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The $S=1/2$ Kitaev honeycomb model has attracted significant attention as an exactly solvable example with a quantum spin liquid ground state. In a properly oriented external magnetic field, chiral Majorana edge modes associated with a…

Strongly Correlated Electrons · Physics 2022-03-23 Pedro M. Cônsoli , Eric C. Andrade

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

Materials Science · Physics 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

YbOCl is a representative member of the van der Waals layered honeycomb rare-earth chalcohalide REChX (RE = rare earth, Ch = O, S, Se, and Te, and X = F, Cl, Br, and I) family reported recently. Its spin ground state remains to be explored…

Strongly Correlated Electrons · Physics 2024-09-13 Zheng Zhang , Yanzhen Cai , Jinlong Jiao , Jing Kang , Dehong Yu , Bertrand Roessli , Anmin Zhang , Jianting Ji , Feng Jin , Jie Ma , Qingming Zhang

We show that a magnetic field in the high-symmetry direction lifts the macroscopic classical ground-state degeneracy of the honeycomb $\Gamma$ model and induces a long-range magnetic order. While a simple spin-polarized state is stabilized…

Strongly Correlated Electrons · Physics 2021-07-01 Zhongzheng Tian , Zhijie Fan , Preetha Saha , Gia-Wei Chern

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

Strongly Correlated Electrons · Physics 2023-09-14 Xu-Guang Zhou , Han Li , Yasuhiro H. Matsuda , Akira Matsuo , Wei Li , Nobuyuki Kurita , Gang Su , Koichi Kindo , Hidekazu Tanaka

Layered $\alpha$-RuCl3 has been discussed as a proximate Kitaev spin liquid compound. Raman and THz spectroscopy of magnetic excitations confirm that the low-temperature antiferromagnetic ordered phase features a broad Raman continuum,…

We investigate the phase diagram of a bilayer Kitaev honeycomb model with Ising interlayer interactions, deriving effective models via perturbation theory and performing Majorana mean-field theory calculations. We show that a diverse array…

Strongly Correlated Electrons · Physics 2024-04-30 Aayush Vijayvargia , Urban F. P. Seifert , Onur Erten

Quantum fluctuations in the effective spin one-half layered structure triangular-lattice quantum Heisenberg antiferromagnet Ba$_3$CoSb$_2$O$_9$ lift the classical degeneracy of the antiferromagnetic ground state in magnetic field, producing…

Strongly Correlated Electrons · Physics 2021-06-02 N. A. Fortune , Q. Huang , T. Hong , J. Ma , E. S. Choi , S. T. Hannahs , Z. Y. Zhao , X. F. Sun , Y. Takano , H. D. Zhou

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

We report a $^{35}$Cl nuclear magnetic resonance study in the honeycomb lattice, $\alpha$-RuCl$_3$, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct…

Strongly Correlated Electrons · Physics 2017-07-26 S. -H. Baek , S. -H. Do , K. -Y. Choi , Y. S. Kwon , A. U. B. Wolter , S. Nishimoto , Jeroen van den Brink , B. Büchner

Compounds of transition metal ions with strong spin-orbit coupling recently attracted attention due to the possibility to host frustrated bond-dependent anisotropic magnetic interactions. In general, such interactions lead to complex phase…

Strongly Correlated Electrons · Physics 2019-02-21 Juraj Rusnačko , Dorota Gotfryd , Jiří Chaloupka

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

Spin systems with honeycomb structures have recently attracted a great deal of attention in connection with the Kitaev quantum spin liquid state (QSL) predicted theoretically. One possible Kitaev QSL candidate is Na$_2$Co$_2$TeO$_6$…

Strongly Correlated Electrons · Physics 2023-12-11 A. K. Bera , S. M. Yusuf , F. Orlandi , P. Manuel , L. Bhaskaran , S. A. Zvyagin

We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor…

Strongly Correlated Electrons · Physics 2015-12-08 Ioannis Rousochatzakis , Johannes Reuther , Ronny Thomale , Stephan Rachel , N. B. Perkins

Motivated by recent experiments, we consider a generic spin model in the $j_{\text{eff}}=1/2$ basis for the hyperhoneycomb and harmonic-honeycomb iridates. Based on microscopic considerations, the effect of an additional bond-dependent…

Strongly Correlated Electrons · Physics 2015-02-09 Eric Kin-Ho Lee , Yong Baek Kim

We report the existence of a phase transition at high temperature in the 3D Kitaev candidate material, $\beta$-Li$_2$IrO$_3$. We show that the transition is bulk, intrinsic and orders a tiny magnetic moment with a spatially anisotropic…

Intensive studies of the interplay between spin-orbit coupling (SOC) and electronic correlations in transition metal compounds have recently been undertaken. In particular, $j_{\rm eff}$ = 1/2 bands on a honeycomb lattice provide a pathway…

Strongly Correlated Electrons · Physics 2015-06-24 Heung-Sik Kim , V. Vijay Shankar , Andrei Catuneanu , Hae-Young Kee

Motivated by the magnetic phase transition of a proximate Kitaev system $\alpha$-RuCl$_3$ in the presence of a magnetic field, we study the simplest but essential quantum spin model with the ferromagnetic nearest neighboring (NN) Kitaev…

Strongly Correlated Electrons · Physics 2020-10-14 Beom Hyun Kim , Shigetoshi Sota , Tomonori Shirakawa , Seiji Yunoki , Young-Woo Son

In candidate Kitaev materials, the off-diagonal $\Gamma$ and $\Gamma'$ interactions are identified to come from the spin-orbit coupling and trigonal distortion, respectively. They have generated intense research efforts because of their…

Strongly Correlated Electrons · Physics 2022-05-30 Qiang Luo , Hae-Young Kee

The magnetic orders in Na$_2$IrO$_3$ and $\alpha-$RuCl$_3$, honeycomb systems with strong spin-orbit coupling and correlations, have been recently described by models with the dominant Kitaev interactions. In this work we discuss how the…

Strongly Correlated Electrons · Physics 2017-02-10 Yuriy Sizyuk , Peter Woelfle , Natalia B. Perkins