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We report the discovery of an intriguing pressure-driven phase transformation in the layered Kitaev-material $\alpha$-RuCl$_3$. By analyzing both the Bragg scattering as well as the diffuse scattering of high-quality single crystals, we…

Strongly Correlated Electrons · Physics 2022-09-20 Quirin Stahl , Tobias Ritschel , Gaston Garbarino , Frederico Cova , Anna Isaeva , Thomas Doert , Jochen Geck

We discuss the magnetic phases of the Hubbard model for the honeycomb lattice both in two and three spatial dimensions. A ground state phase diagram is obtained depending on the interaction strength U and electronic density n. We find a…

Strongly Correlated Electrons · Physics 2016-08-31 N. M. R. Peres , M. A. N. Araujo , Daniel Bozi

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

Muon spin rotation measurements have been performed on a powder sample of a-RuCl3, a layered material which previously has been proposed to be a quantum magnet on a honeycomb lattice close to a quantum spin liquid ground state. Our data…

Strongly Correlated Electrons · Physics 2016-07-20 F. Lang , P. J. Baker , A. A. Haghighirad , Y. Li , D. Prabhakaran , R. Valenti , S. J. Blundell

KCuCl$_3$ is a three-dimensional coupled spin-dimer system and has a singlet ground state with an excitation gap ${\Delta}/k_{\rm B}=31$ K. High-field magnetization measurements for KCuCl$_3$ have been performed in static magnetic fields of…

Strongly Correlated Electrons · Physics 2009-11-07 A. Oosawa , T. Takamasu , K. Tatani , H. Abe , N. Tsujii , O. Suzuki , H. Tanaka , G. Kido , K. Kindo

$\alpha$-RuCl$_3$ has been extensively studied recently because of potential bond-dependent Kitaev magnetic exchange interactions and the resulting quantum spin liquid phase that can be realized therein. It has been known that the covalency…

Strongly Correlated Electrons · Physics 2022-01-13 Heung-Sik Kim

Motivated by intense research on two-dimensional spin-1/2 Kitaev materials, Kitaev spin chains and ladders, though geometrically limited, have been studied for their numerical simplicity and insights into extended Kitaev models. The phase…

Strongly Correlated Electrons · Physics 2026-04-21 Mandev Bhullar , Haoting Xu , Hae-Young Kee

Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $\alpha$-RuCl$_3$. Here we propose the monoclinic YbCl$_3$ with a Yb$^{3+}$ honeycomb lattice for the…

Strongly Correlated Electrons · Physics 2020-07-22 Jie Xing , Erxi Feng , Yaohua Liu , Eve Emmanouilidou , Chaowei Hu , Jinyu Liu , David Graf , Arthur P. Ramirez , Gang Chen , Huibo Cao , Ni Ni

The pursuit of quantum spin liquid (QSL) in the Kitaev honeycomb magnets has drawn intensive attention recently. In particular, $\alpha$-RuCl$_3$ has been widely recognized as a promising candidate for the Kitaev QSL. Although the compound…

Strongly Correlated Electrons · Physics 2023-03-29 Han Li , Wei Li , Gang Su

Heisenberg antiferromagnet with an easy-plane anisotropy is discussed in which a magnetic spiral is induced by Dzyaloshinskii-Moriya interaction and/or frustration of the exchange coupling. The distortion of the spiral by small in-plane…

Strongly Correlated Electrons · Physics 2026-05-05 P. T. Bolokhova , A. V. Syromyatnikov

$\alpha$-RuCl$_3$ has attracted enormous attention since it has been proposed as a prime candidate to study fractionalized magnetic excitations akin to Kitaev's honeycomb-lattice spin liquid. We have performed a detailed specific-heat…

Strongly Correlated Electrons · Physics 2017-07-19 A. U. B. Wolter , L. T. Corredor , L. Janssen , K. Nenkov , S. Schönecker , S. -H. Do , K. -Y. Choi , R. Albrecht , J. Hunger , T. Doert , M. Vojta , B. Büchner

The Kitaev material $\alpha$-RuCl$_3$ is among the most prominent candidates to host a quantum spin-liquid state endowed with fractionalized excitations. Recent experimental and theoretical investigations have separately revealed the…

The honeycomb iridates A2IrO3 (A=Na, Li) constitute promising candidate materials to realize the Heisenberg-Kitaev model (HKM) in nature, hosting unconventional magnetic as well as spin liquid phases. Recent experiments suggest, however,…

Strongly Correlated Electrons · Physics 2015-06-19 Johannes Reuther , Ronny Thomale , Stephan Rachel

The crystal structure, magnetic ground state, and the temperature dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet Na2Co2TeO6 have been investigated by powder neutron diffraction. A three…

Strongly Correlated Electrons · Physics 2017-03-29 A. K. Bera , S. M. Yusuf , Amit Kumar , C. Ritter

Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real…

We explore a phenomenological phase diagram for the magnetic helical state with 90$^{\circ}$ turn angle between neighboring spins in the external magnetic field. Such state is formed by the Eu spin layers in the superconducting iron…

Strongly Correlated Electrons · Physics 2022-04-04 A. E. Koshelev

Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the…

Strongly Correlated Electrons · Physics 2024-12-17 John S. Pearce , David A. S. Kaib , Zeyu Ma , Danrui Ni , R. J. Cava , Roser Valenti , Radu Coldea , Amalia I. Coldea

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

We discuss theoretically phase transitions in frustrated antiferromagnets with biaxial anisotropy or dipolar forces in magnetic field applied along the easy axis at $T=0$. There are well-known sequences of phase transitions upon the field…

Strongly Correlated Electrons · Physics 2019-09-04 O. I. Utesov , A. V. Syromyatnikov

We present comprehensive inelastic neutron spectroscopic maps of the magnetic field-induced disordered phase of the Kitaev quantum spin liquid candidate material $\alpha$-RuCl$_3$. For fields along both in-plane high-symmetry directions we…