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Van der Waals materials provide a versatile toolbox for the emergence of new quantum phenomena and the fabrication of functional heterostructures. Among them, the trihalide VI3 stands out for its unique magnetic and structural landscape.…

Materials Science · Physics 2024-02-07 A. De Vita , R. Sant , V. Polewczyk , G. van der Laan , N. B. Brookes , T. Kong , R. J. Cava , G. Rossi , G. Vinai , G. Panaccione

The van der Waals ferromagnet (FM), VI$_3$, was studied by muon spin relaxation ($\mu^+$SR) and first principle calculations based on density functional theory (DFT). Temperature dependent zero field muon spin relaxation ($\mu^+$SR)…

Strongly Correlated Electrons · Physics 2022-11-01 Ola Kenji Forslund , Yuqing Ge , Hiroto Ohta , Chennan Wang , Mahmoud Abdel-Hafiez , Jun Sugiyama , Martin Månsson , Yasmine Sassa

VI$_{3}$ is a ferromagnet with planar honeycomb sheets of bonded V$^{3+}$ ions held together by van der Waals forces. We apply neutron spectroscopy to measure the two dimensional ($J/J_{c} \approx 17$) magnetic excitations in the…

Strongly Correlated Electrons · Physics 2021-07-23 H. Lane , E. Pachoud , J. A. Rodriguez-Rivera , M. Songvilay , G. Xu , P. M. Gehring , J. P. Attfield , R. A. Ewings , C. Stock

Van-der-Waals (vdW) ferromagnets have enabled the development of heterostructures assembled from exfoliated monolayers with spintronics functionalities, making it important to understand and ultimately tune their magnetic properties at the…

Here, we investigate the spin waves in room-temperature van der Waals ferromagnet $(\rm Fe_{0.78}Co_{0.22})_{5}GeTe_{2}$ by utilizing Brillouin light scattering technique. The spin wave dispersion in flakes of different thicknesses shows…

Mesoscale and Nanoscale Physics · Physics 2025-11-21 Guofu Xu , Feihao Pan , Jiyang Ou , Wenjun Ma , Xu Zhang , Xiling Li , Guoqiang Yu , Peng Cheng , Hongjun Xu , Guozhi Chai

The marked interplay between the crystalline, electronic, and magnetic structure of atomically thin magnets has been regarded as the key feature for designing next-generation magneto-optoelectronic devices. In this respect, a detailed…

Strongly Correlated Electrons · Physics 2020-05-25 Michele Pizzochero , Ravi Yadav , Oleg V. Yazyev

Antiferromagnetic van der Waals family $\rm \textit{M}P\textit{X}_{3}\ (M=Fe,\ Mn,\ Co,\text{ and}\ Ni; X=S\text{ and}\ Se)$ have attracted significant research attention due to the possibility of realizing long-range magnetic order down to…

Strongly Correlated Electrons · Physics 2024-06-11 Junbo Liao , Zhentao Huang , Yanyan Shangguan , Bo Zhang , Shufan Cheng , Hao Xu , Ryoichi Kajimoto , Kazuya Kamazawa , Song Bao , Jinsheng Wen

Layered van der Waals ferromagnets, which preserve their magnetic properties down to exfoliated monolayers, are fueling an abundance of fundamental research and nanoscale device demonstration. CrGeTe$_3$ is a prime example for this class of…

Strongly Correlated Electrons · Physics 2023-09-27 Han-Xiang Xu , Makoto Shimizu , Daniel Guterding , Junya Otsuki , Harald O. Jeschke

Two-dimensional van der Waals compounds with magnetic ions on a honeycomb lattice are hosts to a variety of exotic behavior. The magnetic interactions in one such compound, MnPSe$_3$, are investigated with elastic and inelastic neutron…

Strongly Correlated Electrons · Physics 2021-01-20 S. Calder , A. V. Haglund , A. I. Kolesnikov , D. Mandrus

We investigate the impact of mechanical strain, stacking order, and external electric fields on the magnetic interactions of a two-dimensional (2D) van der Waals (vdW) heterostructure in which a 2D ferromagnetic metallic Fe$_3$GeTe$_2$…

Materials Science · Physics 2023-03-30 Dongzhe Li , Soumyajyoti Haldar , Tim Drevelow , Stefan Heinze

Van der Waals materials hosting Kitaev interactions are promising platforms for exploring exotic quantum phenomena. Here, we report inelastic neutron scattering investigations of the van der Waals antiferromagnet VBr3, which forms a…

Strongly Correlated Electrons · Physics 2026-03-03 Zeyu Kao , Yimeng Gu , Yiqing Gu , Hao Zhang , Shiyi Zheng , Naoki Murai , Seiko Ohira-Kawamura , Jun Zhao

We present an ab initio investigation of magnetic exchange interactions using the spin-spiral method implemented in the VASP code, with a comparative analysis of the self-consistent (SC) and magnetic force theorem (MFT) approaches. Using…

Materials Science · Physics 2025-10-30 Umit Dogan Daglum , Maria Stamenova , Ersoy Sasioglu , Stefano Sanvito

The collective behavior of spins in a dilute magnetic semiconductor is determined by their mutual interactions and influenced by the underlying crystal structure. Hence, we begin with the atomic quantum-mechanical description of this system…

Materials Science · Physics 2010-10-12 Agnieszka Werpachowska , Tomasz Dietl

Two-dimensional (2D) magnetic materials are of great current interest for their promising applications in spintronics. Here we propose the van der Waals (vdW) material VI3 to be a 2D Ising ferromagnet (FM), using density functional…

Materials Science · Physics 2020-03-18 Ke Yang , Fengren Fan , Hongbo Wang , D. I. Khomskii , Hua Wu

Materials manifesting the Kitaev model, characterized by bond-dependent interactions on a honeycomb lattice, can host exotic phenomena like quantum spin liquid states and topological magnetic excitations. However, finding such materials…

Strongly Correlated Electrons · Physics 2024-12-31 Yiqing Gu , Yimeng Gu , Feiyang Liu , Seiko Ohira-Kawamura , Naoki Murai , Jun Zhao

In the local or itinerant extreme, magnetic excitations can be described by the Heisenberg model which treats electron spins as localized moments, or by the itinerant-electron model where the exchange interaction between electrons leads to…

Quantum mechanical calculations based on an extended Heisenberg model are compared with ferromagnetic resonance (FMR) experiments on prototype trilayer systems Ni_7/Cu_n/Co_2/Cu(001) in order to determine and separate for the first time…

Strongly Correlated Electrons · Physics 2009-11-11 S. Schwieger , J. Kienert , K. Lenz , J. Lindner , K. Baberschke , W. Nolting

Van der Waals (vdW) heterostructures have attracted great interest because of their rich material combinations.The discovery of two-dimensional magnets has provided a new platform for magnetic vdW heterointerfaces; however, research on…

Recently discovered ferromagnetism of the layered van der Waals material VI$_3$ attracts much research attention. Despite substantial progress,in the following important aspects no consensus has been reached: (i) a possible deviation of the…

Materials Science · Physics 2021-07-07 L. M. Sandratskii , K. Carva

The two-dimensional van der Waals (vdW) materials MPS_3(M = Mn, Fe, Co, Ni) display antiferromagnetic ordering of the magnetic moments at the transition metal ions. The possibility to exfoliate thin layers that preserve the magnetic order…

Materials Science · Physics 2024-08-28 Mohammad Amirabbasi , Peter Kratzer
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