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Various properties of interlayer excitons in double-layer transition metal dichalcogenides quantum dots are analyzed using a low-energy effective Hamiltonian with Coulomb interaction. We solve the single-particle Hamiltonian with and…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Xiang Liu , Zheng Tao , Wenchen Luo , Tapash Chakraborty

We use helicity-resolved ultrafast transient absorption spectroscopy to study spin-valley polarization dynamics in a vertically stacked MoSe$_{2}$/WSe$_{2}$ heterostructure. The experimental findings reveal details of interlayer charge…

Light emission from higher-order correlated excitonic states has been recently reported in hBN-encapsulated monolayer WSe2 and WS2 upon optical excitation. These exciton complexes are found to be bound states of excitons residing in…

Mesoscale and Nanoscale Physics · Physics 2019-04-19 Matthias Paur , Aday J. Molina-Mendoza , Rudolf Bratschitsch , Kenji Watanabe , Takashi Taniguchi , Thomas Mueller

Monolayers (MLs) of MoS2 and WSe2 are 2D semiconductors with strong, direct optical transitions that are governed by tightly Coulomb bound eletron-hole pairs (excitons). The optoelectronic properties of these transition metal…

Materials Science · Physics 2015-03-06 G. Wang , X. Marie , I. Gerber , T. Amand , D. Lagarde , L. Bouet , M. Vidal , A. Balocchi , B. Urbaszek

Using first-principles calculations within density functional theory, we investigate the intrinsic spin Hall effect in monolayers of group-VI transition-metal dichalcogenides MX2 (M = Mo, W and X = S, Se). MX2 monolayers are direct band-gap…

Materials Science · Physics 2012-10-10 Wanxiang Feng , Yugui Yao , Wenguang Zhu , Jinjian Zhou , Wang Yao , Di Xiao

We show that excitonic resonances and interexciton transitions can enhance the probability of spontaneous parametric down-conversion, a second-order optical response which generates entangled photon pairs. We benchmark our ab initio…

Computational Physics · Physics 2024-06-18 Fengyuan Xuan , MingRui Lai , Yaze Wu , Su Ying Quek

We report that an external electric field applied normal to bilayers of transition-metal dichalcogenides TX2, M = Mo, W, X = S, Se, creates significant spin-orbit splittings and reduces the electronic band gap linearly with the field…

Materials Science · Physics 2015-06-22 Nourdine Zibouche , Pier Philipsen , Agnieszka Kuc , Thomas Heine

More than fifty years ago, excitonic insulators, formed by the pairing of electrons and holes due to Coulomb interactions, were first predicted. Since then, excitonic insulators have been observed in various classes of materials, including…

An inverse spin Hall effect (ISHE) in n-type silicon was observed experimentally when conduction electrons were scattered on the spin-orbit potential of bismuth. The spin current in the silicon layer was generated by excitation of the…

Mesoscale and Nanoscale Physics · Physics 2020-05-27 A. A. Ezhevskii , D. V. Guseinov , A. V. Soukhorukov , A. V. Novikov , D. V. Yurasov , N. S. Gusev

Spin or valley degrees of freedom in condensed matter have been proposed as efficient information carriers towards next generation spintronics. It is therefore crucial to develop effective strategies to generate and control spin or…

Mesoscale and Nanoscale Physics · Physics 2023-04-26 Ying Shi , Yusong Gan , Yuzhong Chen , Yubin Wang , Sanjib Ghosh , Alexey Kavokin , Qihua Xiong

Bose-Fermi mixtures naturally appear in various physical systems. In semiconductor heterostructures, such mixtures can be realized, with bosons as excitons and fermions as dopant charges. However, the complexity of these hybrid systems…

Van der Waals heterostructures composed of transition metal dichalcogenide monolayers (TMDs) are characterized by their truly rich excitonic properties which are determined by their structural, geometric and electronic properties: In…

The electronic states at the direct band gap of monolayer WSe2 at the $K^+$ and $K^-$ valleys are related by time reversal and may be viewed as pseudo-spins. The corresponding optical interband transitions are governed by robust excitons.…

Materials Science · Physics 2015-09-16 G. Wang , M. M. Glazov , C. Robert , T. Amand , X. Marie , B. Urbaszek

Because of the reduced dielectric screening and enhanced Coulomb interactions, two-dimensional (2D) materials like phosphorene and transition metal dichalcogenides (TMDs) exhibit strong excitonic effects, resulting in fascinating…

Materials Science · Physics 2019-11-04 Xiaoyang Zheng , Xian Zhang

We introduce density imbalanced electron-hole bilayers at a commensurate 2 : 1 density ratio as a platform for realizing novel phases involving electrons, excitons and trions. Three length scales are identified which characterize the…

Strongly Correlated Electrons · Physics 2024-05-28 David D. Dai , Liang Fu

Transition metal dichalcogenides (TMDCs) heterostructure with a type II alignment hosts unique interlayer excitons with the possibility of spin-triplet and spin-singlet states. However, the associated spectroscopy signatures remain elusive,…

Moir\'e superlattices in transition-metal dichalcogenide semiconductor heterobilayers enable the quantum confinement of interlayer excitons with large out-of-plane permanent electric dipoles and spin-valley control. Here, we report a novel…

Transition metal dichalcogenides integrated within a high-quality microcavity support well-defined exciton polaritons. While the role of intralayer excitons in 2D polaritonics is well studied, interlayer excitons have been largely ignored…

Mesoscale and Nanoscale Physics · Physics 2022-12-07 Jonas K. König , Jamie M. Fitzgerald , Joakim Hagel , Daniel Erkensten , Ermin Malic

We report on small-cluster exact-diagonalization calculations which prove the formation of electron-hole pairs (excitons) as prerequisite for spontaneous interlayer phase coherence in bilayer systems described by the extended…

Strongly Correlated Electrons · Physics 2013-07-25 T. Kaneko , S. Ejima , H. Fehske , Y. Ohta

We present a comprehensive investigation of optical properties in MoSe$_2$/CrSBr heterostructures, unveiling the presence of localized excitons represented by a new emission feature, X$^*$. We demonstrate through temperature- and…

Mesoscale and Nanoscale Physics · Physics 2024-05-28 Xinyue Huang , Zhigang Song , Yuchen Gao , Pingfan Gu , Kenji Watanabe , Takashi Taniguchi , Shiqi Yang , Zuxin Chen , Yu Ye
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