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We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom,…

Atomic Physics · Physics 2020-02-19 A. Eckey , A. B. Voitkiv , C. Müller

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

Atomic Physics · Physics 2015-05-27 C. Müller , A. B. Voitkiv

Ionization is one of the basic physical processes, occurring when charged particles penetrate atomic matter. When atoms are bombarded by very dense and compact beams of extreme relativistic electrons, two qualitatively new -- and very…

Atomic Physics · Physics 2025-10-07 S. Kim , C. Müller , A. B. Voitkiv

The balance of the linear photon momentum in multiphoton ionization is studied experimentally. In the experiment argon and neon atoms are singly ionized by circularly polarized laser pulses with a wavelength of 800 nm and 1400 nm in the…

Optics · Physics 2011-06-01 C Smeenk , L Arissian , B Zhou , A Mysyrowicz , D M Villeneuve , A Staudte , P B Corkum

The feasibility of complete photoionization experiments, in which the full set of photoionization matrix elements are determined, using multiphoton ionization schemes with polarization-shaped pulses has recently been demonstrated [Hockett…

Atomic Physics · Physics 2015-07-22 P. Hockett , M. Wollenhaupt , C. Lux , T. Baumert

Nonsequential two-photon ionization of inner-shell $np$ subshell of neutral atoms by circularly polarized light is investigated. Detection of subsequent fluorescence as a signature of the process is proposed and the dependence of…

Atomic Physics · Physics 2019-07-17 J. Hofbrucker , A. V. Volotka , S. Fritzsche

Intense laser ionization expands Einstein's photoelectric effect rules giving a wealth of phenomena widely studied over the last decades. In all cases, so far, photons were assumed to carry one unit of angular momentum. However it is now…

Quantum Physics · Physics 2010-02-09 A. Picón , J. Mompart , J. R. Vázquez de Aldana , L. Plaja , G. F. Calvo , L. Roso

We measure the absolute absorption cross section of molecules using a matter-wave interferometer. A nanostructured density distribution is imprinted onto a dilute molecular beam through quantum interference. As the beam crosses the light…

Quantum Physics · Physics 2014-08-20 Sandra Eibenberger , Xiaxi Cheng , J. P. Cotter , Markus Arndt

The photoionization of a two-shell endohedral A@CN1@CN2 is considered. Formulas are presented for cross-sections and angular anisotropy parameters, both dipole and non-dipole. The effect of the fullerenes shell upon photoelectron from atom…

Atomic and Molecular Clusters · Physics 2013-05-29 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

We show that interference phenomena plays a big role for the electron yield in ionization of atoms by an ultra-short laser pulse. Our theoretical study of single ionization of atoms driven by few-cycles pulses extends the photoelectron…

Quantum Physics · Physics 2009-11-13 Diego Arbo , Emil Persson , Joachim Burgdoerfer

Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…

Atomic Physics · Physics 2021-02-03 Joss Wiese , Jolijn Onvlee , Sebastian Trippel , Jochen Küpper

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

Multi-photon absorption is a well-known phenomenon. With atom lasers a similar process could take place for massive particles, the ionization of an atom or molecule by the successive interaction with various particles. This process would…

Quantum Physics · Physics 2009-11-13 Pedro Sancho

Shape resonances in photoionization of atoms and molecules arise from a particular geometry of the ionic potential which traps the receding photoelectron in a quasi-bound state in a particular partial wave. This mechanism allows us to…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets , Stephen Catsamas

Partial polarization is the manifestation of the correlation between two mutually orthogonal transverse field components associated with a light beam. We show both theoretically and experimentally that the origin of this correlation can be…

Absorption spectroscopy is a fundamental tool for probing molecular structure. However, performing absorption spectroscopy on individual molecules is challenging due to the low signal-to-noise ratio. Here, we report on a nondestructive…

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…