Related papers: Chiral high-harmonic generation and spectroscopy o…
The bi-circular scheme for high harmonic generation, which combines two counter-rotating circular fields with frequency ratio 2:1, has recently permitted to generate high harmonics with essentially circular polarization, opening the way for…
We examined, in backward (reflection) geometry, the generation of the 3rd and 5th harmonics, located in the deep and vacuum ultraviolet, on the surface of silicon and on the interface between silicon and silica when a thin silica film was…
We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…
High-energy spin-polarized electron, positron, and $\gamma$-photon beams have many significant applications in the study of material properties, nuclear structure, particle physics, and high-energy astrophysics. Thus,efficient production of…
In strong laser fields, the electron density in solids can show up tidal motions caused by the laser ``pulling'' on the electrons, which forms an electron density tide (EDT). However, the strong field processes in solids are always…
High-harmonic generation in two-colour ($\omega-2\omega$) counter-rotating circularly polarised laser fields opens the path to generate isolated attosecond pulses and attosecond pulse trains with controlled ellipticity. The generated…
Cylindrical vector (CV) gamma rays can introduce spatially structured polarization as a new degree of freedom for fundamental research and practical applications. However, their generation and control remain largely unexplored. Here, we put…
Nonlinear optical microscopy such as in the optical second-harmonic generation (SHG) modality has become a popular tool today for probing materials in the physical and biological sciences. While imaging and spectroscopy are widely used in…
High-order harmonic generation (HHG) is a fundamental process which can be simplified as the production of high energetic photons from a material subjected to a strong driving laser field. This highly nonlinear optical process contains rich…
Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…
Tailoring optical nonlinear effects (e.g. harmonic generation, sum-frequency mixing, etc.) in the recently emerging all-dielectric platform is important for both the fundamental science and industrial development of high-efficiency,…
We study the effective second-harmonic generation (SHG) susceptibility in graded metallic films by invoking the local field effects exactly, and further numerically demonstrate that the graded metallic films can serve as a novel optical…
Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium…
Ultrafast imaging of molecular chirality is a key step towards the dream of imaging and interpreting electronic dynamics in complex and biologically relevant molecules. Here, we propose a new ultrafast chiral phenomenon exploiting recent…
An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical…
We investigate theoretically the strong-field regime of light-matter interactions in the topological-insulator class of quantum materials. In particular, we focus on the process of non-perturbative high-order harmonic generation from the…
High-order harmonic generation (HHG) in solids has entered a new phase of intensive research, with envisioned band-structure mapping on an ultrashort time scale. This partly benefits from a flurry of new HHG materials discovered, but so far…
Structured {\gamma} rays, particularly cylindrical vector {\gamma} rays, offer promising tools for sub-nuclear imaging and polarization-sensitive probes in fundamental research and applications, but conventional optical methods face great…
The emergence of strong-field nanoplasmonics brings extreme laser field-matter interaction into the realm of nanoscale science, unveiling exciting new physics. Highly nonlinear interaction is enabled by tightly confined electric fields in…
Nonlinear Compton scattering driven by ultraintense lasers presents a promising avenue for enhancing the photon energy, brilliance, and setup compactness of $\gamma$-ray sources. However, a significant challenge lies in achieving a high…