Related papers: Non-Loudon-Fleury Raman scattering in spin-orbit c…
Motivated by the lack of an obvious spectroscopic probe to investigate non-conventional order such as quadrupolar orders in spin S>1/2 systems, we present a theoretical approach to inelastic light scattering for spin-1 quantum magnets in…
In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…
Iron-based superconducting layered compounds have the second highest transition temperature after cuprate superconductors. Their discovery is a milestone in the history of high-temperature superconductivity and will have profound…
We report a polarized Raman scattering study of the lattice dynamics of $\beta$-Li$_2$IrO$_3$ under hydrostatic pressures up to 7.62 GPa. At ambient pressure, $\beta$-Li$_2$IrO$_3$ exhibits the hyperhoneycomb crystal structure and a…
The current efforts to find the materials hosting Kitaev model physics have been focused on Mott insulators of d^5 pseudospin-1/2 ions Ir^{4+} and Ru^{3+} with t_{2g}^5(S=1/2, L=1) electronic configuration. Here we propose that the Kitaev…
The electronic properties of Mott insulators realized in (111) bilayers of perovskite transition-metal oxides are studied. The low-energy effective Hamiltonians for such Mott insulators are derived in the presence of a strong spin-orbit…
Motivated by the rich interplay among electronic correlation, spin-orbit coupling (SOC), crystal-field splitting, and geometric frustrations in the honeycomb-like lattice, we systematically investigated the electronic and magnetic…
Raman scattering experiments on stoichiometric, Mott-insulating LaTiO$_3$ over a wide range of excitation energies reveal a broad electronic continuum which is featureless in the paramagnetic state, but develops a gap of $\sim 800$…
Ultrafast characterization and control of many-body interactions and elementary excitations are critical to understanding and manipulating emergent phenomena in strongly correlated systems. In particular, spin interaction plays an important…
We calculate magnon dispersions and damping in the Kitaev-Heisenberg model with an off-diagonal exchange $\Gamma$ and isotropic third-nearest-neighbor interaction $J_3$ on a honeycomb lattice. This model is relevant to a description of the…
Magnetic Raman scattering from a frustrated spin-1/2 Heisenberg-chain is considered with a focus on the uniform phase of the spin-Peierls compound CuGeO_3. The Raman intensity is analyzed in terms of a Loudon-Fleury scattering process using…
Kitaev interactions underlying a quantum spin liquid have been long sought, but experimental data from which their strengths can be determined directly is still lacking. Here, by carrying out inelastic neutron scattering measurements on…
The emergence of quasiparticles in quantum many-body systems underlies the rich phenomenology in many strongly interacting materials. In the context of doped Mott insulators, magnetic polarons are quasiparticles that usually arise from an…
There have been substantial recent efforts, both experimentally and theoretically, to find a material realization of the Kitaev spin-liquid--the ground state of the exactly solvable Kitaev model on the honeycomb lattice. Candidate materials…
Recent experiments on inelastic light scattering in a number of insulating cuprates [1] revealed a new excitation appearing in the case of crossed polarizations just below the optical absorption threshold. This observation suggests that…
An effective spin model for Mott insulators is determined by the symmetries involved among magnetic sites, electron fillings, and their interactions. Such a spin Hamiltonian offers insight to mechanisms of magnetic orders and magnetic…
Effects of electron many-body interactions amplify in an electronic system with a narrow bandwidth opening a way to exotic physics. A narrow band in a two-dimensional (2D) honeycomb lattice is particularly intriguing as combined with Dirac…
The Mott insulator a-RuCl3, featuring the intertwined interplay of spin-orbit coupling (SOC) and Kitaev spin correlations, provides an unparalleled platform for probing quantum many-body physics. Using scanning tunneling…
Cobaltates with 3$d$ based layered honeycomb structure were recently proposed as Kitaev magnets and putative candidates to host the long-sought Kitaev spin liquid. Here we present inelastic neutron scattering results down to 50 mK for…
Polarization-resolved Raman spectroscopy was performed and analyzed from large, high quality, mono-domain single crystal of {\alpha}-RuCl3, a proximate Kitaev quantum spin liquid. Spectra were collected with laser polarizations parallel and…