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The possibility of strong coupling between a single molecule and surface plasmons is analyzed on the basis of a microscopic classical description. It is predicted that strong single molecule - plasmon coupling can happen for a silver…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Mykhaylo M. Dvoynenko

We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 Adi Salomon , Robert J. Gordon , Yehiam Prior , Tamar Seideman , Maxim Sukharev

Plasmonic structures interacting with light provide electromagnetic resonances which result in a high degree of local field confinement enabling the enhancement of light-matter interaction. Plasmonic structures typically consist of metals…

The strong coupling of molecules with surface plasmons results in hybrid states which are part molecule, part surface-bound light. Since molecular resonances may acquire the spatial coherence of plasmons, which have mm-scale propagation…

Optics · Physics 2022-05-26 Marie S Rider , Rakesh Arul , Jeremy J Baumberg , William L Barnes

The strong coupling between two subsystems consisting of quantum emitters and photonic modes, at which the level splitting of mixed quantum states occurs, has been a central subject of quantum physics and nanophotonics due to various…

Optics · Physics 2021-06-30 Renming Liu , Yi-Cong Yu , Xue-Hua Wang

We simulate the near-field effects of strong coupling between molecular excitons and localized surface plasmons, supported by aluminum nanodisks. The simulations are done using a simple model of a two-level system, implemented in a…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Nadav Fain , Tal Ellenbogen , Tal Schwartz

We provide a simple method that enables readily acquired experimental data to be used to predict whether or not a candidate molecular material may exhibit strong coupling. Specifically, we explore the relationship between the hybrid…

Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition…

The strong interaction of individual quantum emitters with resonant cavities is of fundamental interest for understanding light matter interactions. Plasmonic cavities hold the promise of attaining the strong coupling regime even under…

Optics · Physics 2016-06-28 Kotni Santhosh , Ora Bitton , Lev Chuntonov , Gilad Haran

We study the strong coupling between the molecular excited state and the plasmonic modes of silver hole arrays with a resonant frequency very close to the asymptotic line of the plasmonic dispersion relation, at the nonlinear regime. We…

Mesoscale and Nanoscale Physics · Physics 2017-01-26 Lihi Efremushkin , Maxim Sukharev , Adi Salomon

When two or more metallic nanoparticles are in close proximity, their plasmonic modes may interact through the near field, leading to additional resonances of the coupled system or to shifts of their resonant frequencies. This process is…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

Localized plasmonic modes of metallic nanoparticles may hybridize like those of atoms forming a molecule. However, the rapid decay of the plasmonic fields outside the metal severely limits the range of these interactions to tens of…

Optics · Physics 2013-03-05 Adi Salomon , Yehiam Prior , Radoslaw Kolkowski , Joseph Zyss

We investigate theoretically the photo absorbtion of the cluster of alkali atoms embedded into a single mode quantum microcavity. We show that when the energy of the giant plasmonic resonance lies close to the energy of the cavity mode, the…

Mesoscale and Nanoscale Physics · Physics 2013-03-15 I. G. Savenko , R. G. Polozkov , I. A. Shelykh

Recent years have seen a growing interest in strong coupling between plasmons and excitons, as a way to generate new quantum optical testbeds and influence chemical dynamics and reactivity. Strong coupling to bright plasmonic modes has been…

Mesoscale and Nanoscale Physics · Physics 2020-02-11 Ora Bitton , Satyendra Nath Gupta , Lothar Houben , Michal Kvapil , Vlastimil Křápek , Tomas Šikola , Gilad Haran

Strong light-matter interactions in both the single-emitter and collective strong coupling regimes attract significant attention due to emerging quantum and nonlinear optics applications, as well as opportunities for modifying…

Mesoscale and Nanoscale Physics · Physics 2019-09-11 Tuomas P. Rossi , Timur Shegai , Paul Erhart , Tomasz J. Antosiewicz

Strong light-matter coupling has recently been demonstrated in sub-wavelength volumes by coupling engineered optical transitions in semiconductor heterostructures (e.g., quantum wells) to metasurface resonances via near fields. It has also…

Strong coupling of molecular vibrations with light creates polariton states, enabling control over many optical and chemical properties. However, the near-field signatures of strong coupling are difficult to map as most cavities are closed…

The manipulation of coupled quantum excitations is of fundamental importance in realizing novel photonic and optoelectronic devices. We use electroluminescence to probe plasmon-exciton coupling in hybrid structures consisting of a nanoscale…

We use a recently derived gauge-invariant formulation of the problem of a two-level system coupled to an optical cavity, to explore the transition between the weak, and the ultra-strong coupling regimes of light-matter interaction. We…

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