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Characterizing time delays in molecular photoionization as a function of the ejected electron emission direction relative to the orientation of the molecule and the light polarization axis pro-vides unprecedented insights into the…

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

Atomic Physics · Physics 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

Time-resolved photoelectron spectroscopy provides access to the electronic structure and non-equilibrium electron dynamics in matter. At solid surfaces photoemission dynamics can be investigated on its natural time scale by measuring…

Time-delays in the photoionization of molecules are investigated. As compared to atomic ionization, the time-delays expected from molecular ionization present a much richer phenomenon, with a strong spatial dependence due to the anisotropic…

Atomic Physics · Physics 2017-02-14 P. Hockett , E. Frumker , D. M. Villeneuve , P. B. Corkum

Photon exchange due to nuclear bremsstrahlung during nuclear collisions can cause Coulomb excitation in the projectile and the target nuclei. The corresponding process originated in nuclear timescales can also be observed in atomic…

We study ionization of aligned H$_2^+$ in strong elliptically-polarized laser fields numerically and analytically. The calculated offset angle in photoelectron momentum distribution is several degrees larger for the molecule than a model…

Atomic Physics · Physics 2023-01-03 J. Y. Che , Y. G. Peng , F. B. Zhang , X. J. Xie , G. G. Xin , Y. J. Chen

More than 100 years after its discovery and its explanation in the energy domain, the duration of the photoelectric effect is still heavily studied. The emission time of a photoelectron can be quantified by the Wigner time delay.…

The photophysics and photochemistry associated with irradiating UV light in liquid water is central to numerous physical, chemical and biological processes. One of the key events involved in this process is the generation of the hydrated…

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

Recently the time delay in the attosecond photoemission was observed (Science,2010). In this paper we propose the description of that time delay in the framework of hyperbolic heat transport equation. We argue that the observed time delay…

General Physics · Physics 2013-02-20 J. Marciak-Kozlowska , M. Kozlowski

We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…

Atomic Physics · Physics 2018-04-03 Ruihua Xu , Zhaoyan Zhou , Xu Wang

After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecondresolved photoemission experiments. According…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Mauro Fanciulli , Henrieta Volfová , Stefan Muff , Jürgen Braun , Hubert Ebert , Jan Minár , Ulrich Heinzmann , J. Hugo Dil

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we…

Atomic Physics · Physics 2020-02-19 Benjamin Willenberg , Jochen Maurer , Benedikt W. Mayer , Ursula Keller

Photoionization by high-energy photons creates nonthermal electrons with a broad range of energies that heat and chemically transform the atmospheres of planets. The specifics of the interactions are notably different when the gas is atomic…

Earth and Planetary Astrophysics · Physics 2025-06-17 Antonio García Muñoz , Ewan Bataille

The photoelectric effect has a sister process relevant in optoelectronics called internal photoemission. Here an electron is photoemitted from a metal into a semiconductor. While the photoelectric effect takes place within less than 100…

The R-Matrix incorporating Time (RMT) method is a new method for solving the time-dependent Schroedinger equation for multi-electron atomic systems exposed to intense short-pulse laser light. We have employed the RMT method to investigate…

Atomic Physics · Physics 2012-04-27 L. R. Moore , M. A. Lysaght , J. S. Parker , H. W. van der Hart , K. T. Taylor

The reionization epoch concludes when ionizing photons reach every corner of the Universe. Reionization has generally been assumed to be limited primarily by the rate at which galaxies produce ionizing photons, but the recent measurement of…

Cosmology and Nongalactic Astrophysics · Physics 2021-09-22 Frederick B. Davies , Sarah E. I. Bosman , Steven R. Furlanetto , George D. Becker , Anson D'Aloisio

Focused laser fields with textured polarization on a sub-wavelength scale allow extracting information on electronic processes which are not directly accessible by homogeneous fields. Here, we consider photoionization in radially and…

Atomic Physics · Physics 2021-06-30 Jonas Wätzel , Jamal Berakdar

Chiral light-matter interactions have been investigated for two centuries, leading to the discovery of many chiroptical processes used for discrimination of enantiomers. Whereas most chiroptical effects result from a response of bound…