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Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…

Atomic Physics · Physics 2026-02-17 Aleksandr V. Boitsov , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT…

We investigate theoretically a nuclear excitation mechanism involving absorption of non-resonant photons leveraged by the coupling to the atomic shell. The nuclear non-resonant photoexcitation is assisted by electron recombination which…

Nuclear Theory · Physics 2026-04-28 Nan Xue , Zuoye Liu , Ziwen Li , Adriana Pálffy , Jianmin Yuan , Yuanbin Wu , Xiangjin Kong , Yu-Gang Ma

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant…

Atomic Physics · Physics 2018-10-03 J. Fedyk , A. B. Voitkiv , C. Müller

We present experimental results for the ionization of aniline and benzene molecules subjected to intense ultrashort laser pulses. Measured parent molecular ions yields were obtained using a recently developed technique capable of…

We present the results of the detailed experimental study of multiple ionization of Ne and Ar by 25 and 7 fs laser pulses. For Ne the highly correlated "instantaneous" emission of up to four electrons is triggered by a recollisional…

Atomic Physics · Physics 2009-11-10 A. Rudenko , K. Zrost , B. Feuerstein , V. L. B. de Jesus , C. D. Schröter , R. Moshammer , J. Ullrich

We present an experimental and theoretical energy- and angle-resolved study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral N$_2$ molecules. Using 9.3 eV photons produced via high…

The present tutorial provides an overview of the time-dependent configuration interaction singles (\acs{TDCIS}) scheme applied to nonlinear ionization over a broad photon-energy range. The efficient propagation of the wave function and the…

Quantum Physics · Physics 2017-02-09 Antonia Karamatskou

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…

Absolute cross-section measurements for valence-shell photoionization of Ar$^{+}$ ions are reported for photon energies ranging from 27.4 eV to 60.0 eV. The data, taken by merging beams of ions and synchrotron radiation at a photon energy…

We present a theoretical study of atomic laser-assisted photoionization emission (LAPE). We consider an atom driven by a linearly polarized XUV laser in two different scenarios: i) a single attosecond pulse (in both the streaking and…

Atomic Physics · Physics 2020-10-21 Renata Della Picca , Marcelo F. Ciappina , Maciej Lewenstein , Diego G. Arbó

We present a detailed experimental and theoretical study on the relativistic non-dipole effects in strong-field atomic ionisation by near-infrared linearly-polarised few-cycle laser pulses in the intensity range 1014 -1015 W/cm2. We record…

We have unveiled coherent multiphoton interferences originating from different quantum paths taken by the Auger electron induced by a high-intensity x-ray/XUV pulse under the presence of a strong optical field. These interferences give rise…

Quantum Physics · Physics 2015-07-03 Antonio Picón , Phay J. Ho , Gilles Doumy , Stephen H. Southworth

Atoms ionization by the simultaneous absorption of multiple photons has found applications in fiber optics, where it leads to unique nonlinear phenomena. To date, studies of the ionization regime have been limited to gas-filled hollow-core…

The analytical structure and absolute values of the generalized cross-section of the two-photon resonance single ionization of the K-shell of a heavy neon-like ion of an iron atom (Fe$^{16+}$) were theoretically predicted. A pronounced…

We present numerical simulations of ultrafast multiphoton ionization dynamics in a two-dimensional atomic model driven by co- and counterrotating circularly polarized single-color and bichromatic carrier envelope phase (CEP) stable…

Atomic Physics · Physics 2020-07-15 T. Bayer , Ch. Philipp , K. Eickhoff , M. Wollenhaupt

Highly excited eigenstates of atoms and ions with open f shell are chaotic superpositions of thousands, or even millions of Hartree-Fock determinant states. The interaction between dielectronic and multielectronic configurations leads to…

Atomic Physics · Physics 2015-06-17 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin , C. Harabati , M. G. Kozlov

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

We study time-delays in atomic multiphoton ionization (MPI) using the phase-sensitive detection of photoelectron vortices. Photoelectron vortices are created by MPI with counter-rotating circularly polarized (CRCP) ultrashort double pulse…

Atomic Physics · Physics 2025-01-13 D. Köhnke , T. Bayer , M. Wollenhaupt

Detection of nascent O($^3P_j$, $j=2,1,0$) atoms using one-photon resonant excitation to the $3s\,^3S^o_1$ state at $\sim 130$ nm followed by near-threshold ionization, i. e., 1 + 1' resonance enhanced multi-photon ionization (REMPI), has…