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We report on two types of Raman laser sources emitting in the near and middle ultraviolet spectral ranges by the use of a solarization-resilient gas-filled inhibited-coupling (IC) hollow-core photonic-crystal fiber (HCPCF) with record low…

We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient…

Atomic Physics · Physics 2021-08-26 J. C. Shaw , J. C. Schnaubelt , D. J. McCarron

We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…

Laser frequency combs are fast becoming critical to reaching the highest radial velocity precisions. One shortcoming is the highly variable brightness of the comb lines across the spectrum (up to 4-5 orders of magnitude). This can result in…

We study coherent anti-Stokes Raman spectroscopy in air-filled anti-resonance hollow-core photonic crystal fiber, otherwise known as 'revolver' fiber. We compare the vibrational coherent anti-Stokes Raman signal of N$_2$, at 2331 cm$^{-1}$,…

Globally, the long-haul transmission of ultra-high bandwidth data is enabled through coherent communications. Driven by the rapid pace of growth in interconnectivity over the last decade, long-haul data transmission has reached capacities…

The capability of focus control has been central to optical technologies that require both high temporal and spatial resolutions. However, existing varifocal lens schemes are commonly limited to the response time on the microsecond…

Frequency combs based on nonlinear-optical phenomena in integrated photonics are a versatile light source that can explore new applications, including frequency metrology, optical communications, and sensing. We demonstrate robust…

Frequency-modulated lasers (FMLs) are widely used in spectroscopy, biology, and LiDAR. The performance of these applications highly depends on the fast and precise tracking of the FMLs' absolute frequency, which remains a challenge. Here we…

Optics · Physics 2025-08-25 Weiwei Yang , Xingyu Jia , Jingyi Wang , Xinlun Cai , Yang Li , Guanhao Wu

We experimentally demonstrate efficient Raman conversion to respective Stokes and anti-Stokes fields in both pulsed and continuous modes with a Rb-87 atomic vapor cell. The conversion efficiency is about 40-50% for the Stokes field and…

Atomic Physics · Physics 2012-10-19 Bing Chen , Kai Zhang , Chun-Hua Yuan , Chengling Bian , Cheng Qiu , L. Q. Chen , Z. Y. Ou , Weiping Zhang

We demonstrate a method to double the collection efficiency in Laser Tweezers Raman Spectroscopy (LTRS) by collecting both the forward and back-scattered light in a single-shot multitrack measurement. Our method can collect signals at…

Optics · Physics 2021-06-09 Tobias Dahlberg , Magnus Andersson

Raman spectroscopy is an appealing technique that probes molecular vibrations in a wide variety of materials with virtually no sample preparation. However, accurate and reliable Raman measurements are still a challenge and require more…

Optics · Physics 2020-02-14 Hugo Kerdoncuff , Mikael Lassen , Jan C. Petersen

From the famous 1918 H1N1 influenza to the present COVID-19 pandemic, the need for improved virial detection techniques is all too apparent. The aim of the present paper is to show that identification of individual virus particles in…

Medical Physics · Physics 2020-11-23 V. Deckert , T. Deckert-Gaudig , D. Cialla , J. Popp , R. Zell , A. V. Sokolov , Z. Yi , M. O. Scully

We present a compact laser frequency stabilization method by locking a 556 nm laser to a high-precision wavelength meter. Unlike traditional schemes that rely on optical cavities or atomic references, we stabilize the laser frequency via a…

Optics · Physics 2025-06-27 Mengde Gan , Haoyi Zhang , Xiaodong Tan , Jiaming Li , Le Luo

We present a theoretical investigation of coherent anti-Stokes Raman scattering (CARS) that is modulated by periodically depleting the ground state population through Rabi oscillations driven by an additional control laser. We find that…

Using the shifted-excitation Raman difference spectroscopy technique and an optical fibre featuring a negative curvature excitation core and a coaxial ring of high numerical aperture collection cores, we have developed a portable,…

We present a detailed analysis of an application of frequency modulation (FM) spectroscopy in the high modulation depth limit. We have recently completed and reported a measurement of the Stark shift in the indium $5p_{1/2}\rightarrow…

Atomic Physics · Physics 2013-10-25 Nathan A. Schine , Gambhir Ranjit , Protik K. Majumder

The spectral resolution of broadband Fourier-transform coherent anti-Stokes Raman spectroscopy is limited by the maximum optical path length difference that can be scanned within a short time in an interferometer. However, alternatives to…

Multimode hollow microcavities in three-dimensional (3D) photonic crystals (PhCs) are designed for achieving enhanced coherent anti-Stokes Raman scattering, which requires a cavity to have three high quality-factor (Q) modes with equally…

Optics · Physics 2010-07-08 Jing Ouyang , Minghao Qi

Multi-photon microscopy is a powerful tool in biomolecular research. Less complex and more cost effective excitation light sources will make this technique accessible to a broader community. Especially semiconductor diode seeded fiber…