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We report on the theoretical and experimental investigation of valley-selective optical Stark and Bloch-Siegert shifts of exciton resonances in monolayers WSe$_2$ and MoS$_2$ induced by strong circularly polarized nonresonant optical…

Mesoscale and Nanoscale Physics · Physics 2022-12-13 A. O. Slobodeniuk , P. Koutenský , M. Bartoš , F. Trojánek , P. Malý , T. Novotný , M. Kozák

High degree of valley polarization of optically active excitons in transition-metal dichalcogenide monolayers (TMD-MLs) is vital in valley-based photonic applications but known to be likely spoiled by the intrinsic electron-hole exchange…

Mesoscale and Nanoscale Physics · Physics 2021-06-15 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

The rapidly growing class of atomically thin and tunable van der Waals materials is intensely investigated both in the context of fundamental science and for new technologies. There is in this connection a widespread need for new ways to…

Mesoscale and Nanoscale Physics · Physics 2026-04-28 Shanshan Ding , Jose Antonio Valerrama Botia , Aleksi Julku , Zhigang Wu , G. M. Bruun

Excitons in atomically-thin semiconductors necessarily lie close to a surface, and therefore their properties are expected to be strongly influenced by the surrounding dielectric environment. However, systematic studies exploring this role…

Mesoscale and Nanoscale Physics · Physics 2016-12-06 Andreas V. Stier , Nathan P. Wilson , Genevieve Clark , Xiaodong Xu , Scott A. Crooker

Spin-valley coupling in monolayer transition metal dichalcogenides gives rise to valley polarization and coherence effect, limited by intervalley scattering caused by exciton-phonon, exciton-impurity, and electron-hole exchange interaction…

The optical spectra of vertically stacked MoSe$_2$/WSe$_2$ heterostructures contain additional 'interlayer' excitonic peaks that are absent in the individual monolayer materials and exhibit a significant spatial charge separation in…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Roland Gillen

Excitonic states trapped in harmonic moir\'e wells of twisted heterobilayers is an intriguing testbed. However, the moir\'e potential is primarily governed by the twist angle, and its dynamic tuning remains a challenge. Here we demonstrate…

Based on \emph{ab initio} theoretical calculations of the optical spectra of vertical heterostructures of MoSe$_2$ (or MoS$_2$) and WSe$_2$ sheets, we reveal two spin-orbit-split Rydberg series of excitonic states below the \textsl{A}…

Mesoscale and Nanoscale Physics · Physics 2018-04-18 Roland Gillen , Janina Maultzsch

Excitons are elementary optical excitation in semiconductors. The ability to manipulate and transport these quasiparticles would enable excitonic circuits and devices for quantum photonic technologies. Recently, interlayer excitons in 2D…

Mesoscale and Nanoscale Physics · Physics 2022-04-06 Ruoming Peng , Adina Ripin , Yusen Ye , Jiayi Zhu , Changming Wu , Seokhyeong Lee , Huan Li , Takashi Taniguchi , Kenji Watanabe , Ting Cao , Xiaodong Xu , Mo Li

A new degree of freedom, the valley pseudospin, emerges in atomically thin two-dimensional transition metal dichalcogenides (MX2) and has attracted great scientific interest. The capability to manipulate the valley pseudospin, in analogy to…

Mesoscale and Nanoscale Physics · Physics 2014-12-10 Jonghwan Kim , Xiaoping Hong , Chenhao Jin , Su-Fei Shi , Chih-Yuan S. Chang , Ming-Hui Chiu , Lain-Jong Li , Feng Wang

Optical excitations in moir\'e transition metal dichalcogenide bilayers lead to the creation of excitons, as electron-hole bound states, that are generically considered within a Bose-Hubbard framework. Here, we demonstrate that these…

Mesoscale and Nanoscale Physics · Physics 2024-05-03 Tsung-Sheng Huang , Peter Lunts , Mohammad Hafezi

In monolayers of semiconducting transition metal dichalcogenides, the light helicity ($\sigma^+$ or $\sigma^-$) is locked to the valley degree of freedom, leading to the possibility of optical initialization of distinct valley populations.…

Mesoscale and Nanoscale Physics · Physics 2016-05-25 T. Smoleński , M. Goryca , M. Koperski , C. Faugeras , T. Kazimierczuk , K. Nogajewski , P. Kossacki , M. Potemski

Photonic bound states in the continuum (BICs) have emerged as a versatile tool for enhancing light-matter interactions by strongly confining light fields. Chiral BICs are photonic resonances with a high degree of circular polarisation,…

Fabricating van der Waals (vdW) bilayer heterostructures (BL-HS) by stacking the same or different two-dimensional (2D) layers, offers a unique physical system with rich electronic and optical properties. Twist-angle between component…

Mesoscale and Nanoscale Physics · Physics 2020-12-17 Kha Tran , Junho Choi , Akshay Singh

The monolayer transition metal dichalcogenides are an emergent semiconductor platform exhibiting rich excitonic physics with coupled spin-valley degree of freedom and optical addressability. Here, we report a new series of low energy…

Strong magnetic fields profoundly affect the quantum physics of charged particles, as seen for example by the integer and fractionally quantized Hall effects, and the fractal `Hofstadter butterfly' spectrum of electrons in the presence of a…

Mesoscale and Nanoscale Physics · Physics 2023-12-19 Jie Wang , Jiawei Zang , Jennifer Cano , Andrew J. Millis

Valleytronic materials, characterized by local extrema (valley) in their bands, and topological insulators have separately attracted great interest recently. However, the interplay between valleytronic and topological properties in one…

Mesoscale and Nanoscale Physics · Physics 2018-08-27 Tong Zhou , Jiayong Zhang , Hua Jiang , Igor Zutic , Zhongqin Yang

Dipolar (or spatially indirect) excitons (IXs) in semiconductor double quantum well (DQW) subjected to an electric field are neutral species with a dipole moment oriented perpendicular to the DQW plane. Here, we theoretically study…

Mesoscale and Nanoscale Physics · Physics 2020-07-29 C. Hubert , K. Cohen , A. Ghazaryan , M. Lemeshko , R. Rapaport , P. V. Santos

Moir\'e superlattice-induced sub-bands in twisted van der Waals homo- and hetero-structures govern their optical and electrical properties, rendering additional degrees of freedom such as twist angle. Here, we demonstrate the moir\'e…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Medha Dandu , Garima Gupta , Pushkar Dasika , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Layered 2D van der Waals materials, such as transition metal dichalcogenides, are promising for nanoscale spintronic and optoelectronic applications. Harnessing their full potential requires understanding both intrinsic transport and the…