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Variational and perturbative relativistic energies are computed and compared for two-electron atoms and molecules with low nuclear charge numbers. In general, good agreement of the two approaches is observed. Remaining deviations can be…

Chemical Physics · Physics 2022-09-21 Dávid Ferenc , Péter Jeszenszki , Edit Mátyus

Canonically, the quantum electrodynamic radiative corrections in bound systems have been evaluated in photon energy regularization, i. e. using a noncovariant overlapping parameter that separates the high-energy relativistic scales of the…

High Energy Physics - Phenomenology · Physics 2013-09-10 B. J. Wundt , U. D. Jentschura

We calculate single-particle excitation energies for a series of 33 molecules using fully selfconsistent GW, one-shot G$_0$W$_0$, Hartree-Fock (HF), and hybrid density functional theory (DFT). All calculations are performed within the…

Materials Science · Physics 2015-05-14 C. Rostgaard , K. W. Jacobsen , K. S. Thygesen

We calculate groundstate total energies and single-particle excitation energies of seven pi conjugated molecules described with the semi-empirical Pariser-Parr-Pople (PPP) model using self-consistent many-body perturbation theory at the GW…

Mesoscale and Nanoscale Physics · Physics 2013-11-22 K. Kaasbjerg , K. S. Thygesen

We perform $GW$ calculations on atoms and diatomic molecules at different levels of self-consistency and investigate the effects of self-consistency on total energies, ionization potentials and on particle number conservation. We further…

Other Condensed Matter · Physics 2015-05-13 Adrian Stan , Nils Erik Dahlen , Robert van Leeuwen

An ab initio approach formulated under an entropy-inspired repartitioning of the electronic Hamiltonian is presented. This ansatz produces orbital eigenvalues each shifted by entropic contributions expressed as subsets of scaled pair…

Chemical Physics · Physics 2025-06-10 Abdulrahman Y. Zamani , Kevin Carter-Fenk

We compute the low energy threshold corrections to neutrino masses and mixing in the Standard Model (SM) and its minimal supersymmetric version, using the effective theory technique. We demonstrate that they stabilize the renormalization…

High Energy Physics - Phenomenology · Physics 2011-09-13 P. H. Chankowski , P. Wasowicz

A new scheme for the numerical evaluation of the one-loop self-energy correction to all orders in Z \alpha is presented. The scheme proposed inherits the attractive features of the standard potential-expansion method but yields a…

Atomic Physics · Physics 2009-11-11 Vladimir A. Yerokhin , Krzysztof Pachucki , Vladimir M. Shabaev

The basis-set correction method based on density-functional theory consists in correcting the energy calculated by a wave-function method with a given basis set by a density functional. This basis-set correction density functional…

Chemical Physics · Physics 2023-07-05 Diata Traore , Emmanuel Giner , Julien Toulouse

We substantiate the need for account of the proper electromagnetic field of the electron in the canonical problem of hydrogen in relativistic quantum mechanics. From mathematical viewpoint, the goal is equivalent to determination of the…

Quantum Physics · Physics 2021-01-12 Leon V. Biguaa , Vladimir V. Kassandrov

Kohn-Sham regularizer (KSR) is a differentiable machine learning approach to finding the exchange-correlation functional in Kohn-Sham density functional theory (DFT) that works for strongly correlated systems. Here we test KSR for weak…

Chemical Physics · Physics 2022-03-22 Bhupalee Kalita , Ryan Pederson , Jielun Chen , Li Li , Kieron Burke

According to time-dependent density functional theory, the exact exchange-correlation kernel f$_{xc}$(n, q, $\omega$) determines not only the ground-state energy but also the excited-state energies/lifetimes and time-dependent linear…

Chemical Physics · Physics 2020-07-01 Adrienn Ruzsinszky , Niraj K. Nepal , J. M. Pitarke , John P. Perdew

An approach aimed to extend the applicability range of non-relativistic microscopic calculations of electronuclear response functions is reviewed. In the quasielastic peak region the calculations agree with experiment at momentum transfers…

Nuclear Theory · Physics 2015-06-23 V. D. Efros

We introduce a systematic hierarchy of one-body Green's function methods derived from the $GW$ approximation, constructed by progressively reducing the dynamical content of the self-energy. Starting from the fully dynamical Dyson…

Chemical Physics · Physics 2026-04-10 Pierre-François Loos , Johannes Tölle

The Colle and Salvetti approach [Theoret. Chim. Acta, 37, 329 (1975)] to the calculation of the correlation energy of a system is modified in order to explicitly include into the theory the kinetic contribution to the correlation energy.…

Materials Science · Physics 2007-05-23 Sebastien Ragot , Pietro Cortona

We present a novel technique to obtain relativistic corrections to the central force problem in the Lagrangian formulation, using a generalized potential energy function. We derive a general expression for a generalized potential energy…

Classical Physics · Physics 2017-07-12 Ashmeet Singh , Binoy Krishna Patra

Ab initio many-body perturbation theory within the $GW$ approximation is a Green's function formalism widely used in the calculation of quasiparticle excitation energies of solids. In what has become an increasingly standard approach,…

The one-loop radiative correction in an ultraviolet (UV) complete electroweak (EW) model without a Higgs particle is calculated. The $\rho$ parameter determining the ratio of the charged to neutral currents is derived for the dominant top…

High Energy Physics - Phenomenology · Physics 2011-07-07 J. W. Moffat

We present and test a new approximation for the exchange-correlation (xc) energy of Kohn-Sham density functional theory. It combines exact exchange with a compatible non-local correlation functional. The functional is by construction free…

Chemical Physics · Physics 2014-05-23 Tobias Schmidt , Eli Kraisler , Adi Makmal , Leeor Kronik , Stephan Kümmel

Trinucleon longitudinal response functions R_L(q,omega) are calculated for q values up to 500 MeV/c. These are the first calculations beyond the threshold region in which both three-nucleon (3N) and Coulomb forces are fully included. We…

Nuclear Theory · Physics 2009-11-10 Victor D. Efros , Winfried Leidemann , Giuseppina Orlandini , Edward L. Tomusiak