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A study is made of nuclear size corrections to the energy levels of single-electron atoms for the ground state of hydrogen like atoms. We consider Fermi charge distribution to the nucleus and calculate atomic energy level shift due to the…

Atomic Physics · Physics 2017-01-02 Babak Nadiri Niri

The random phase approximation (RPA) for the correlation energy functional of density functional theory has recently attracted renewed interest. Formulated in terms of the Kohn-Sham (KS) orbitals and eigenvalues, it promises to resolve some…

Other Condensed Matter · Physics 2009-11-13 Hong Jiang , Eberhard Engel

This work provides a self-consistent extension of the recently proposed density-based basis-set correction method for wave-function electronic-structure calculations [J. Chem. Phys. 149, 194301 (2018)]. In contrast to the previously used…

Classical Physics · Physics 2021-08-25 Emmanuel Giner , Diata Traore , Barthélemy Pradines , Julien Toulouse

The first fully relativistic, rigorous QED calculations of the self-energy correction to the fine-structure levels of heavy muonic atoms are reported. We discuss nuclear model and parameter dependence for this contribution as well as…

Atomic Physics · Physics 2022-06-14 Natalia S. Oreshkina

The self-consistent random phase approximation (RPA) approach with the residual interaction derived from a relativistic point-coupling energy functional is applied to evaluate the isospin symmetry-breaking corrections {\delta}c for the…

Nuclear Theory · Physics 2015-03-19 Z. X. Li , J. M. Yao , H. Chen

We investigate the exchange effect between the final atom's bound electrons and those emitted in the allowed $\beta$-decay of the initial nucleus. The electron wave functions are obtained with the Dirac-Hartree-Fock-Slater self-consistent…

Atomic Physics · Physics 2024-07-17 O. Niţescu , S. Stoica , F. Šimkovic

This paper investigates the influence of the basis set on the GW self-energy correction in the full-potential linearized augmented-plane-wave (LAPW) approach and similar linearized all-electron methods. A systematic improvement is achieved…

Materials Science · Physics 2007-05-23 Christoph Friedrich , Arno Schindlmayr , Stefan Blügel , Takao Kotani

Based on self-consistent field (SCF) atomic mean-field (amf) quantities, we present two simple, yet computationally efficient and numerically accurate matrix-algebraic approaches to correct both scalar-relativistic \textit{and} spin-orbit…

Chemical Physics · Physics 2023-02-03 Stefan Knecht , Michal Repisky , Hans Jørgen Aagaard Jensen , Trond Saue

The fully self-consistent $GW$ (sc$GW$) method with the iterative solution of Dyson equation provides a consistent approach for describing the ground and excited states without any dependence on the mean-field reference. In this work, we…

Chemical Physics · Physics 2024-01-23 Vibin Abraham , Gaurav Harsha , Dominika Zgid

We develop relativistic short-range exchange energy functionals for four-component relativistic range-separated density-functional theory using a Dirac-Coulomb Hamiltonian in the no-pair approximation. We show how to improve the short-range…

Chemical Physics · Physics 2020-06-24 Julien Paquier , Emmanuel Giner , Julien Toulouse

The single particle energies obtained in a Kohn--Sham density functional theory (DFT) calculation are generally known to be poor approximations to electron excitation energies that are measured in transport, tunneling and spectroscopic…

Numerical Analysis · Mathematics 2017-12-29 Meiyue Shao , Lin Lin , Chao Yang , Fang Liu , Felipe H. da Jornada , Jack Deslippe , Steven G. Louie

An exact quantization rule for the Schr\"{o}dinger equation is presented. In the exact quantization rule, in addition to $N\pi$, there is an integral term, called the quantum correction. For the exactly solvable systems we find that the…

Computational Physics · Physics 2015-06-26 Zhong-Qi Ma , Bo-Wei Xu

We introduce an alternative route to quasiparticle self-consistent $GW$ calculations ($\mathrm{qs}GW$) on the basis of a Joint Approximate Diagonalization of the one-body $GW$ Green's functions $G(\varepsilon_n^{QP})$ taken at the input…

Materials Science · Physics 2024-12-05 Ivan Duchemin , Xavier Blase

We use the random phase approximation (RPA) method with the singles correlation energy contributions to calculate lattice energies of ten molecular solids. While RPA gives too weak binding, underestimating the reference data by $13.7$\% on…

Chemical Physics · Physics 2016-09-21 Jiří Klimeš

Considering the nuclear motion, the authors give out the nonrelativistic ground energy of a helium atom by using a simple but effective variational wave function with a flexible parameter $k$. Based on this result, the relativistic and…

Quantum Physics · Physics 2009-11-11 Yi-Shi Duan , Yu-Xiao Liu , Li-Jie Zhang

We study relativistic nuclear matter in the $\sigma - \omega$ model including the ring-sum correlation energy. The model parameters are adjusted self-consistently to give the canonical saturation density and binding energy per nucleon with…

Nuclear Theory · Physics 2008-11-26 J. A. McNeil , C. E. Price , J. R. Shepard

The total energies and the spin states for atoms and their first ions with Z = 1-86 are calculated within the the local spin-density approximation (LSDA) and the generalized-gradient approximation (GGA) to the exchange-correlation (xc)…

Chemical Physics · Physics 2015-05-20 Eli Kraisler , Guy Makov , Itzhak Kelson

The relativistic corrections for the Dirac-Coulomb system are derived through the method of non-relativistic expansion. By expanding the large and small components of the Dirac wave function and the energy eigenvalues in terms of the square…

Atomic Physics · Physics 2024-12-03 Wanping Zhou , Sanjiang Yang , Haoxue Qiao

We give a detailed presentation of our recent scheme to include correlation effects in molecular transport calculations using the GW approximation within the non-equilibrium Keldysh formalism. We restrict the GW self-energy to the central…

Materials Science · Physics 2009-11-13 Kristian S. Thygesen , Angel Rubio

Accurate results for nonrelativistic energy, relativistic, QED, and finite nuclear mass corrections are obtained for $2^1S_{1/2}$, $3^1S_{1/2}$ and $2^1P_{1/2}$ states of the Li atom and Be$^+$ ion. Our computational approach uses the…

Atomic Physics · Physics 2009-11-13 Mariusz Puchalski , Krzysztof Pachucki