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We demonstrate efficient transfer of ultracold molecules into a deeply bound rovibrational level of the singlet ground state potential in the presence of an optical lattice. The overall molecule creation efficiency is 25%, and the transfer…

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

Atomic Physics · Physics 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

We use the phenomenon of electromagnetically-induced transparency in a three-level atomic system for hyperfine spectroscopy of upper states that are not directly coupled to the ground state. The three levels form a ladder system: the probe…

Optics · Physics 2007-05-23 Anusha Krishna , Kanhaiya Pandey , Ajay Wasan , Vasant Natarajan

Control over all internal and external degrees of freedom of molecules at the level of single quantum states will enable a series of fundamental studies in physics and chemistry. In particular, samples of ground-state molecules at ultralow…

We propose an alternative method to laser cooling. Our approach utilizes the extreme brightness of a supersonic atomic beam, and the adiabatic atomic coilgun to slow atoms in the beam or to bring them to rest. We show how internal-state…

The precise control and knowledge over the atomic dynamics is central to the advancement of quantum technology. The different experimental conditions namely, atoms in a vacuum, an anti-relaxation coated and a buffer gas filled atomic cell…

Atomic Physics · Physics 2022-07-21 Swarupananda Pradhan , Saptarshi Roy Chowdhury

Erbium doped solids are potential candidates for the realization of a quantum memory for photons at telecommunication wavelengths. The implementation of quantum memory proposals in rare earth ion doped solids require spectral tailoring of…

Quantum Physics · Physics 2010-02-15 B. Lauritzen , S. R. Hastings-Simon , H. de Riedmatten , M. Afzelius , N. Gisin

We propose and implement a novel scheme for dissipatively pumping two qubits into a singlet Bell state. The method relies on a process of collective optical pumping to an excited level, to which all states apart from the singlet are…

We propose a novel cooling scheme for realising single photon sideband cooling on particles trapped in a state-dependent optical potential. We develop a master rate equation from an ab-initio model and find that in experimentally feasible…

Quantum Gases · Physics 2022-02-11 Federico Berto , Elia Perego , Lucia Duca , Carlo Sias

Room temperature Terahertz stimulated emission and population inversion in optically pumped graphene is reported. We experimentally observe fast relaxation and relatively slow recombination dynamics of photogenerated electrons/holes in an…

Materials Science · Physics 2012-08-27 Stephane Boubanga Tombet , Silvia Chan , Taiichi Otsuji , Akira Satou , and Victor Ryzhii

We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…

Atomic Physics · Physics 2026-01-14 Emanuel F. de Lima

Coherent dark states in atoms, created by simultaneous interaction of two coherent light fields with a 3-level system, are of prime importance in quantum state manipulation. They are used extensively in quantum sensing and quantum…

Atomic Physics · Physics 2019-09-09 M. Shuker , J. W. Pollock , V. I. Yudin , J. Kitching , E. A. Donley

We demonstrate subpicosecond-time-scale population transfer between the pair of hyperfine ground states of atomic rubidium using a single laser-pulse. Our scheme utilizes the geometric and dynamic phases induced during Rabi oscillation…

Atomic Physics · Physics 2018-05-23 Yunheung Song , Han-gyeol Lee , Hyosub Kim , Hanlae Jo , Jaewook Ahn

We present a hyperfine-resolved state preparation scheme for thallium fluoride (TlF) molecules based on microwave-driven adiabatic passage (AP) in a spatially varying electric field. This method enables efficient and robust population…

We propose a multilevel scheme to coherently transfer the population of a diatomic molecule from a rovibrational level to a target rovibrational level of the same electronic state or another. It involves a linear chain of N rovibrational…

Quantum Physics · Physics 2024-12-11 Diego F. Uribe , Mateo Londoño , Julio C. Arce

We use two-laser optical pumping on a continuous atomic fountain in order to prepare cold cesium atoms in the same quantum ground state. A first laser excites the F=4 ground state to pump the atoms toward F=3 while a second pi-polarized…

Atomic Physics · Physics 2015-05-19 Gianni Di Domenico , Laurent Devenoges , Claire Dumas , Pierre Thomann

We present a new method for the generation of rotationally and vibrationally state-selected, translationally cold molecular ions in ion traps. Our technique is based on the state-selective threshold photoionization of neutral molecules…

Chemical Physics · Physics 2010-06-30 Xin Tong , Alexander H. Winney , Stefan Willitsch

We produce an ultracold and dense sample of rovibronic ground state Cs_2 molecules close to the regime of quantum degeneracy, in a single hyperfine level, in the presence of an optical lattice. The molecules are individually trapped, in the…

We demonstrate the production of ultracold polar RbCs molecules in their vibronic ground state, via photoassociation of laser-cooled atoms followed by a laser-stimulated state transfer process. The resulting sample of $X ^1\Sigma^+ (v=0)$…

Atomic Physics · Physics 2009-11-11 J. M. Sage , S. Sainis , T. Bergeman , D. DeMille

We use optimal control theory to show that for a closed $\Lambda$-system where the excited intermediate level decays to the lower levels with a common large rate, the optimal scheme for population transfer between the lower levels is…

Quantum Physics · Physics 2022-12-27 Dionisis Stefanatos , Emmanuel Paspalakis