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Atom-like defects in hexagonal boron nitride (hBN) provide room-temperature single-photon emission and coherent spin states, making them attractive for quantum-computing and -sensing applications. However, their random spatial and spectral…

The photon statistics of CdSe/CdS dot-in-rods nanocrystals is studied with a method involving post-selection of the photon detection events based on the photoluminescence count rate. We show that flickering between two states needs to be…

Quantum Physics · Physics 2015-02-09 M. Manceau , S. , Vezzoli , Q. Glorieux , F. Pisanello , E. Giacobino , L. Carbone , M. De Vittorio , A. Bramati

Quantum emitters in hexagonal boron nitride (hBN) are emerging as bright and robust sources of single photons for applications in quantum optics. In this work we present detailed studies on the limiting factors to achieve Fourier Transform…

Hexagonal boron nitride (hBN) hosts robust room-temperature single-photon emitters, yet their coherence is typically limited by phonon induced dephasing and spectral broadening. Here, we show that thermally induced curvature in bulk like…

We report first-principles calculations of the effects of quasiparticle self-energy and electron-hole interaction on the optical properties of single-walled BN nanotubes. Excitonic effects are shown to be even more important in BN nanotubes…

Materials Science · Physics 2007-08-23 Cheol-Hwan Park , Catalin D. Spataru , Steven G. Louie

Single-photon emitters play a key role in present and emerging quantum technologies. Several recent measurements have established monolayer WSe$_2$ as a promising candidate for a reliable single photon source. The origin and underlying…

Mesoscale and Nanoscale Physics · Physics 2019-10-09 L. Linhart , M. Paur , V. Smejkal , J. Burgdörfer , T. Mueller , F. Libisch

In this study, we employ a first-principles approach to conduct a comprehensive investigation of the properties of nine common native point defects in cubic boron nitride. This analysis combines standard semi-local and dielectric hybrid…

Materials Science · Physics 2024-02-14 Ngoc Linh Nguyen , Hung The Dang , Tien Lam Pham , Thi Minh Hoa Nghiem

Single photon emitters in hexagonal boron nitride are based on fluorescent point-like defects. These defects typically have exceptional photophysical properties and therefore been the focus of extensive research due to their potential to…

Key properties of nine possible defect sites in hexagonal boron nitride (h-BN) are predicted using density-functional theory and are corrected by applying results from high-level ab initio calculations. Observed h-BN electron-paramagnetic…

Computational Physics · Physics 2018-02-12 A. Sajid , Jeffrey R. Reimers , Michael J. Ford

Rhombohedral boron nitride (rBN) is an emerging wide-bandgap van der Waals (vdW) material that combines strong second-order nonlinear optical properties with the structural flexibility of layered 2D systems. Here we show that rBN hosts…

Boron nitride single layer belongs to the family of 2D materials whose optical properties are currently receiving considerable attention. Strong excitonic effects have already been observed in the bulk and still stronger effects are…

The deterministic production of single-photons from two dimensional materials promises to usher in a new generation of photonic quantum devices. In this work, we outline criteria by which single-photon emission can be realised in two…

Mesoscale and Nanoscale Physics · Physics 2020-08-27 Joshua J. P. Thompson , Samuel Brem , Hanlin Fang , Joey Frey , Saroj P. Dash , Witlef Wieczorek , Ermin Malic

Radiative defects in hexagonal boron nitride (hBN) are active in a broad spectral range from deep ultraviolet to near-infrared wavelengths. Representatives of these defects act as bright single photon sources, spin-1 systems, and…

Electron spins coupled with optical transitions in solids stand out as a promising platform for developing spin-based quantum technologies. Recently, hexagonal boron nitride (hBN) - a layered Van der Waals (vdW) crystal, has emerged as a…

Boron nitride exhibits diverse crystal structures, predominantly a layered arrangement with strong intraplanar covalent bonds and weak interplanar van der Waals bonds. While commonly referred to as hexagonal BN (hBN), the sp$^2$-bonded BN…

Point defects in solid-state quantum systems are vital for enabling single-photon emission at specific wavelengths, making their precise identification essential for advancing applications in quantum technologies. However, pinpointing the…

Materials Science · Physics 2025-03-03 Chanaprom Cholsuk , Asli Cakan , Volker Deckert , Sujin Suwanna , Tobias Vogl

Hexagonal boron nitride (hBN) is an emerging material for use in quantum technologies, hosting bright and stable single photon emitters (SPEs). The B-center is one promising SPE in hBN, due to the near-deterministic creation methods and…

Materials Science · Physics 2025-02-24 Evan Williams , Angus Gale , Jake Horder , Dominic Scognamiglio , Milos Toth , Igor Aharonovich

Microcavity exciton-polaritons are two-dimensional bosonic quasiparticles composed by excitons and photons. Using model Hamiltonian with parameters generated from ab initio density-functional theory and Bathe-Salpeter Equation calculations,…

Materials Science · Physics 2021-12-01 Huaiyuan Yang , Xinqiang Wang , Xin-Zheng Li

Optically addressable defect qubits in wide band gap materials are favorable candidates for room temperature quantum information processing. The two-dimensional (2D) hexagonal boron nitride (hBN) is an attractive solid state platform with a…

Materials Science · Physics 2024-09-10 Song Li , Anton Pershin , Adam Gali

Hexagonal boron nitride is rapidly gaining interest as a platform for photonic quantum technologies, due to its two-dimensional nature and its ability to host defects deep within its large band gap that may act as room-temperature…