English
Related papers

Related papers: Complete characterization of multi-channel single …

200 papers

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

We report on a kinematically complete experiment on strong field double ionization of helium using laser pulses with a wavelength of 394\,nm and intensities of $3.5-5.7\times10^{14}\,W/cm^2$. Our experiment reaches the most complete level…

Many atomic processes result in the emission of photons. Analysis of the properties of emitted photons, such as energy and angular distribution as well as polarization, is regarded as a powerful tool for gaining more insight into the…

Atomic Physics · Physics 2018-04-18 V. A. Zaytsev , A. S. Surzhykov , V. M. Shabaev , Th. Stöhlker

We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…

Optics · Physics 2017-11-22 Jan Marcus Dahlström , Stefan Pabst , Eva Lindroth

We develop a wave packet molecular dynamics framework for modeling the structural properties of partially-ionized dense plasmas, based on a chemical model that explicitly includes bound state wavefunctions. Using hydrogen as a…

We present a complete polarization characterization of any quantum state of two orthogonal polarization modes, and give a systematic measurement procedure to collect the necessary data. Full characterization requires measurements of the…

Quantum Physics · Physics 2015-06-11 Jonas Soderholm , Gunnar Bjork , Andrei B. Klimov , Luis L. Sanchez-Soto , Gerd Leuchs

Amplitude and phase of wavepackets encode the dynamics of quantum systems. However, the rapidity of electron dynamics on the attosecond timescale has precluded their complete measurement in the time domain. Here, we demonstrate that…

The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…

Atomic Physics · Physics 2012-06-26 Philipp V Demekhin , Lorenz S Cederbaum

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

Single and multi-photon ionization of aligned molecular ensembles is examined, with a particular focus on the link between the molecular axis distribution and observable in various angle-integrated and angle-resolved measurements. To…

Chemical Physics · Physics 2015-03-04 Paul Hockett

We present momentum resolved covariance measurements of entangled electronic-nuclear wave packets created and probed with octave spanning phaselocked ultrafast pulses. We launch vibrational wave packets on multiple electronic states via…

Quantum Physics · Physics 2023-11-20 Gonenc Mogol , Brian Kaufman , Chuan Cheng , Itzik Ben-Itzhak , Thomas Weinacht

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

Mathematical Physics · Physics 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

Multiphoton ionization provides a clear window into the nature of electron correlations in the helium atom. In the present study, the final state energy range extends up to the region near the $N=2$ and $N=3$ ionization thresholds, where…

Atomic Physics · Physics 2021-03-10 Yimeng Wang , Chris H. Greene

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu

This is a sequel to an earlier article on the theory of angular correlation for double photoionization. Here we consider the two-step double photoionization of a rare gas atom under the influence of a polarized photon beam described by…

Atomic Physics · Physics 2009-11-07 Chiranjib Sur , Dipankar Chattarji

Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…

Atomic Physics · Physics 2022-02-24 A. Plunkett , M. A. Alarcon , J. K. Wood , C. H. Greene , A. Sandhu

We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…

Atomic Physics · Physics 2018-04-03 Ruihua Xu , Zhaoyan Zhou , Xu Wang

We present a rather elaborate theoretical model describing the dynamics of Neon under radiation of photon energies $\sim 93$ eV and pulse duration in the range of 15 fs, within the framework of Lowest non-vanishing Order of Perturbation…

Atomic Physics · Physics 2015-06-18 G. M. Nikolopoulos , P. Lambropoulos

Observing the motion of the nuclear wavepackets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational…

When polarized light is absorbed by an atom, the excited atomic system carries information about the initial polarization of light. For the light that carries an orbital angular momentum, or the twisted light, the polarization states are…

Quantum Physics · Physics 2020-05-18 Andrei Afanasev , Carl E. Carlson , Hao Wang