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We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$…

Atomic Physics · Physics 2018-07-11 D. J. McCarron , M. H. Steinecker , Y. Zhu , D. DeMille

In the early days of laser spectroscopy Letokhov and Chebotayev proposed a scheme for measuring narrow spectral lines where the resolution is not restricted to Doppler effects because the molecules are entrained in a standing-wave light…

Diatomic polar molecules are one of the most promising platforms of quantum computing due to their rich internal states and large electric dipole moments. Here, we propose entangling rotational states of adjacent polar molecules via a…

Atomic Physics · Physics 2021-05-07 Eunmi Chae

A special class of molecules that are important to many subfields in molecular dynamics and chemical physics, namely free radical molecules, now enjoy a significant degree of center-of-mass motion control in the laboratory frame. The…

Atomic Physics · Physics 2009-11-10 J. R. Bochinski , Eric R. Hudson , H. J. Lewandowski , Jun Ye

Understanding collisions between ultracold molecules is crucial for making stable molecular quantum gases and harnessing their rich internal degrees of freedom for quantum engineering. Transient complexes can strongly influence collisional…

A recent expansion of cold and ultracold molecule applications has led to renewed focus on molecular species preparation under ultrahigh vacuum conditions. Meanwhile, molecular beams have been used to study gas phase chemical reactions for…

Atomic Physics · Physics 2016-02-23 M. G. Kokish , V. Rajagopal , J. P. Marler , B. C. Odom

Simultaneous two-dimensional trapping of neutral dipolar molecules in low- and high-field seeking states is analyzed. A trapping potential of the order of 20 mK can be produced for molecules like ND3 with time-dependent electric fields. The…

Chemical Physics · Physics 2009-11-10 T. Junglen , T. Rieger , S. A. Rangwala , P. W. H. Pinkse , G. Rempe

A detailed treatment of an electro-optical trap for polar molecules, realized by embedding an optical trap within a uniform electrostatic field, is presented and the trap's properties analyzed and discussed. The electro-optical trap offers…

Atomic Physics · Physics 2022-06-15 Bretislav Friedrich

Under the local plasmonic excitation, the Raman images of a single molecule can now reach sub-nanometer resolution. We report here a theoretical description of the interaction between a molecule and a highly confined plasmonic field. It is…

Mesoscale and Nanoscale Physics · Physics 2015-08-06 Sai Duan , Guangjun Tian , Yongfei Ji , Jiushu Shao , Zhenchao Dong , Yi Luo

We propose a method for sensitive parallel detection of low-frequency electromagnetic fields based on the fine structure interactions in paramagnetic polar molecules. Compared to the recently implemented scheme employing ultracold $^{87}$Rb…

Atomic Physics · Physics 2013-04-25 Sergey V. Alyabyshev , Mikhail Lemeshko , Roman V. Krems

Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule…

Atomic Physics · Physics 2015-06-12 Jun-Ren Chen , Cheng-Yang Kao , Hung-Bin Chen , Yi-Wei Liu

We propose a novel type of precision laser spectrometer for trapped, highly charged ions nearly at rest. It consists of a cylindrical open-endcap Penning trap in which an externally produced bunch of highly charged ions can be confined and…

Atomic Physics · Physics 2009-11-11 M. Vogel , D. F. A. Winters , D. M. Segal , R. C. Thompson

We propose and demonstrate the laser cooling and trapping of Rydberg-dressed Sr atoms. By off-resonantly coupling the excited state of a narrow (7 kHz) cooling transition to a high-lying Rydberg state, we transfer Rydberg properties such as…

Atomic Physics · Physics 2018-05-09 A. D. Bounds , N. C. Jackson , R. K. Hanley , R. Faoro , E. M. Bridge , P. Huillery , M. P. A. Jones

The electronic energy level structure of yttrium monoxide (YO) provides a long-lived, low-lying $^{2}\Delta$ state ideal for high-precision molecular spectroscopy, narrowline laser cooling at the single photon-recoil limit, and studying…

Optical dipole-traps are used in various scientific fields, including classical optics, quantum optics and biophysics. Here, we propose and implement a dipole-trap for nanoparticles that is based on focusing from the full solid angle with a…

We study theoretically light propagations at the zigzag edge of a honeycomb photonic crystal consisting of dielectric rods in air, analogous to graphene. Within the photonic band gap of the honeycomb photonic crystal, a unimodal edge state…

Mesoscale and Nanoscale Physics · Physics 2012-12-27 Chunfang Ouyang , Dezhuan Han , Fangyuan Zhao , Xinhua Hu , Xiaohan Liu , Jian Zi

A recent progress on laser cooling of molecules is summarized. Since the development during 1980s for atomic species, laser cooling has been the very beginning step to cool and trap atoms for frontier research on quantum simulations,…

Atomic Physics · Physics 2023-03-29 Eunmi Chae

We explore the feasibility of optically forming long-range tetratomic and larger polyatomic molecules in their ground electronic state from ultracold pairs of polar molecules aligned by external fields. Depending on the relative orientation…

Atomic Physics · Physics 2021-06-16 Marko Gacesa , Jason N. Byrd , Jonathan Smucker , John A. Montgomery, , Robin Côté

We report on the creation and characterization of heteronuclear KRb Feshbach molecules in an optical dipole trap. Starting from an ultracold gas mixture of K-40 and Rb-87 atoms, we create as many as 25,000 molecules at 300 nK by rf…

Other Condensed Matter · Physics 2008-08-22 J. J. Zirbel , K. -K. Ni , S. Ospelkaus , T. L. Nicholson , M. L. Olsen , C. E. Wieman , J. Ye , D. S. Jin , P. S. Julienne

We demonstrate a laser frequency stabilization technique for laser cooling of Potassium atoms, based on saturated absorption spectroscopy in the C-Band optical telecommunication window, using ro-vibrationel transitions of the acetylene…

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