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Assembled arrays of individual atoms with Rydberg-mediated interactions provide a powerful platform for the simulation of many-body spin Hamiltonians as well as the implementation of universal gate-based quantum information processing. We…

The general formalism of the multipolar expansion of electrostatic interactions is applied to the calculation the potential energy between an excited atom (without fine structure) and a ground state diatomic molecule at large separations.…

Quantum Physics · Physics 2017-04-11 M. Lepers , O. Dulieu , V. Kokoouline

Strong interactions can amplify quantum effects such that they become important on macroscopic scales. Controlling these coherently on a single particle level is essential for the tailored preparation of strongly correlated quantum systems…

The properties and behaviour of a Ring Rydberg Composite are explicated. This system consists of a ring of ground state atoms centered on a Rydberg atom, whose electron elastically scatters off the ground state atoms. We transform the…

Atomic Physics · Physics 2020-02-19 Matthew T. Eiles , Andrew L. Hunter , Jan M. Rost

Radio-frequency (rf) fields in the MHz range are used to induce resonant energy transfer between cold Rydberg atoms in spatially separated volumes. After laser preparation of the Rydberg atoms, dipole-dipole coupling excites the 49s atoms…

Scheme to prepare three-dimensional entangled state between a pair of Rydberg atoms is proposed via dissipative dynamics and Electromagnetic Induced Transparency (EIT) associated with the single-atom dark state. The prepared entangled state…

Quantum Physics · Physics 2019-01-15 Shi-Lei Su

We study angular-momentum couplings in $^{87}$Rb$_2$ Rydberg molecules formed between Rydberg and 5S$_{1/2}$ ground-state atoms. We use a Fermi model that includes S-wave and P-wave singlet and triplet scattering of the Rydberg electron…

Atomic Physics · Physics 2016-01-12 David A. Anderson , Stephanie A. Miller , Georg Raithel

Rydberg atoms, with their giant electronic orbitals, exhibit dipole-dipole interaction reaching the GHz range at a distance of a micron, making them a prominent contender for realizing quantum operations well within their coherence time.…

Ultracold Rydberg molecules have been extensively studied both theoretically and ex-perimentally. Here the authors review the recent realizations of various ultralong-range Rydberg molecules and macrodimers, and explore their potential for…

Atomic Physics · Physics 2018-07-04 J. P. Shaffer , S. T. Rittenhouse , H. R Sadeghpour

A spatial structure of the zone blocked by the dipolar electric field of a Rydberg atom is calculated taking into account a possibility of excitation to the states with neighboring values of the principal quantum number. As a result, it was…

Atomic Physics · Physics 2014-08-26 Yurii V. Dumin

We propose a mechanism of ground-state blockade between two $N$-type Rydberg atoms in virtue of Rydberg-antiblockade effect and Raman transition. Inspired by the quantum Zeno effect, the strong Rydberg antiblockade interaction plays a role…

Quantum Physics · Physics 2017-12-07 X. Q. Shao , D. X. Li , Y. Q. Ji , J. H. Wu , X. X. Yi

Recent theoretical studies with alkali atoms A$^{\ast}$ excited to high Rydberg states predicted the existence of ultra long-range molecular bound states. Such excited dimers have large electric dipole moments which, in combination with…

Atomic Physics · Physics 2009-11-13 Chris H. Greene , Edward L. Hamilton , Heather Crowell , Cedomil Vadla , Kay Niemax

We explore the feasibility of optically forming long-range tetratomic and larger polyatomic molecules in their ground electronic state from ultracold pairs of polar molecules aligned by external fields. Depending on the relative orientation…

Atomic Physics · Physics 2021-06-16 Marko Gacesa , Jason N. Byrd , Jonathan Smucker , John A. Montgomery, , Robin Côté

Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary…

We study the quantum properties of Rydberg atoms in a magnetic Ioffe-Pritchard trap which is superimposed by a homogeneous electric field. Trapped Rydberg atoms can be created in long-lived electronic states exhibiting a permanent electric…

Atomic Physics · Physics 2007-09-17 Michael Mayle , Bernd Hezel , Igor Lesanovsky , Peter Schmelcher

The long-range dipole-dipole interaction can create delocalized states due to the exchange of excitation between Rydberg atoms. We show that even in a random gas many of the single-exciton eigenstates are surprisingly delocalized, composed…

Atomic Physics · Physics 2020-05-20 Ghassan Abumwis , Matthew T. Eiles , Alex Eisfeld

Arrays of Rydberg atoms interacting via dipole-dipole interactions offer a powerful platform for probing quantum many-body physics. However, these intrinsic interactions also determine and constrain the models -- and parameter regimes…

Quantum Gases · Physics 2025-12-16 Mingsheng Tian , Rhine Samajdar , Bryce Gadway

We investigate theoretically the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects on the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited…

Quantum Physics · Physics 2017-04-19 Maxence Lepers , Olivier Dulieu

Recent developments in the study of ultracold Rydberg gases demand an advanced level of experimental sophistication, in which high atomic and optical densities must be combined with excellent control of external fields and sensitive Rydberg…

A Rydberg molecule is composed of an outer electron that collides on the residual ionic core. Typical states of Rydberg molecules display entanglement between the outer electron and the core. In this work we quantify the average…

Quantum Physics · Physics 2007-05-23 M Lombardi , A Matzkin