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We have investigated multiphoton multiple ionization dynamics of argon and xenon atoms using a new x-ray free electron laser (XFEL) facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that highly charged…

We present a multichannel photoelectron interferometry technique based on trichromatic pulse shaping for unambiguous determination of quantum phases in multiphoton ionization (MPI) of potassium atoms. The colors of the laser field are…

Atomic Physics · Physics 2022-05-25 K. Eickhoff , D. Köhnke , L. Feld , T. Bayer , M. Wollenhaupt

High-resolution photoelectron momentum distributions of Xe atoms ionized by 800-nm linearly polarized laser fields have been traced at intensities from 1.1*1013 to 3.5*1013W/cm2 using velocity-map imaging techniques. At certain laser…

Atomic Physics · Physics 2015-12-09 Min Li , Peng Zhang , Siqiang Luo , Yueming Zhou , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We report the observation of multiple ionization of Argon through multi-XUV-photon absorption induced by an unprecedentedly powerful laser driven high-harmonic-generation source. Comparing the measured intensity dependence of the yield of…

Resonance-enhanced multiphoton ionization (REMPI) is a widely used technique for studying molecular photoionization and producing molecular cations for spectroscopy and dynamics studies. Here, we present a model for describing…

Chemical Physics · Physics 2016-08-24 Matthias Germann , Stefan Willitsch

In this paper, we theoretically study x-ray multiphoton ionization dynamics of heavy atoms taking into account relativistic and resonance effects. When an atom is exposed to an intense x-ray pulse generated by an x-ray free-electron laser…

Atomic Physics · Physics 2017-04-26 Koudai Toyota , Sang-Kil Son , Robin Santra

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

Resonance-enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the…

Atomic Physics · Physics 2025-03-10 Wankai Li , Yixuan Wang , Xing Li , Tao Yang , Dongdong Zhang , Dajun Ding

Using Resonant Pulsed Rydberg Field-ionization (RPRFI) technique, we generate low-energy electron bunches at high repetition rates. By combining continuous-wave laser excitation with a pulsed electric field, this method selectively ionizes…

Atomic Physics · Physics 2024-01-10 R. Hahn , D. Comparat

A simple model for sequential multiphoton ionization by ultra-intense x-rays is presented. The derived scaling of the ion yield with pulse energy quantitatively reproduces the experimental data, which shows that the ion yield increases…

Atomic Physics · Physics 2021-09-29 Xiang Li , Rebecca Boll , Daniel Rolles , Artem Rudenko

We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are…

The production of high-quality electron bunches in Laser Wake Field Acceleration relies on the possibility to inject ultra-low emittance bunches in the plasma wave. In this paper we present a new bunch injection scheme in which electrons…

We theoretically study the process of photoelectron emission of the Helium atom by a high-intensity short-wavelength laser at a resonance condition of the residual singly charged ion. Photoionization followed by strong resonance coupling in…

Atomic Physics · Physics 2014-01-14 Song Bin Zhang , Nina Rohringer

Recently a new injection scheme for Laser Wake Field Acceleration, employing a single 100-TW-class laser system, has been proposed. In the Resonant Multi-Pulse Ionization injection (ReMPI) a resonant train of pulses drives a large amplitude…

Accelerator Physics · Physics 2018-12-26 P. Tomassini , S. De Nicola , L. Labate , P. Londrillo , R. Fedele , D. Terzani , F. Nguyen , G. Vantaggiato , L. A. Gizzi

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

We report on efficient rovibrational state-selective loading of single H$_2^+$ molecular ions into a cryogenic linear Paul trap using (2+1) resonance-enhanced multi-photon ionization (REMPI). The H$_2^+$ ions are created by resonant…

Atomic Physics · Physics 2026-05-05 Ho June Kim , Fabian Schmid , David Holzapfel , Daniel Kienzler

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

Atomic Physics · Physics 2015-05-27 C. Müller , A. B. Voitkiv

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light-matter interaction was, so far, not studied…

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

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