English

Controlled coherent-coupling and dynamics of exciton complexes in a MoSe$_2$ monolayer

Mesoscale and Nanoscale Physics 2023-02-28 v1 Materials Science

Abstract

Quantifying and controlling the coherent dynamics and couplings of optically active excitations in solids is of paramount importance in fundamental research in condensed matter optics and for their prospective optoelectronic applications in quantum technologies. Here, we perform ultrafast coherent nonlinear spectroscopy of a charge-tunable MoSe2_2 monolayer. The experiments show that the homogeneous and inhomogeneous line width and the population decay of exciton complexes hosted by this material can be directly tuned by an applied gate bias, which governs the Fermi level and therefore the free carrier density. By performing two-dimensional spectroscopy, we also show that the same bias-tuning approach permits us to control the coherent coupling strength between charged and neutral exciton complexes.

Keywords

Cite

@article{arxiv.2302.13109,
  title  = {Controlled coherent-coupling and dynamics of exciton complexes in a MoSe$_2$ monolayer},
  author = {Aleksander Rodek and Thilo Hahn and James Howarth and Takashi Taniguchi and Kenji Watanabe and Marek Potemski and Piotr Kossacki and Daniel Wigger and Jacek Kasprzak},
  journal= {arXiv preprint arXiv:2302.13109},
  year   = {2023}
}