Related papers: Lineshape Analysis of Double-Quantum Multidimensio…
Absorption imaging with quasi-resonant laser light is a commonly used technique to probe ultra-cold atomic gases in various geometries. Here we investigate some non-trivial aspects of this method when it is applied to in situ diagnosis of a…
We propose and demonstrate an interferometric scheme for measuring the two-dimensional two-point cross-spectral density function in a two-shot manner. Our scheme comprises a Michelson interferometer with a converging lens in one of the arms…
Recent experiments on cuprates have shown the possibility of opening a gap above the superconducting critical temperature, in the so-called phase-fluctuating state, by enhancing the phase coherence of preformed Cooper pairs. Quench-drive…
Two-dimensional electronic spectroscopy (2DES) has enabled significant discoveries in both biological and synthetic energy-transducing systems. Although deriving chemical information from 2DES is a complex task, machine learning (ML) offers…
Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing…
Electronic energy transfer in photosynthesis occurs over a range of time scales and under a variety of intermolecular coupling conditions. Recent work has shown that electronic coupling between chromophores can lead to coherent oscillations…
Optical solitary waves (solitons) that interact in a nonlinear system can bind and form a structure similar to a molecule. The rich dynamics of this process have created a demand for rapid spectral characterization to deepen the…
Spectroscopic polarimetry (SP) is a powerful tool for evaluation of thin film, optical materials, and biological samples because it can provide both polarimetric and spectroscopic characteristics of objects. However, its performance is…
Two-dimensional coherent spectroscopy (2DCS) provides insights into the nonlinear response of correlated lattice systems. We simulate multipulse excitations in the Hubbard model using nonequilibrium dynamical mean-field theory to extract…
Doppler-free spectroscopy using two counter-propagating dual-frequency laser beams in alkali vapor cells has been demonstrated recently, providing the detection of high-contrast sign-reversed natural-linewidth sub-Doppler resonances.…
We introduce dissipative spectroscopy as a framework for extracting spectral information from quantum systems via controlled dissipation. By establishing a general dissipative response theory applicable to both Markovian and non-Markovian…
A fluorescence correlation spectroscopy (FCS) system based on two independent measurement volumes is presented. The optical setup and data acquisition hardware are detailed, as well as a complete protocol to control the location, size and…
Optical spectroscopy techniques such as differential reflectance and transmittance have proven to be very powerful techniques to study 2D materials. However, a thorough description of the experimental setups needed to carry out these…
The following article presents a multi-length-scale characterization approach for investigating doping chemistry and spatial distributions within semiconductors, as demonstrated using a state-of-the-art CMOS image sensor. With an intricate…
Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…
Linear-response quantum electrodynamical density functional theory (QEDFT) enables the description of molecular spectra under strong coupling to quantized photonic modes, such as those in optical cavities. Recently, this approach was…
We study the optical properties of an ensemble of two-level atoms coupled to a 1D photonic crystal waveguide (PCW), which mediates long-range coherent dipole-dipole interactions between the atoms. We show that the long-range interactions…
In the current study, a quantum-cascade-laser-based dual-comb spectrometer (DCS) was used to paint a detailed picture of a 1.0 ms high-temperature reaction between propyne and oxygen. The DCS interfaced with a shock tube to provide…
We measure many-body interactions in isolated quantum dot states using double-quantum multidimensional coherent spectroscopy. Few states are probed in a diffraction limited spot, which is enabled by a novel collinear scheme in which…
We have developed a microscopic many-body theory of two-dimensional coherent spectroscopy (2DCS) for a model of polarons in one-dimensional (1D) materials. Our theory accounts for contributions from all three processes: excited-state…