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The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

This perspective introduces attosecond path qubits: measurement-defined two-level subsystems that arise naturally in strong-field physics from the coherent interference of distinguishable quantum pathways. These effective qubits are…

Optics · Physics 2026-01-14 Oren Cohen

Entanglement is one of the most intriguing aspects of quantum mechanics and lies at the heart of the ongoing Second Quantum Revolution, where it is a resource that is used in quantum key distribution, quantum computing and quantum…

Quantum Physics · Physics 2022-02-02 Lisa-Marie Koll , Laura Maikowski , Lorenz Drescher , Tobias Witting , Marc J. J. Vrakking

We numerically study 2-photon processes using a set of harmonics from a Ti:Sapphire laser and in particular interference effects in the Above Threshold Ionization spectra. We compare the situation where the harmonic phases are assumed…

Quantum Physics · Physics 2009-10-31 Eric Cormier , Anna Sanpera , Maciej Lewenstein , Pierre Agostini

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

We present an analytical model that characterizes two-photon transitions in the presence of autoionising states. We applied this model to interpret resonant RABITT spectra, and show that, as a harmonic traverses a resonance, the phase of…

Atomic Physics · Physics 2016-01-20 Álvaro Jiménez Galán , Luca Argenti , Fernando Martín

We have calculated the resonant and nonresonant contributions to attosecond impulsive stimulated electronic Raman scattering (SERS) in regions of autoionizing transitions. Comparison with Multiconfiguration Time-Dependent Hartree-Fock…

Atomic Physics · Physics 2016-10-06 Matthew R. Ware , Philip H. Bucksbaum , James P. Cryan , Daniel J. Haxton

We measure the photoelectron energy spectra from strong-field ionization of Kr in a two-color laser pulse consisting of a strong 400-nm field and a weak 800-nm field. The intensities of the main above-threshold ionization (ATI) and sideband…

Atomic Physics · Physics 2019-12-11 Yudi Feng , Min Li , Siqiang Luo , Kun Liu , Baojie Du , Yueming Zhou , Peixiang Lu

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

In a recent experiment by Eichmann et al., polarization-sensitive measurements of the fluorescence from two four-level ions driven by a linearly polarized laser were made. Depending on the polarization chosen, different degrees of…

Atomic Physics · Physics 2009-10-30 T. Wong , S. M. Tan , M. J. Collett , D. F. Walls

We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and neutral particles with permanent dipole moments. Interference is studied when electrons or atomic…

Quantum Physics · Physics 2009-11-11 Fernando C. Lombardo , Paula I. Villar

We study both experimentally and theoretically, considering bosonic atoms in a periodic potential, the influence of interactions in a Talbot interferometer. While interactions decrease the contrast of the revivals, we find that over a wide…

We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into…

Atomic Physics · Physics 2015-06-04 Xinhua Xie

We study the isotropic Heisenberg chain with nearest and next-nearest neighbour interactions. The ground state phase diagram is constructed in dependence on the additonal interactions and an external magnetic field. The thermodynamics is…

Strongly Correlated Electrons · Physics 2009-11-13 Christian Trippe , Andreas Klümper

Multi-photon interference reveals strictly non-classical phenomena. Its applications range from fundamental tests of quantum mechanics to photonic quantum information processing, where a significant fraction of key experiments achieved so…

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we…

Atomic Physics · Physics 2020-02-19 Benjamin Willenberg , Jochen Maurer , Benedikt W. Mayer , Ursula Keller

We present the development and implementation of an experimental setup designed to investigate attosecond photoionization delays using a dual-sideband RABBITT (Reconstruction of Attosecond Beating By Interference of Two-Photon Transitions)…

Large conditional phase shifts from coupled atom-cavity systems are a key requirement for building a spin photon interface. This in turn would allow the realisation of hybrid quantum information schemes using spin and photonic qubits. Here…

We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a…

Atomic Physics · Physics 2015-01-14 Álvaro J. Galán , Luca Argenti , Fernando Martín