion of optically levitated magnetic nanoparticles is presented. The theoretical cooling scheme involves the sympathetic cooling of a ferromagnetic YIG nanosphere with a spin-polarized atomic gas.…

Atomic Physics · Physics 2020-11-17 T. Seberson , Peng Ju , Jonghoon Ahn , Jaehoon Bang , Tongcang Li , F. Robicheaux

We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…

Atomic Physics · Physics 2022-08-24 S. F. Vázquez-Carson , Q. Sun , J. Dai , D. Mitra , T. Zelevinsky

We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle.…

Chemical Physics · Physics 2015-05-28 Erez Gershnabel , Ilya Sh. Averbukh

We present a magnetically enhanced laser cooling scheme applicable to multi-level type-II transitions and further diatomic molecules with adiabatic transfer. An angled magnetic field is introduced to not only remix the dark states, but also…

Atomic Physics · Physics 2019-05-07 Qian Liang , Tao Chen , Wenhao Bu , Yuhe Zhang , Bo Yan

Sympathetic cooling of trapped ions has been established as a powerful technique for manipulation of non-laser-coolable ions (Raizen1992,Waki1992,Bowe1999,Barrett2003). For molecular ions, it promises vastly enhanced spectroscopic…

Quantum Physics · Physics 2018-06-06 Soroosh Alighanbari , Michael Georg Hansen , Vladimir Korobov , Stephan Schiller

We theoretically and computationally investigate the cooling of antihydrogen, $\bar{H}$, using optical molasses cooling. This updates the results in Ref. [1] to the current capabilities of the ALPHA experiment. Through Monte Carlo…

Atomic Physics · Physics 2025-02-11 Spencer J. Walsh , C. Ø. Rasmussen , F. Robicheaux