Related papers: High-resolution 'magic'-field spectroscopy on trap…
The collective response of metal nanostructures to optical excitation leads to localized plasmon generation with nanoscale field confinement driving applications in e.g. quantum optics, optoelectronics, and nanophotonics, where a bottleneck…
Atoms in spatially dependent light fields are attracted to local intensity maxima or minima depending on the sign of the frequency difference between the light and the atomic resonance. For light fields confined in open high-Q optical…
We present a rigorous theoretical study of low-temperature collisions of polyatomic molecular radicals with ^1S_0 atoms in the presence of an external magnetic field. Accurate quantum scattering calculations based on ab initio and scaled…
We have demonstrated a high temperature vapor cell for absorption spectroscopy on the Ca intercombination line. The cell uses a dual chamber design to achieve the high temperatures necessary for an optically dense vapor while avoiding the…
Deep laser cooling of atoms, ions, and molecules facilitates the study of fundamental physics as well as applied research. In this work, we report on the narrow-line laser cooling of thulium atoms at the wavelength of $506.2\,\textrm{nm}$…
It is shown that the translational degrees of freedom of a large variety of molecules, from light diatomic to heavy organic ones, can be cooled sympathetically and brought to rest (crystallized) in a linear Paul trap. The method relies on…
We use optical frequency comb Fourier transform spectroscopy to record high-resolution, low-pressure, room-temperature spectra of formaldehyde (H$_2$$^{12}$C$^{16}$O) in the range of 1250 to 1390 cm$^{-1}$. Through line-by-line fitting, we…
Single-photon cooling is a recently introduced method to cool atoms and molecules for which standard methods might not be applicable. We numerically examine this method in a two-dimensional wedge trap as well as in a two-dimensional…
The problem of deep laser cooling of $^{24}$Mg atoms is theoretically studied. We propose two-stage sub-Doppler cooling strategy using electro-dipole transition $3^3P_2$$\to$$3^3D_3$ ($\lambda$=383.9 nm). The first stage implies exploiting…
We demonstrate a novel atom chip trapping system that allows the placement and high-resolution imaging of ultracold atoms within microns from any <100 um-thin, UHV-compatible material, while also allowing sample exchange with minimal…
A computational model study for complete frequency redistribution linear incoherent two-level atomic radiation trapping in optically dense media using the multiple scattering representation is presented. This model study discuss at length…
We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…
We propose and analyze a scheme for sympathetic cooling of the translational motion of polar molecules in an optical lattice, interacting one by one with laser-cooled ions in a radio-frequency trap. The energy gap between the excitation…
Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…
A new scheme of three-dimensional (3D) all-optical (nonmagnetic) cooling and trapping of resonant atoms, based on using of so-called rectified radiation forces in non-monochromatic light fields is presented. It can be applied to the atoms…
We propose a laser cooling technique in which atoms are selectively excited to a dressed metastable state whose light shift and decay rate are spatially correlated for Sisyphus cooling. The case of cooling magnetically trapped…
We present a versatile electric trap for the exploration of a wide range of quantum phenomena in the interaction between polar molecules. The trap combines tunable fields, homogeneous over most of the trap volume, with steep gradient fields…
We present experimental results from a new scheme for magneto-optically trapping strontium monofluoride (SrF) molecules, which provides increased confinement compared to our original work. The improved trap employs a new approach to…
We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…
Using first-principles calculations, we identify magic wavelengths for the 2s-2p and 2s-3p transitions in lithium. The ns and np atomic levels have the same ac Stark shifts at the corresponding magic wavelength, which facilitates…