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We analyze theoretically the effects of electron-phonon interaction in the dynamics of an electron that can be trapped to a localized state and detrapped to an extended band state of a small quantum dot (QD) using a simple model system. In…

Mesoscale and Nanoscale Physics · Physics 2021-12-03 R. Carmina Monreal

Nonlinear phononics holds the promise for controlling properties of quantum materials on the ultrashort timescale. Using nonequilibrium dynamical mean-field theory, we solve a model for the description of organic solids, where correlated…

Strongly Correlated Electrons · Physics 2021-01-27 Francesco Grandi , Jiajun Li , Martin Eckstein

The interaction of graphene with metallic substrates reveals phenomena and properties of great relevance for applications in nanotechnology. In this review, the vibrational characterization by means of various inelastic scattering…

Materials Science · Physics 2016-01-08 Antonio Politano

Hydrodynamic phonon transport phenomena, like second sound, have been observed in liquid Helium more than 50 years ago. More recently second sound has been observed in graphite at over 200 K using transient thermal grating techniques. In…

Mesoscale and Nanoscale Physics · Physics 2024-03-13 Laurenz Kremeyer , Tristan L. Britt , Bradley J. Siwick , Samuel C. Huberman

The unique optical properties of graphene, with broadband absorption and ultrafast response, make it a critical component of optoelectronic and spintronic devices. Using time-resolved momentum microscopy with high data rate and high dynamic…

We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

The spectral response and physical features of the 2D Hubbard-Holstein model are calculated both in equilibrium at zero and low chemical dopings, and after an ultra short powerful light pulse, in undoped systems. At equilibrium and at…

Strongly Correlated Electrons · Physics 2015-06-05 G. De Filippis , V. Cataudella , E. A. Nowadnick , T. P. Devereaux , A. S. Mishchenko , N. Nagaosa

Conclusive experimental evidence of a supersolid phase in any known condensed matter system is presently lacking. On the other hand, a supersolid phase has been recently predicted for a system of spinless bosons in continuous space,…

Quantum Gases · Physics 2012-04-27 Sebastiano Saccani , Saverio Moroni , Massimo Boninsegni

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…

Efforts to push the spatiotemporal imaging-resolution limits of femtosecond (fs) laser-driven ultrafast electron microscopes (UEMs) to the combined angstrom-fs range will benefit from stable sources capable of generating high bunch charges.…

Materials Science · Physics 2024-09-25 Jialiang Chen , Simon A. Willis , David J. Flannigan

Ultrafast laser irradiation of solids leads to a thermodynamic nonequilibrium within and between the electron and phonon subsystems of the material. Due to electron-electron and phonon-phonon collisions, both subsystems relax into…

Materials Science · Physics 2018-10-24 Isabel Klett , Baerbel Rethfeld

Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

We propose a theoretical framework for the detection of order parameter fluctuations in three dimensions using ultrafast coherent phonon spectroscopy. We focus our attention on long wavelength charge density fluctuations (plasmons), and…

Strongly Correlated Electrons · Physics 2019-07-03 Chandan Setty , Kridsanaphong Limtragool , Byron Freelon , Philip W. Phillips

The development of many optical quantum technologies depends on the availability of solid-state single quantum emitters with near-perfect optical coherence. However, a standing issue that limits systematic improvement is the significant…

Understanding of the energy exchange between electrons and phonons in metals is important for micro- and nano-manufacturing and system design. The electron-phonon (e-ph) coupling constant is to describe such exchange strength, yet its…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Wuli Miao , Moran Wang

We present an exact Monte Carlo method to simulate the nonequilibrium dynamics of electron-phonon models in the adiabatic limit of zero phonon frequency. The classical nature of the phonons allows us to sample the equilibrium phonon…

Strongly Correlated Electrons · Physics 2022-02-16 Manuel Weber , James K. Freericks

Hot electron effects in graphene are significant because of graphene's small electronic heat capacity and weak electron-phonon coupling, yet the dynamics and cooling mechanisms of hot electrons in graphene are not completely understood. We…

Time and angular resolved photoelectron spectroscopy is a powerful technique to measure electron dynamics in solids. Recent advances in this technique have facilitated band and energy resolved observations of the effect that excited…

Materials Science · Physics 2020-09-30 Umberto De Giovannini , Hannes Hübener , Shunsuke A. Sato , Angel Rubio

The increasing need to simulate the dynamics of photoexcited molecular and nanosystems in the sub-picosecond regime demands new efficient tools able to describe the quantum nature of matter at a low computational cost. By combining the…

Dynamic scattering and imaging with coherent, ultrafast, extreme ultraviolet (EUV) light sources can resolve charge, phonon and spin processes on their intrinsic length and time scales. However, full field coherent diffraction imaging…

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