Related papers: Chiral high-harmonic generation and spectroscopy o…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
The discovery of topological phases has introduced a new dimension to materials science. Three-dimensional (3D) topological insulators (TIs) are a remarkable class of matter that is insulating in the bulk while hosting conductive…
Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…
Nonlinear propagation of intense femtosecond laser pulses in bulk transparent media leads to a specific propagation regime, termed femtosecond filamentation, which in turn produces dramatic spectral broadening, or superbroadening, termed…
We present a numerical study of the resonant high harmonic generation by tin ions in an elliptically-polarised laser field along with a simple analytical model revealing the mechanism and main features of this process. We show that the…
Second-harmonic generation microscopy is a powerful technique capable of probing local crystal symmetries and electric fields at interfaces. However, it often suffers from weak signal strength and is difficult to understand in multilayer…
Light-matter interactions are key in providing fundamental information about materials. Even in the linear-response regime, the spectroscopic response of a material encodes in it many properties of the ground state as well as of its…
Optical analog computing enables powerful functionalities, including spatial differentiation, image processing, and ultrafast linear operations. Yet, most existing approaches rely on resonant or periodic structures, whose performance is…
Chiral materials display a property called optical activity, which is the capability to interact differentially with left and right circularly polarised light. This leads to the ability to manipulate the polarisation state of light, which…
Squeezing of optical fields, used as a powerful resource for many applications, and the radiation properties in the process of high harmonic generation have thus far been considered separately. In this Letter, we want to clarify that the…
Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…
A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…
We propose and numerically demonstrate a new very robust and highly selective method for femtosecond time-resolved chiral spectroscopy using high harmonic generation (HHG). The method is based on dynamical symmetry breaking from chiral…
Circularly polarized light plays a key role in many applications including spectroscopy, microscopy, and control of atomic systems. Particularly in the latter, high polarization purity is often required. Integrated technologies for atomic…
We present measurements of hard x-rays in the 50-300 keV range from copper plasmas produced by 100 fs, 806 nm laser pulses at a peak intensity ~ 1016 W cm-2. Surface roughness, even at the tens of nanometer level, is shown to influence the…
We review the physics and some applications of photonic structures designed for the realisation of strong $\textit{nonlinear chiroptical response}$. We pay much attention to the recent strategy of utilizing different types of…
Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…
We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…
Strain engineering is a versatile method to boost the carrier mobility of two-dimensional materials-based electronics and optoelectronic devices. In addition, strain is ubiquitous during device fabrication via material deposition on a…
Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…