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Accurately described excitonic properties of transition metal dichalcogenide heterobilayers (HBLs) are crucial to comprehend the optical response and the charge carrier dynamics of them. Excitons in multilayer systems posses inter or…

Materials Science · Physics 2018-08-01 E. Torun , A. Molina-Sánchez , H. P. C. Miranda , L. Wirtz

Moir\'e superlattices of transition metal dichalcogenide (TMD) heterostructures give rise to rich excitonic phenomena associated with the interlayer twist angle and induced changes in the involved quantum states. Theoretical calculations of…

Materials Science · Physics 2022-09-13 Sudipta Kundu , Tomer Amit , H. R. Krishnamurthy , Manish Jain , Sivan Refaely-Abramson

We study experimentally and theoretically the hybridization among intralayer and interlayer moir\'e excitons in a MoSe$_2$/WS$_2$ heterostructure with antiparallel alignment. Using a dual-gate device and cryogenic white light reflectance…

Quantifying and controlling the coherent dynamics and couplings of optically active excitations in solids is of paramount importance in fundamental research in condensed matter optics and for their prospective optoelectronic applications in…

Bilayer van der Waals (vdW) heterostructures such as MoS2/WS2 and MoSe2/WSe2 have attracted much attention recently, particularly because of their type II band alignments and the formation of interlayer exciton as the lowest-energy…

Mesoscale and Nanoscale Physics · Physics 2017-12-14 Shiyuan Gao , Li Yang , Catalin D. Spataru

Photoexcited intralayer excitons in van der Waals heterostructures (vdWHs) with type-II band alignment have been observed to tunnel into interlayer excitons on ultrafast timescales. Such interlayer excitons have sufficiently long lifetimes…

Mesoscale and Nanoscale Physics · Physics 2020-04-02 Høgni C. Kamban , Thomas G. Pedersen

Metal monochalcogenide GaSe is a classic layered semiconductor that has received increasing research interest due to its highly tunable electronic and optical properties for ultrathin electronics applications. Despite intense research…

Materials Science · Physics 2024-05-14 Fanhao Jia , Zhao Tang , Greis J. Cruz , Weiwei Gao , Shaowen Xu , Wei Ren , Peihong Zhang

Monolayer transition metal dichalcogenide (TMD) semiconductors such as MoSe$_2$ host strongly bound excitons which are known to exhibit a strong resonant third-order nonlinear response. Although there have been numerous studies of the…

Optical properties of heterostructures composed of layered 2D materials, such as transition metal dichalcogenides (TMDs) and graphene, are broadly explored. Of particular interest are light-induced energy transfer mechanisms in these…

Materials Science · Physics 2024-09-17 Amir Kleiner , Daniel Hernangómez-Pérez , Sivan Refaely-Abramson

This letter reports a time resolved pump-probe reflectance spectroscopic study on moir\'e excitons in a twisted monolayer WS2/WSe2 heterostructure. By probing at the resonant energies of intralayer excitons, we observed their distinct…

Mesoscale and Nanoscale Physics · Physics 2024-10-08 Feng Kai , Xiong Wang , Yiqin Xie , Yuhui Yang , Kenji Watanabe , Takashi Taniguchi , Hongyi Yu , Wang Yao , Xiaodong Cui

Two-dimensional (2D) materials, such as graphene1, boron nitride2, and transition metal dichalcogenides (TMDs)3-5, have sparked wide interest in both device physics and technological applications at the atomic monolayer limit. These 2D…

We theoretically investigated the coupling between the exciton internal and center-of-mass motions in monolayer transition metal dichalcogenides subjected to a periodic electrostatic potential. The coupling leads to the emergence of…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Fujia Lu , Qianying Hu , Yang Xu , Hongyi Yu

Monolayers of transition-metal dichalcogenides (TMDs) are characterized by an extraordinarily strong Coulomb interaction giving rise to tightly bound excitons with binding energies of hundreds of meV. Excitons dominate the optical response…

Materials Science · Physics 2018-05-30 Samuel Brem , Gunnar Berghaeuser , Malte Selig , Ermin Malic

In semiconductor physics, many essential optoelectronic material parameters can be experimentally revealed via optical spectroscopy in sufficiently large magnetic fields. For monolayer transition-metal dichalcogenide semiconductors, this…

Mesoscale and Nanoscale Physics · Physics 2020-08-20 M. Goryca , J. Li , A. V. Stier , T. Taniguchi , K. Watanabe , E. Courtade , S. Shree , C. Robert , B. Urbaszek , X. Marie , S. A. Crooker

Van der Waals heterostructures (vdWH) provide an ideal playground for exploring light-matter interactions at the atomic scale. In particular, structures with a type-II band alignment can yield detailed insight into free carrier-to-photon…

Materials Science · Physics 2017-04-05 Simone Latini , Kirsten T. Winther , Thomas Olsen , Kristian S. Thygesen

Van der Waals heterostructures of two-dimensional transition metal dichalcogenides provide a unique platform to engineer optoelectronic devices tuning their optical properties via stacking, twisting, or straining. Using ab initio Many-Body…

Mesoscale and Nanoscale Physics · Physics 2025-03-21 R. Reho , A. R. Botello-Méndez , D. Sangalli , M. J. Verstraete , Zeila Zanolli

The vertical stacking of two-dimensional materials into heterostructures gives rise to a plethora of intriguing optoelectronic properties and presents an unprecedented potential for technological development. While much progress has been…

Mesoscale and Nanoscale Physics · Physics 2022-06-27 Joshua J. P. Thompson , Victoria Lumsargis , Maja Feierabend , Quichen Zhao , Kang Wang , Letian Dou , Libai Huang , Ermin Malic

We reveal the higher energetic luminescence part of interlayer exciton ensembles in MoSe$_2$/WSe$_2$ heterostructures upon excitation by an optical Laguerre-Gaussian mode. The excitation is achieved with the help of a spatial light…

Stacking atomic monolayers of semiconducting transition metal dichalcogenides (TMDs) has emerged as an effective way to engineer their properties. In principle, the staggered band alignment of TMD heterostructures should result in the…

Mesoscale and Nanoscale Physics · Physics 2017-09-14 M. Baranowski , A. Surrente , L. Klopotowski , J. M. Urban , N. Zhang , D. K. Maude , K. Wiwatowski , S. Mackowski , Y. C. Kung , D. Dumcenco , A. Kis , P. Plochocka

We use femtosecond pump-probe spectroscopy to study the coherent interaction of excited exciton states in WSe2 and MoSe2 monolayers via the optical Stark effect. For co-circularly polarized pump and probe, we measure a blueshift which…

Mesoscale and Nanoscale Physics · Physics 2025-06-09 Max Wegerhoff , Moritz Scharfstädt , Stefan Linden , Andrea Bergschneider