Related papers: Chiral high-harmonic generation and spectroscopy o…
Due to the mirror symmetry breaking, chiral structures show fantastic electromagnetic (EM) properties involving negative refraction, giant optical activity, and asymmetric transmission. Aligned electric and magnetic dipoles excited in…
Light is one of the most powerful and precise tools allowing us to control, shape and create new phases of matter. In this task, the magnetic component of a light wave has so far played a unique role in defining the wave's helicity, but its…
Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher…
Synthetic chiral light enables ultrafast and highly efficient imaging of molecular chirality. Unlike standard circularly polarized light, the handedness of synthetic chiral light does not rely on the spatial structure of the light field: it…
Linear polarization analysis of hard x-rays is employed to probe electronic anisotropies in metal-containing complexes with very high selectivity. We use the pronounced linear dichroism of nuclear resonant x-ray scattering to determine…
We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…
High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended…
High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…
We introduce an ultrafast all-optical approach for efficient chiral recognition which relies on the interference between two low-order nonlinear processes which are ubiquitous in nonlinear optics: sum-frequency generation and third-harmonic…
Using a high-frequency field superposed to a linearly polarized bichromatic laser field composed by a wave with frequency $\omega $ and a wave with frequency $2\omega $, we show it is possible to enhance the intensity of a group of high…
The ability to create surface structures with precisely controlled chirality remains a major challenge in laser-matter interaction experiments. In this work, we theoretically study the interaction of vortex laser beams, characterized by…
We generate high-order harmonics of a mid-infrared laser from a silicon single crystal and find their origin in the recollision of coherently accelerated electrons with their holes, analogously to the atomic and molecular case, and to ZnO…
We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…
We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…
High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…
Charge acceleration during an intense light field application to solids attracts much attention as elementary processes in high-harmonic generation and photoelectron emission [1-7]. For manipulating such attosecond dynamics of charge,…
High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…
The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…
Coherent synchrotron radiation (CSR) is crucial for the development of powerful ultrashort light sources. We present a mechanism for generating CSR in the form of generalised superradiance, based on surface plasmon polaritons (SPPs), which…
We present a theoretical study of second-harmonic generation from a singular metasurface. The singular metasurfaces strongly interact with the incident light, where the large field enhancement forms an intense surface polarization that…