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Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state…

Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom, which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, the spontaneous decay from the Rydberg state to an…

Quantum Physics · Physics 2021-12-21 Chang Qiao , Wenxian Zhang

We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…

Atomic Physics · Physics 2020-09-02 Andrew L. Hunter , Matthew T. Eiles , Alex Eisfeld , Jan M. Rost

We show that the recently observed class of long-range ion-Rydberg molecules can be divided into two families of states, which are characterised by their unique electronic structures resulting from the ion-induced admixture of quantum…

Atomic Physics · Physics 2023-02-14 Daniel J. Bosworth , Frederic Hummel , Peter Schmelcher

We observe that when an ultracold ground state cesium (Cs) atom becomes bound within the electronic cloud of an extended Cs electronic orbit, ultralong-range molecules with giant (kilo-Debye) permanent electric dipole moments form. Large…

Atomic Physics · Physics 2015-06-23 Donald Booth , Seth Rittenhouse , Jin Yang , Hossein Sadeghpour , James Shaffer

We present an entanglement scheme for Rydberg atoms using the van der Waals interaction phase induced by Ramsey-type pulsed interactions. This scheme realizes not only controlled phase operations between atoms at a distance larger than…

Atomic Physics · Physics 2020-01-29 Hanlae Jo , Yunheung Song , Minhyuk Kim , Jaewook Ahn

We show the existence of ultra-long-range giant dipole molecules formed by a neutral alkali ground state atom that is bound to the decentered electronic wave function of a giant dipole atom. The adiabatic potential surfaces emerging from…

Atomic Physics · Physics 2012-03-14 Markus Kurz , Michael Mayle , Peter Schmelcher

Experimental control over the strength and angular dependence of interactions between atoms is a key capability for advancing quantum technologies. Here, we use microwave dressing to manipulate and enhance Rydberg-Rydberg interactions in an…

Rydberg molecules, often exemplified by long-range "trilobite" molecules, are a subject of much recent interest at high principal quantum number $n$. States that use the same bonding mechanism can exist at much lower $n$ and less-extreme…

Atomic Physics · Physics 2017-05-01 R. A. Carollo , J. L. Carini , E. E. Eyler , P. L. Gould , W. C. Stwalley

We show that microwave spectroscopy of a dense Rydberg gas trapped on a superconducting atom chip in the dipole blockade regime reveals directly the dipole-dipole many-body interaction energy spectrum. We use this method to investigate the…

Recognition of multifrequency microwave (MW) electric fields is challenging because of the complex interference of multifrequency fields in practical applications. Rydberg atom-based measurements for multifrequency MW electric fields is…

Quantum Physics · Physics 2022-04-18 Zong-Kai Liu , Li-Hua Zhang , Bang Liu , Zheng-Yuan Zhang , Guang-Can Guo , Dong-Sheng Ding , Bao-Sen Shi

Rydberg atom arrays constitute a promising quantum information platform, where control over several hundred qubits has been demonstrated. Further scaling could significantly benefit from coupling to integrated optical or electronic devices,…

Since their first experimental observation, ultralong-range Rydberg molecules consisting of a highly excited Rydberg atom and a ground state atom have attracted the interest in the field of ultracold chemistry. Especially the intriguing…

We propose a Rydberg molecule dressing scheme to create strong and long-ranged interactions at selective distances. This is achieved through laser coupling ground-state atoms off-resonantly to an attractive molecular curve of two…

Quantum Physics · Physics 2022-06-16 Huaizhi Wu , Xin-Yu Lin , Zong-Xing Ding , Shi-Biao Zheng , Igor Lesanovsky , Weibin Li

Controlling molecular binding at the level of single atoms is one of the holy grails of quantum chemistry. Rydberg macrodimers -- bound states between highly excited Rydberg atoms -- provide a novel perspective in this direction. Resulting…

Atomic Physics · Physics 2023-06-14 Simon Hollerith , Johannes Zeiher

The Rydberg blockade is a key ingredient for entangling atoms in arrays. However, it requires atoms to be spaced well within the blockade radius, which limits the range of local quantum gates. Here we break this constraint using Floquet…

Quantum Physics · Physics 2023-11-08 Luheng Zhao , Michael Dao Kang Lee , Mohammad Mujahid Aliyu , Huanqian Loh

Trilobites are exotic giant dimers with enormous dipole moments. They consist of a Rydberg atom and a distant ground-state atom bound together by short-range electron-neutral attraction. We show that highly polar, polyatomic trilobite…

Atomic Physics · Physics 2017-11-22 Perttu J. J. Luukko , Jan-Michael Rost

Over the past few years we have built an apparatus to demonstrate the entanglement of neutral Rb atoms at optically resolvable distances using the strong interactions between Rydberg atoms. Here we review the basic physics involved in this…

Quantum Physics · Physics 2025-11-18 Thad G. Walker , Mark Saffman

Rydberg atoms in dc electric fields acquire static dipole moments. When the atoms are close to a surface producing an inhomogeneous electric field, such as by the adsorbates on an atom chip, depending on the sign of the dipole moment of the…

We present photodissociation of ultracold long-range Rydberg molecules as a tool to characterize their electronic properties. We photoassociate K2 37P molecules with highly entangled electronic and nuclear spins of the two bound atoms and…

Atomic Physics · Physics 2021-01-07 Michael Peper , Johannes Deiglmayr
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