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We explore coherent multi-photon processes in $^{87}$Rb$^{133}$Cs molecules using 3-level lambda and ladder configurations of rotational and hyperfine states, and discuss their relevance to future applications in quantum computation and…

Quantum Gases · Physics 2020-11-13 Jacob A. Blackmore , Philip D. Gregory , Sarah L. Bromley , Simon L. Cornish

Optical pumping of molecules provides unique opportunities for control of chemical reactions at a wide range of rotational energies. This work reports a chemical reaction with extreme rotational excitation of a reactant and its kinetic…

We demonstrate coherent storage and retrieval of pulsed light using the atomic frequency comb quantum memory protocol in a room temperature alkali vapour. We utilise velocity-selective optical pumping to prepare multiple velocity classes in…

Quantum Physics · Physics 2021-06-17 D. Main , T. M. Hird , S. Gao , I. A. Walmsley , P. M. Ledingham

We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…

Quantum Physics · Physics 2009-10-07 M. Zeppenfeld , M. Motsch , P. W. H. Pinkse , G. Rempe

We propose an experimental procedure to cool fermionic atoms loaded into an optical lattice. The central idea is to spatially divide the system into entropy-rich and -poor regions by shaping the confining potential profile. Atoms in regions…

Inspired by recent work [A. W. Carr and M. Saffman, Phys. Rev. Lett. 111, 033607 (2013)], we propose a simplified scheme to prepare the two-atom maximally entangled states via dissipative Rydberg pumping. Compared with the former scheme,…

Quantum Physics · Physics 2015-09-01 Shi-Lei Su , Qi Guo , Hong-Fu Wang , Shou Zhang

Laser cooling and trapping of atoms and atomic ions has led to numerous advances including the observation of exotic phases of matter, development of exquisite sensors and state-of-the-art atomic clocks. The same level of control in…

We report the 1-D cooling of $^{85}$Rb atoms using a velocity-dependent optical force based upon Ramsey matter-wave interferometry. Using stimulated Raman transitions between ground hyperfine states, 12 cycles of the interferometer sequence…

Atomic Physics · Physics 2015-08-19 Alexander Dunning , Rachel Gregory , James Bateman , Matthew Himsworth , Tim Freegarde

Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…

Quantum Physics · Physics 2010-08-09 J. Deiglmayr , A. Grochola , M. Repp , K. Mörtlbauer , C. Glück , J. Lange , O. Dulieu , R. Wester , M. Weidemüller

We present the prospects for photoassociation, optical control of interspecies scattering lengths and finally, the production of ultracold absolute ground state molecules in the Rb+Hg system. We use the "gold standard" ab initio methods for…

We spectroscopically investigate a pathway for the conversion of $^{23}\textrm{Na}^{39}\textrm{K}$ Feshbach molecules into rovibronic ground state molecules via STImulated Raman Adiabatic Passage (STIRAP). Using photoassociation…

We demonstrate steady-state, mirrorless superradiance in a cold vapor pumped by weak optical fields. Beyond a critical pump intensity of 1 mW/cm$^2$, the vapor spontaneously transforms into a spatially self-organized state: a density…

Atomic Physics · Physics 2015-06-04 Joel A. Greenberg , Daniel J. Gauthier

We propose a two-step protocol for inverting ultrafast spectroscopy experiments on a molecular aggregate to extract the time-evolution of the excited state density matrix. The first step is a deconvolution of the experimental signal to…

Quantum Physics · Physics 2013-05-29 Stephan Hoyer , K. Birgitta Whaley

We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…

Atomic Physics · Physics 2026-05-01 Wu Wang , Ke Zhang , Ke-Mi Xu , Shan-Gui Zhou

We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the…

Quantum Gases · Physics 2012-05-15 Sebastian D. Huber , Hans Peter Büchler

A method of sideband Raman cooling to the vibrational ground state of the $m=0$ Zeeman sublevel in a far-detuned two-dimensional optical lattice is proposed. In our scheme, the Raman coupling between vibrational manifolds of the adjacent…

Atomic Physics · Physics 2007-05-23 A. V. Taichenachev , A. M. Tumaikin , V. I. Yudin , L. Hollberg

Here we report on spectroscopic measurements of the aluminum monofluoride molecule (AlF) that are relevant to laser cooling and trapping experiments. We measure the detailed energy level structure of AlF in the X$^1\Sigma^+$ electronic…

The efficient preparation of collective eigenstates of subwavelength-spaced optical dipoles is a prerequisite for observing their signature radiative properties and for their applications in quantum information processing. We theoretically…

Quantum Physics · Physics 2026-03-27 Johannes Kerber , Laurin Ostermann , Vikas Remesh , Helmut Ritsch , Arpita Pal

We demonstrate high atomic mercury vapor pressure in a kagom\'e-style hollow-core photonic crystal fiber at room temperature. After a few days of exposure to mercury vapor the fiber is homogeneously filled and the optical depth achieved…

Quantum state reconstruction based on weak continuous measurement has the advantage of being fast, accurate, and almost non-perturbative. In this work we present a pedagogical review of the protocol proposed by Silberfarb et al., PRL 95…

Quantum Physics · Physics 2015-05-20 Carlos A. Riofrío , Poul S. Jessen , Ivan H. Deutsch