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We present a mechanism for cooling atoms by a laser beam reflected from a single mirror. The cooling relies on the dipole force and thus in principle applies to arbitrary refractive particles including atoms, molecules, or dielectric…

Quantum Physics · Physics 2009-08-05 André Xuereb , Peter Horak , Tim Freegarde

We explore whether localized surface plasmon polariton modes can transfer heat between molecules placed in the hot spot of a nanoplasmonic cavity through optomechanical interaction with the molecular vibrations. We demonstrate that external…

Quantum Physics · Physics 2019-07-16 S. Mahmoud Ashrafi , R. Malekfar , A. R. Bahrampour , Johannes Feist

The problem of deep laser cooling of $^{24}$Mg atoms is theoretically studied. We propose two-stage sub-Doppler cooling strategy using electro-dipole transition $3^3P_2$$\to$$3^3D_3$ ($\lambda$=383.9 nm). The first stage implies exploiting…

We experimentally observe the action of multiple light pulses on the transverse motion of a continuous beam of fullerenes. The light potential is generated by non-resonant ultra-short laser pulses in perpendicular spatial overlap with the…

Atomic and Molecular Clusters · Physics 2013-07-02 Paul Venn , Hendrik Ulbricht

The recent progress towards production of near-ground state quantum-degenerate molecules raises the issue of how such "small" molecules behave in an optical lattice. In this Letter we show that the coupling of the molecular orientation to…

Other Condensed Matter · Physics 2007-07-09 J. R. Holt , J. M. F. Gunn

Manipulating mega biomolecules and micro-devices with light is highly appealing. Opto driving torque can propel micro-rotors to translational motion in viscous liquid, and then separate microsystems according to their handedness. We study…

Fluid Dynamics · Physics 2018-09-05 Yiwen Tang , Zhibing Li

Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…

Atomic Physics · Physics 2023-06-06 Nickolas H. Pilgram , Arian Jadbabaie , Chandler J. Conn , Nicholas R. Hutzler

We demonstrate a laser frequency stabilization technique for laser cooling of Potassium atoms, based on saturated absorption spectroscopy in the C-Band optical telecommunication window, using ro-vibrationel transitions of the acetylene…

We analyze the laser cooling of polarizable particles by continuous dispersive position detection and active feedback. The magnitude of the dissipative force is proportional to the particles' photon scattering rate into the detector, while…

Quantum Physics · Physics 2013-05-29 Vladan Vuletic , Adam T. Black , James K. Thompson

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

A thermal atomic beam of dysprosium (Dy) atoms is cooled using the $4f^{10}6s^2 (J=8) \to 4f^{10}6s6p (J=9)$ transition at 421 nm. The cooling is done via a standing light wave orthogonal to the atomic beam. Efficient transverse cooling to…

Atomic Physics · Physics 2013-05-29 N. Leefer , A. Cingöz , B. Gerber-Siff , Arijit Sharma , J. R. Torgerson , D. Budker

We propose an array of ultracold polar molecules as a platform to study alignment transport between molecules. We envision a polar molecule being aligned with an intense off-resonant laser field whose alignment migrates to a nearby molecule…

Chemical Physics · Physics 2024-02-27 Jonathan Smucker , Jesus Pérez-Ríos

It is predicted that nuclear spin conversion in molecules can be efficiently controlled by strong laser radiation resonant to rovibrational molecular transition. The phenomenon can be used for substantial enrichment of spin isomers, or for…

Chemical Physics · Physics 2009-11-06 P. L. Chapovsky

We present a detailed theoretical and experimental study of the rotation of the plane of polarization of light traveling through a gas of fast-spinning molecules. This effect is similar to the polarization drag phenomenon predicted by Fermi…

Methods of enhanced laser cooling of particle beams in storage rings and Robinson's damping criterion are discussed. The dynamics of amplitudes of betatron oscillations and instantaneous orbits of electrons interacting with laser beams…

Classical Physics · Physics 2007-05-23 E. G. Bessonov

We propose to repeatedly load laser-cooled molecules into optical tweezers, and transfer them to storage states that are rotationally excited by two additional quanta. Collisional loss of molecules in these storage states is suppressed, and…

Atomic Physics · Physics 2024-05-16 Etienne F. Walraven , Michael R. Tarbutt , Tijs Karman

We combine experimental and theoretical approaches to explore excited rotational states of molecules embedded in helium nanodroplets using CS$_2$ and I$_2$ as examples. Laser-induced nonadiabatic molecular alignment is employed to measure…

The dynamics of non-polar diatomic molecules interacting with a far-detuned narrow-band laser field, that only may drive rotational transitions, is studied. The rotation of the molecule is considered both classically and quantum…

Quantum Physics · Physics 2009-11-10 A. Adelswaerd , S. Wallentowitz

It is shown that the translational degrees of freedom of a large variety of molecules, from light diatomic to heavy organic ones, can be cooled sympathetically and brought to rest (crystallized) in a linear Paul trap. The method relies on…

Quantum Physics · Physics 2009-11-10 S. Schiller , C. Laemmerzahl

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

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