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Molecular vibrations couple to visible light only weakly, have small mutual interactions, and hence are often ignored for non-linear optics. Here we show the extreme confinement provided by plasmonic nano- and pico-cavities can sufficiently…

Plexciton is the formation of new hybridized energy states originated from the coupling between plasmon and exciton. To reveal the optical properties of both exciton and plexciton, we develop a classic oscillator model to describe the…

Optics · Physics 2022-07-12 Yuqing Cheng , Mengtao Sun

Scattering processes have played a crucial role in the development of quantum theory. In the field of optics, scattering phase shifts have been utilized to unveil interesting forms of light-matter interactions. Here, we investigate the…

We observe strong collective coupling between an optical cavity and the forbidden spin singlet to triplet optical transition $^1$S$_0$ to $^3$P$_1$ in an ensemble of $^{88}$Sr. Despite the transition being 1000 times weaker than a typical…

Atomic Physics · Physics 2016-02-10 Matthew A. Norcia , James K. Thompson

The central theme of cavity quantum electrodynamics is the coupling of a single optical mode with a single matter excitation, leading to a doublet of cavity polaritons which govern the optical properties of the coupled structure. Especially…

Sharp metal corners and tips support plasmons localized on the scale of the curvature radius -- superlocalized plasmons. We analyze plasmonic properties of nanoparticles with small and sharp corner- and tip-shaped surface perturbations in…

Optics · Physics 2016-01-20 M. V. Gorkunov , B. I. Sturman , E. V. Podivilov

We study the interplay between electron-electron interaction and Rashba spin-orbit coupling in the two-dimensional electron gas. Using the random phase approximation we predict new screening properties of the electron gas which result in…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Pletyukhov , V. Gritsev

Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…

Chemical Physics · Physics 2021-09-01 Jacopo Fregoni , Tor S. Haugland , Silvio Pipolo , Tommaso Giovannini , Henrik Koch , Stefano Corni

Plasmon decay via the surface or interface is a critical process for practical energy conversion and plasmonic catalysis. However, the relationship between plasmon damping and the coupling between the plasmon and 2D materials is still…

We study the charge-density dynamics within the two-dimensional extended Hubbard model in the presence of long-range Coulomb interaction across the metal-insulator transition point. To take into account strong correlations we start from…

Strongly Correlated Electrons · Physics 2014-12-24 E. G. C. P. van Loon , H. Hafermann , A. I. Lichtenstein , A. N. Rubtsov , M. I. Katsnelson

We show that a two-component mixture of a few repulsively interacting ultracold atoms in a one-dimensional trap possesses very different quantum regimes and that the crossover between them can be induced by tuning the interactions in one of…

Quantum Gases · Physics 2013-12-10 M. A. Garcia-March , B. Julia-Diaz , G. E. Astrakharchik , Th. Busch , J. Boronat , A. Polls

We investigate the quantum optical properties of a single photon emitter coupled to a finite-size metal nanoparticle using a photon Green function technique that rigorously quantizes the electromagnetic fields. We first obtain pronounced…

Mesoscale and Nanoscale Physics · Physics 2012-02-07 C. Van Vlack , Philip Trøst Kristensen , S. Hughes

We simulate vibrational strong (VSC) and ultrastrong coupling (V-USC) for liquid water with classical molecular dynamics simulations. When the cavity modes are resonantly coupled to the O-H stretch mode of liquid water, the infrared…

Chemical Physics · Physics 2020-07-21 Tao E. Li , Joseph E. Subotnik , Abraham Nitzan

Measurements of interactions between cold molecules and ultracold atoms can allow for a detailed understanding of fundamental collision processes. These measurements can be done using various experimental geometries including where both…

Atomic Physics · Physics 2020-03-25 N. J. Fitch , L. P. Parazzoli , H. J. Lewandowski

Intermolecular interactions are pivotal for aggregation, solvation, and crystallization. We demonstrate that the collective strong coupling of several molecules to a single optical mode results in notable changes in the molecular…

Quantum Physics · Physics 2024-02-19 Matteo Castagnola , Tor S. Haugland , Enrico Ronca , Henrik Koch , Christian Schäfer

We present a detailed study of the electroluminescence of intersubband devices operating in the light-matter strong coupling regime. The devices have been characterized by performing angle resolved spectroscopy that shows two distinct light…

Mesoscale and Nanoscale Physics · Physics 2012-12-27 Pierre Jouy , Angela Vasanelli , Yanko Todorov , Luca Sapienza , Raffaele Colombelli , Ulf Gennser , Carlo Sirtori

The ultrastrong light-matter interaction regime was investigated in metallic and superconducting complementary split ring resonators coupled to the cyclotron transition of two dimensional electron gases. The sub-wavelength light confinement…

The optical responses of structured array of noble-metal nanoparticle dimers immersed in a glass matrix are investigated theoretically, motivated by the recent experimental observation of the splitting of the surface plasmon bands in silver…

Optics · Physics 2007-05-23 J. J. Xiao , J. P. Huang , K. W. Yu

We demonstrate strong coupling between a single J-aggregate and an inverse bowtie plasmonic structure, when the J-aggregate is located at a specific axial distance from the metallic surface. Three hybrid modes are clearly observed,…

Optics · Physics 2021-12-20 Adam Weissman , Maxim Sukharev , Adi Salomon

In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , W. Skomorowski , R. Moszynski , T. Zelevinsky
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