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We present a theoretical investigation of an integrated nonlinear light source for coherent anti-Stokes Raman scattering (CARS) based on silicon nitride waveguides. Wavelength tunable and temporally synchronized signal and idler pulses are…

Far field radiation pattern under tight focusing condition is investigated in Coherent Anti-stokes Raman Scattering (CARS) microscopy both in the forward (F-CARS) and backward (E-CARS) directions. While we assume no refraction index…

Optics · Physics 2009-11-11 D. Gachet , N. Sandeau , H. Rigneault

We report on the development of a compact (volume $\approx$ 100\:cm$^3$), multimode diffraction-limited Raman spectrograph and probe designed to be compact as possible. The spectrograph uses `off the shelf' optics, a custom 3D-printed…

Instrumentation and Detectors · Physics 2020-03-04 Christopher H. Betters , Joss Bland-Hawthorn , Salah Sukkarieh , Itandehui Gris-Sanchez , Sergio G. Leon-Saval

Coherent anti-Stokes Raman Spectroscopy (CARS) is a laser-based measurement technique widely applied across many science and engineering disciplines to perform non-intrusive gas diagnostics. CARS is often used to study combustion, where the…

Machine Learning · Computer Science 2022-05-25 Gregory J. Hunt , Cody R. Ground , Andrew D. Cutler

Raman sensing and Raman microscopy are amongst the most specific optical technologies to identify the chemical compounds of unknown samples, and to enable label-free biomedical imaging with molecular contrast. However, the high cost and…

We propose a new technique for comparing two Raman active samples. The method employs optical interference of the signals generated via coherent anti-Stokes Raman scattering (CARS) of broadband laser pulses with noisy spectra. It does not…

Quantum Physics · Physics 2015-05-27 Evgeny A. Shapiro , Stanislav O. Konorov , Valery Milner

Coherent anti-Stokes Raman scattering (CARS) and, in particular, femtosecond adaptive spectroscopic techniques (FAST CARS) have been successfully used for molecular spectroscopy and microscopic imaging. Recent progress in ultrafast…

The sensitivity of classical Raman spectroscopy methods, such as Coherent Anti-Stokes Raman spectroscopy (CARS) or Stimulated Raman spectroscopy (SRS), is ultimately limited by shot-noise from the stimulating fields. We present the complete…

Optics · Physics 2021-10-22 Yoad Michael , Leon Bello , Michael Rosenbluh , Avi Pe'er

We propose an all-fiber-generated dual-soliton pulses based scheme for the background-free detection of coherent anti-Stokes Raman spectroscopy under the spectral focusing mechanism. Due to the strong birefringence and high nonlinearity of…

Optics · Physics 2016-05-30 Kun Chen , Tao Wu , Haoyun Wei , Yan Li

Implementing stimulated Raman scattering in a low-loss microresonator could lead to Raman lasing. Here, we report the demonstration of an efficient Raman laser with $>50 \%$ power efficiency in an integrated silicon carbide platform for the…

We demonstrate a compact fibre-based laser system at 2.05 microns stabilized to a CO2 transition using frequency modulation spectroscopy of a gas-filled hollow-core fibre. The laser exhibits an absolute frequency accuracy of 5 MHz, a…

Instrumentation and Detectors · Physics 2016-03-02 Philip G. Westergaard , Jan W. Thomsen , Martin R. Henriksen , Mattia Michieletto , Marco Triches , Jens K. Lyngsø , Jan Hald

Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

We report on the development of a compact commercial instrument for measuring carotenoids in skin tissue. The instrument uses two light emitting diodes (LEDs) for dual-wavelength excitation and four photomultiplier tubes for multichannel…

Medical Physics · Physics 2009-11-13 S. D. Bergeson , J. B. Peatross , N. J. Eyring , J. F. Fralick , D. N. Stevenson , S. B. Ferguson

We describe a tunable broadband mid-infrared laser source based on difference-frequency mixing of a 100 MHz femtosecond Yb:fiber laser oscillator and a Raman-shifted soliton generated with the same laser. The resulting light is tunable over…

Optics · Physics 2015-05-30 Tyler W. Neely , Todd A. Johnson , Scott A. Diddams

A new interferometric technique is demonstrated for measuring Coherent Anti-Stokes Raman Scattering (CARS) signals. Two forward-directed CARS signals are generated, one in each arm of an interferometer. The deterministic nature of the CARS…

Optics · Physics 2007-05-23 J. S. Bredfeldt , D. L. Marks , C. Vinegoni , S. Hambir , S. A. Boppart

Raman scattering spectroscopy is widely used as an analytical technique in various fields, but its measurement process tends to be slow due to the low scattering cross-section. In the last decade, various broadband coherent Raman scattering…

Optics · Physics 2025-05-06 Takuma Nakamura , Kazuki Hashimoto , Takuro Ideguchi

We demonstrate a single-beam, standoff (>10m) coherent anti-Stokes Raman scattering spectroscopy (CARS) of various materials, including trace amounts of explosives and nitrate samples, under ambient light conditions. The multiplex…

Optics · Physics 2010-12-02 O. Katz , A. Natan , S. Rosenwaks , Y. Silberberg

Wavelength widely tunable infrared fiber lasers that simultaneously deliver high pulse energies with narrow linewidths are critical for applications ranging from spectroscopy to nonlinear optics, yet achieving this combination has remained…

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…

Time-resolved femtosecond stimulated Raman spectroscopy (FSRS) is a powerful tool for investigating ultrafast structural and vibrational dynamics in light absorbing systems. However, the technique generally requires exposing a sample to…

Instrumentation and Detectors · Physics 2018-07-10 Matthew N. Ashner , William A. Tisdale