Related papers: Protocol for Optically Pumping AlH$^+$ to a Pure Q…
We report on direct detection of excited states absorption cross-section using dual wavelength pump-probe technique. Also, we experimentally demonstrate using porphyrin composite molecules (porphyrin derivatives such as…
A method is proposed for preparing any pure and a wide class of mixed quantum states in the decoherence-free ground-state subspace of a degenerate multilevel lambda system. The scheme is a combination of optical pumping and a series of…
We propose a method to stabilize Laughlin states of a large number of strongly interacting photons by combining a frequency-selective incoherent pump with a step-like potential in the angular momentum basis. Analytical expressions for the…
We consider a laser cooling and trapping of alkaline-earth and similar atoms in a bichromatic field resonant to a closed optical transition $^1S_0 \to \, ^1P_1$ or $^1S_0 \to \, ^3P_1$. It is shown that new kinetic effects emerge compared…
We propose a scheme for attaining slow and fast light via coherent control of the hyperfine ground and excited states of an ultracold atomic system. The proposed scheme is theoretically analyzed for the $D_1$ transition of ultracold $^{23}$…
We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage…
We study the nonlinear and resonant process of two-photon ionization of atoms (He and H) in a pump-probe scheme. The pump pulse prepares the quantum system in a superposition of the ground state and an excited bound state. By varying the…
We perform ab-initio calculations needed to predict the cross-section of an experimentally accessible (1+1') resonance-enhanced multiphoton dissociation (REMPD) pathway in AlH+. Experimenting on AlH+ ions held in a radiofrequency Paul trap,…
We describe bichromatic superradiant pump-probe spectroscopy as a tomographic probe of the Wigner function of a dispersing particle beam. We employed this technique to characterize the quantum state of an ultracold atomic beam, derived from…
We propose a novel scheme for the population and depletion of nuclear isomers. The scheme combines the $\gamma$-photons with energies $\gtrsim 10$ keV emitted during the interaction of a contemporary high-intensity laser pulse with a plasma…
We compare two different experimental techniques for the magnetic-sub-level preparation of metastable $^4$He in the $2^3$S$_1$ level in a supersonic beam, namely magnetic hexapole focusing and optical pumping by laser radiation. At a beam…
We study laser-driven isomerization reactions through an excited electronic state using the recently developed Geometrical Optimization procedure [J. Phys. Chem. Lett. 6, 1724 (2015)]. The goal is to analyze whether an initial wave packet…
Controlling the polarization state of light with sub-picosecond speed and subwavelength precision remains a key challenge for next-generation nanophotonic devices. Conventional methods such as birefringent crystals, liquid crystals, or…
We propose a mechanism to produce a superposition of atomic and molecular states by a train of ultrashort laser pulses combined with weak control fields. By adjusting the repetition rate of the pump pulses and the intensity of the coupling…
Cooling down a trapped ion into its motional ground state is a central step for trapped ions based quantum information processing. State of the art cooling schemes often work under a set of optimal cooling conditions derived analytically…
The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…
We propose a simple exact analytical solution for a model consisting of a two-level system and a polychromatically driving field. It helps us to realize a rapid complete population transfer from the ground state to the excited state, and…
Fast and efficient state preparation of molecules can be accomplished by optical pumping. Molecular structure that most obviously facilitates cycling involves a strong electronic transition, with favorable vibrational branching (diagonal…
A coherent state of many spins contains quantum entanglement which increases with a decrease in the collective spin value. We present a scheme to engineer this class of pure state based on incoherent spin pumping with a few collective…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…