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We report on the observation of two vibrational series of pure trilobite rubidium Rydberg molecules. They are created via three-photon photoassociation and lie energetically more than 15 GHz below the atomic 22$F$ state of rubidium. In…

Atomic Physics · Physics 2023-07-06 Max Althön , Markus Exner , Richard Blättner , Herwig Ott

We present photo-excitation of ultra-long-range Rydberg molecules as a probe of spatial correlations in quantum gases. Rydberg molecules can be created with well-defined internuclear spacing, set by the radius of the outer lobe of the…

Rydberg atom-based antennas exploit the quantum properties of highly excited Rydberg atoms, providing unique advantages over classical antennas, such as high sensitivity, broad frequency range, and compact size. Despite the increasing…

Signal Processing · Electrical Eng. & Systems 2025-06-09 Shuai S. A. Yuan , Xinyi Y. I. Xu , Jinpeng Yuan , Guoda Xie , Chongwen Huang , Xiaoming Chen , Zhixiang Huang , Wei E. I. Sha

Long-range dipole-dipole and quadrupole-quadrupole interactions between pairs of Rydberg atoms are calculated perturbatively for calcium, strontium and ytterbium within the Coulomb approximation. Quantum defects, obtained by fitting…

Atomic Physics · Physics 2012-06-11 C. L. Vaillant , M. P. A. Jones , R. M. Potvliege

The dielectric nature of polar liquids underpins much of their ability to act as useful solvents, but its description is complicated by the long-ranged nature of dipolar interactions. This is particularly pronounced under the periodic…

Soft Condensed Matter · Physics 2021-03-25 Stephen J. Cox

Synthetic dimensions, wherein dynamics occurs in a set of internal states, have found great success in recent years in exploring topological effects in cold atoms and photonics. However, the phenomena thus far explored have largely been…

Quantum Gases · Physics 2023-06-02 Tao Chen , Chenxi Huang , Ivan Velkovsky , Kaden R. A. Hazzard , Jacob P. Covey , Bryce Gadway

Coherently manipulating Rydberg atoms in mesoscopic systems has proven challenging due to the unwanted population of nearby Rydberg levels by black-body radiation. Recently, there have been some efforts towards understanding these effects…

Ensembles of atoms interacting via their Rydberg levels, known as "superatoms" for their ability to encode qubits and to emit single photons, attract increasing attention as building blocks for quantum network nodes. Assessing their…

Quantum Physics · Physics 2026-01-27 Valentin Magro , Sébastien Garcia , Alexei Ourjoumtsev

We have studied the associative ionization of a Rydberg atom and a ground state atom in an ultracold Rydberg gas. The measured scattering cross section is three orders of magnitude larger than the geometrical size of the produced molecule.…

Atomic Physics · Physics 2017-08-24 Thomas Niederprüm , Oliver Thomas , Torsten Manthey , Tobias M. Weber , Herwig Ott

The current advances in the field of ultra-cold atoms and atomic traps recall new controllable long-range interactions. These interactions are expected to extend the range of realizable quantum algorithms as well as providing new control…

Quantum Physics · Physics 2021-08-11 Mohammadsadegh Khazali

The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4]…

Mesoscale and Nanoscale Physics · Physics 2021-07-14 Julian Heckötter , Valentin Walther , Stefan Scheel , Manfred Bayer , Thomas Pohl , Marc Aßmann

The spatial evolution of the Rydberg blockade is studied taking into account Stark-split energy levels across several manifolds. We find that the unexpected restoration of a blockaded Rydberg excitation at small interatomic distances, e.g.,…

Atomic Physics · Physics 2017-05-09 Yurii V. Dumin , Jan M. Rost

We show that the resonant dipole-dipole interaction can give rise to bound states between two and three Rydberg atoms with non-overlapping electron clouds. The dimer and trimer states arise from avoided level crossings between states…

Atomic Physics · Physics 2015-06-19 Martin Kiffner , Mingxia Huo , Wenhui Li , Dieter Jaksch

A detailed theoretical framework for highly excited Rydberg molecules is developed based on the generalized local frame transformation. Our approach avoids the use of pseudopotentials and yields analytical expressions for the body-frame…

Atomic Physics · Physics 2020-09-16 P. Giannakeas , Matthew T. Eiles , F. Robicheaux , Jan-Michael Rost

We propose to use a permutation symmetric sample of multi-level atoms to simulate the properties of topologically ordered states. The Rydberg blockade interaction is used to prepare states of the sample which are equivalent to resonating…

Quantum Physics · Physics 2010-11-25 Anne E. B. Nielsen , Klaus Mølmer

We show that the highly excited rovibrational spectra of a diatomic molecule and the closely related slow atomic collision processes contain more systematics and require less parameters to characterize than the Rydberg spectrum of an atom.…

Atomic Physics · Physics 2007-05-23 Bo Gao

We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar…

Quantum Physics · Physics 2017-09-13 Elena Kuznetsova , Seth T. Rittenhouse , Hossein R. Sadeghpour , Susanne F. Yelin

We present a combined experimental and theoretical study of the effects of Rydberg interactions on Autler-Townes spectra of ultracold gases of atomic strontium. Realizing two-photon Rydberg excitation via a long-lived triplet state allows…

Atom-atom interactions within a small volume were investigated through the excitation of ultracold Rb atoms. The application of microwaves enhances these interactions, causing the suppression of Rydberg state excitation. The suppression of…

Atomic Physics · Physics 2015-06-05 E. Brekke , J. O. Day , T. G. Walker

The isotropic and anisotropic coefficients $C^{l,m}_n$ of the long-range spherical expansion $\sim 1/R^n$ ($R$ -- the intermolecular distance) of the dispersion and inductions intermolecular energies are calculated using the first…

Chemical Physics · Physics 2023-04-04 Leonid Shirkov , Michał Tomza