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What is the correct low-energy spin Hamiltonian description of $\alpha$-RuCl$_3$? The material is a promising Kitaev spin liquid candidate, but is also known to order magnetically, the description of which necessitates additional…

Strongly Correlated Electrons · Physics 2020-01-13 Pontus Laurell , Satoshi Okamoto

By incorporating inert KCl into the Na$_2$IrO$_3$ + 2CuCl $\to$ Cu$_2$IrO$_3$ + 2NaCl topochemical reaction, we significantly reduced the synthesis temperature of Cu$_2$IrO$_3$ from the 350$^\circ$C reported in previous studies to…

Materials Science · Physics 2024-07-12 Yuya Haraguchi , Daisuke Nishio-Hamane , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

We use magnetization measurements under pressure along with \textit{ab initio} and cluster many-body calculations to investigate magnetism of the Kitaev candidate Li$_2$RhO$_3$. Hydrostatic compression leads to a decrease in the magnitude…

The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

The temperature dependence of magnetic anisotropy in (113)A (Ga,Mn)As layers grown by molecular beam epitaxy is studied by means of superconducting quantum interference device (SQUID) magnetometry as well as by ferromagnetic resonance (FMR)…

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

We study the magnetic and lattice contributions to the thermal conductivity of electrically insulating strongly spin-orbit coupled magnetically ordered phases on a two-dimensional honeycomb lattice using the Kitaev-Heisenberg model.…

Mesoscale and Nanoscale Physics · Physics 2017-02-20 Georgios L. Stamokostas , Panteleimon E. Lapas , Gregory A. Fiete

The honeycomb $K-\Gamma$ model is known to have both deconfined spin liquid and confined phases. We study here a confinement transition between the Kitaev spin liquid and a dimerized phase in the limit of strong bond anisotropy. By…

Strongly Correlated Electrons · Physics 2019-03-13 Gideon Wachtel , Dror Orgad

Detailed magnetization, specific heat, and $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$ are reported. At high temperatures, {\cred anisotropy of the…

Strongly Correlated Electrons · Physics 2019-07-30 M. Majumder , F. Freund , T. Dey , M. Prinz-Zwick , N. Büttgen , Y. Skourski , A. Jesche , A. A. Tsirlin , P. Gegenwart

In the Kitaev honeycomb model, the quantum spin fractionalizes into itinerant Majorana and gauge flux spontaneously upon cooling, leading to rich experimental ramifications at finite temperature and an upsurge of research interest. In this…

Strongly Correlated Electrons · Physics 2020-10-07 Han Li , Dai-Wei Qu , Hao-Kai Zhang , Yi-Zhen Jia , Shou-Shu Gong , Yang Qi , Wei Li

The temperature-dependent behavior of magnetic domains plays an essential role in the magnetic properties of materials, leading to widespread applications. However, experimental methods to access the three-dimensional (3D) magnetic domain…

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

Magnetic anisotropies often originate from the spin-orbit coupling and determine magnetic ordering patterns. We develop a microscopic theory for DC electric-field controls of magnetic anisotropies in magnetic Mott insulators and discuss its…

Strongly Correlated Electrons · Physics 2024-03-15 Shunsuke C. Furuya , Masahiro Sato

We discuss the finite-temperature phase diagram of the Heisenberg-Kitaev model on the hexagonal lattice, which has been suggested to describe the spin-orbital exchange of the effective spin-1/2 momenta in the Mott insulating Iridate…

Strongly Correlated Electrons · Physics 2011-09-26 Johannes Reuther , Ronny Thomale , Simon Trebst

In this study, we reanalyze the magnetic interactions in the Kitaev spin liquid candidate materials Na$_2$IrO$_3$, $\alpha$-RuCl$_3$, and $\alpha$-Li$_2$IrO$_3$ using nonperturbative exact diagonalization methods. These methods are more…

Strongly Correlated Electrons · Physics 2016-07-06 Stephen M. Winter , Ying Li , Harald O. Jeschke , Roser Valenti

Spinel Cobalt Vanadate CoV$_2$O$_4$ has been grown on (001) SrTiO$_3$ substrates. Using torque magnetometry experiments, we find that the previously observed temperature induced anisotropy change, where the easy axis changes from the out of…

Materials Science · Physics 2023-03-14 Sangsoo Kim , Christie Thompson , Yan Xin , Christianne Beekman

Resistivity and magnetization have been measured at different temperatures and magnetic fields in organic superconductors $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br. The lower critical field and upper critical field are determined, which…

Superconductivity · Physics 2023-06-19 Huijing Mu , Jin Si , Qingui Yang , Ying Xiang , Haipeng Yang , Hai-Hu Wen

Measurements of the magnetic Gr\"uneisen parameter ($\Gamma_B$) and specific heat on the Kitaev material candidate $\alpha$-RuCl$_3$ are used to access in-plane field- and temperature-dependence of the entropy up to 12 T and down to 1 K. No…

Strongly Correlated Electrons · Physics 2020-08-28 S. Bachus , D. A. S. Kaib , Y. Tokiwa , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valenti , P. Gegenwart

$\alpha$-RuCl$_3$ is drawing much attention as a promising candidate Kitaev quantum spin liquid. However, despite intensive research efforts, controversy remains about the form of the basic interactions governing the physics of this…

Strongly Correlated Electrons · Physics 2020-04-16 J. A. Sears , Li Ern Chern , Subin Kim , P. J. Bereciartua , S. Francoual , Yong Baek Kim , Young-June Kim