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Two semiconductor optical frequency combs consuming less than 1 W of electrical power are used to demonstrate high-sensitivity mid-infrared dual-comb spectroscopy in the important 3-4 $\mu$m spectral region. The devices are 4 millimeters…

High-resolution ultrasound based imaging techniques like photoacoustic (PA) imaging that require fast detection of acoustic waves, are often coupled with an opto-mechanical sensor like a Fabry-Perot cavity (FPC) for enhanced sensitivity at…

Correlated rotational alignment spectroscopy correlates observables of ultrafast gas-phase spectroscopy with high-resolution, broad-band rotational Raman spectra. This article reviews the measurement principle of CRASY, existing…

Chemical Physics · Physics 2024-03-07 Thomas Schultz

Doppler-free spectroscopy using two counter-propagating dual-frequency laser beams in alkali vapor cells has been demonstrated recently, providing the detection of high-contrast sign-reversed natural-linewidth sub-Doppler resonances.…

Increasing the sensitivity of chiral spectroscopic techniques such as circular dichroism (CD) spectroscopy is a current aspiration in the research field of nanophotonics. Enhancing CD spectroscopy depends upon of two complementary…

Absolute distance measurement with low return power, fast measurement speed, high precision, and immunity to intensity fluctuations is highly demanded in nanotechnology. However, achieving all these objectives simultaneously remains a…

Optics · Physics 2025-12-30 Zihao Wang , Yifei Wang , Baoqi Shi , Wei Sun , Changxi Yang , Junqiu Liu , Chengying Bao

Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…

Instrumentation and Detectors · Physics 2020-05-12 Ting Qing , Shupeng Li , Yijie Fang , Xiaohu Tang , Lihan Wang , Meihui Cao , Xinyu Li , Shilong Pan

The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…

Optical frequency combs have emerged as a cornerstone for a wide range of areas, including spectroscopy, ranging, optical clocks, time and frequency transfer, waveform synthesis, and communications. However, quantum mechanical fluctuations…

Quantum Physics · Physics 2024-12-30 Abdulkarim Hariri , Shuai Liu , Haowei Shi , Quntao Zhuang , Xudong Fan , Zheshen Zhang

We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…

We report the use of broadband heterodyne spectroscopy to perform continuous measurement of the interaction energy between one atom and a high-finesse optical cavity, during individual transit events of $\sim 250$ $\mu$s duration.…

Quantum Physics · Physics 2009-10-31 Hideo Mabuchi , Jun Ye , H. Jeff Kimble

Ramsey spectroscopy in large, dense ensembles of ultra-cold atoms trapped in optical lattices suffers from dipole-dipole interaction induced shifts and collective superradiance limiting its precision and accuracy. We propose a novel…

Quantum Gases · Physics 2022-01-25 Christoph Hotter , Laurin Ostermann , Helmut Ritsch

Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…

Quantum Physics · Physics 2023-09-20 Haowei Shi , Zaijun Chen , Scott E. Fraser , Mengjie Yu , Zheshen Zhang , Quntao Zhuang

We measure the fluorescence spectrum of broadband emitters in an open optical microcavity with radius of curvature R = 17.7(3) um and finesse F ~= 1000. This geometry enables a combined measurement of emission spectra versus cavity length,…

Optics · Physics 2024-04-04 Corné Koks , Martin P. van Exter

Mid-infrared dual-comb spectroscopy has the potential to supplant conventional high-resolution Fourier transform spectroscopy in applications that require high resolution, accuracy, signal-to-noise ratio, and speed. Until now, dual-comb…

In this paper, we have established the couple system of a spectroscope, CCD and computer and proposed a method of the rapid measurement on spectral characteristics such as central wavelengths, relative intensities, sensitivity lines and the…

Instrumentation and Detectors · Physics 2015-12-03 Chol-Sun Kim , Chol-Su Kim , Song-Jin Im

Recent studies have shown that the nonlinear optical response of crystalline systems is fundamentally a quantum geometric property. In this work, we propose two-dimensional coherent spectroscopy (2DCS), which measures the nonlinear…

Mesoscale and Nanoscale Physics · Physics 2025-07-08 Paul Froese , Mark R. Hirsbrunner , Yong Baek Kim

Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is…

Diffuse correlation spectroscopy (DCS) is a powerful tool for assessing microvascular hemodynamic in deep tissues. Recent advances in sensors, lasers, and deep learning have further boosted the development of new DCS methods. However,…

We have recently introduced the Vernier-based Direct Frequency Comb Cavity-Enhanced Spectroscopy technique and we present the corresponding formalism for quantitative broadband spectroscopy. We achieve high sensitivity and broadband…

Optics · Physics 2016-11-23 Lucile Rutkowski , Jérôme Morville