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Extracting single photoionization time delays associated with atomic (or molecular) species from attosecond time scale two-photon experiments usually relies on the theoretical description of continuum-continuum transitions. The available…

Atomic Physics · Physics 2022-08-29 D. I. R. Boll , L. Martini , O. A. Fojón

The very strong electromagnetic fields present in ultraperipheral relativistic heavy ion collisions lead to important higher order effects of the electromagnetic interaction. These multiphoton exchange processes are studied using…

Nuclear Theory · Physics 2014-11-18 Gerhard Baur , Kai Hencken , Andreas Aste , Dirk Trautmann , Spencer R. Klein

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

We present theoretical studies of above threshold ionization (ATI) produced by spatially inhomogeneous fields. This kind of field appears as a result of the illumination of plasmonic nanostructures and metal nanoparticles with a short laser…

New ab-initio surface hopping simulations of the excited state dynamics of CS$_2$ including spin-orbit coupling are compared to new experimental measurements using a multiphoton ionisation probe in a photoelectron spectroscopy experiment.…

In this article we theoretically study the phase shift a single atom imprints onto a coherent state light beam in free space. The calculations are performed in a semiclassical framework. The key parameters governing the interaction and thus…

Quantum Physics · Physics 2013-10-03 Markus Sondermann , Gerd Leuchs

Interferometric measurements of high-harmonics induced by multiple laser fields in an emerging field of research that promises optimized yield of harmonics, and time and space-resolved nonlinear spectroscopy. Most of the measurements have…

Nonlinear metasurfaces that dynamically manipulate the phase of a passing light beam are of interest for a wide range of applications. The controlled operation of such devices requires accurate measurements of the optical transmission phase…

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

In quantum information science, the external control of qubits must be balanced with the extreme isolation of the qubits from the environment. Atomic qubit systems typically mitigate this balance through the use of gated laser fields that…

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

Atomic ensembles strongly interacting with light constitute rich quantum-optical many-body systems, with the potential for observing cooperative effects and dissipative nonequilibrium phase transitions. We theoretically analyze the…

Quantum Physics · Physics 2025-01-28 Janne Ruostekoski

In strong laser fields, sub-femtosecond control of chemical reactions with the carrier-envelope phase (CEP) becomes feasible. We have studied the control of reaction dynamics of acetylene and allene in intense few-cycle laser pulses at 750…

We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of…

Atomic Physics · Physics 2016-03-02 Álvaro Jiménez Galán , Fernando Martín , Luca Argenti

Particle-wave duality has allowed physicists to establish atomic interferometers as celebrated complements to their optical counterparts in a broad range of quantum devices. However, interactions naturally lead to decoherence and have been…

Quantum Gases · Physics 2020-04-15 Changyuan Lyu , Qi Zhou

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

We study the influence of off-resonant two photon transitions on high precision measurements with atom interferometers based on stimulated Raman transitions. These resonances induce a two photon light shift on the resonant Raman condition.…

The analysis of phase shifts in executed and proposed interferometry experiments on photons and neutrons neglected forces exerted at the boundaries of spatial constrictions. When those forces are included it is seen that the observed…

Quantum Physics · Physics 2007-05-23 Murray Peshkin

A quantum two-path interferometer allows for direct measurement of the transmission phase shift of an electron, providing useful information on coherent scattering problems. In mesoscopic systems, however, the two-path interference is…

Mesoscale and Nanoscale Physics · Physics 2015-08-13 S. Takada , M. Yamamoto , C. Bäuerle , K. Watanabe , A. Ludwig , A. D. Wieck , S. Tarucha