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Related papers: Single-shot X-ray Absorption Spectroscopy at X-ray…

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The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…

Resonant inelastic X-ray scattering (RIXS) has become an important scientific tool. Nonetheless, conventional high-resolution RIXS measurements (<100 meV), especially in the soft x-ray range, require large and low-throughput grating…

Materials Science · Physics 2020-06-22 Daniel J. Higley , Hirohito Ogasawara , Sioan Zohar , Georgi L. Dakovski

The photon spectrum from free-electron laser (FEL) light sources offers valuable information in time-resolved experiments and machine optimization in the spectral and temporal domains. We have developed a compact single-shot photon…

Time-resolved X-ray Emission/Absorption Spectroscopy (Tr-XES/XAS) is an informative experimental tool sensitive to electronic dynamics in materials, widely exploited in diverse research fields. Typically, Tr-XES/XAS requires X-ray pulses…

We have implemented the newly-introduced, coherence-based technique of x-ray near-field speckle (XNFS) at 8-ID-I at the Advanced Photon Source. In the near field regime of high-brilliance synchrotron x-rays scattered from a sample of…

Soft Condensed Matter · Physics 2011-02-16 Xinhui Lu , Simon GJ Mochrie , S. Narayanan , A. R. Sandy , M. Sprung

X-ray absorption spectroscopy (XAS) is a premier technique for materials characterization, providing key information about the local chemical environment of the absorber atom. In this work, we develop a database of sulfur K-edge XAS spectra…

The European X-ray Free Electron Laser (XFEL) will deliver 30,000 fully coherent, high brilliance X-ray pulses per second each with a duration below 100 fs. This will allow the recording of diffraction patterns of single complex molecules…

Instrumentation and Detectors · Physics 2015-06-03 Jiaguo Zhang , Eckhart Fretwurst , Robert Klanner , Hanno Perrey , Ioana Pintilie , Thomas Poehlsen , Joern Schwandt

X-ray Free Electron Lasers (XFEL) are revolutionary photons sources, whose ultrashort, brilliant pulses are expected to allow single molecule diffraction experiments providing structural information on the atomic length scale. This ultimate…

Optics · Physics 2015-05-20 Andrea Fratalocchi , Giancarlo Ruocco

Recently developed instrumentation at the University of Washington has allowed for nonresonant x-ray emission spectra (XES) to be measured in a laboratory-setting with an inexpensive, easily operated system. We present a critical evaluation…

Materials Science · Physics 2016-06-22 Devon R. Mortensen , Gerald T. Seidler , Alexander S. Ditter , Pieter Glatzel

Single-shot absorption measurements have been performed using the multi-keV X-rays generated by a laser wakefield accelerator. A 200 TW laser was used to drive a laser wakefield accelerator in a mode which produced broadband electron beams…

An easily accessible method is presented that permits to calculate spectra involving atomic multiplets relevant to X-ray Absorption Spectroscopy (XAS) and Resonant Inelastic X-ray Scattering (RIXS) experiments. We present specific examples…

Strongly Correlated Electrons · Physics 2009-03-16 F. Vernay , B. Delley

X-ray absorption near edge structure (XANES) spectroscopy is a powerful technique for characterizing the chemical state and symmetry of individual elements within materials, but requires collecting data at many energy points which can be…

Applied Physics · Physics 2025-04-25 Ming Du , Mark Wolfman , Chengjun Sun , Shelly D. Kelly , Mathew J. Cherukara

Single-shot terahertz (THz) spectroscopy probes sub-picosecond, non-repetitive events by combining the advantages of laser absorption techniques with the phase-sensitive detection of interferometric methods. However, its usage as a…

Optics · Physics 2025-01-07 Charan R. Nallapareddy , Thomas C. Underwood

Time-resolved X-ray absorption spectroscopy (TR-XAS), based on laser-pump/X-ray probe method, is powerful in capturing the change of geometrical and electronic structure of the absorbing atom upon excitation. TR-XAS data analysis is…

Chemical Physics · Physics 2017-03-08 Fei Zhan , Ye Tao , Haifeng Zhao

The lateral resolution of an X-ray photoelectron spectroscopy instrument, which is equipped with a focused X-ray beam, is limited by the nominal X-ray beam diameter and the long tail intensity distri-bution of the X-ray beam. The long tail…

Instrumentation and Detectors · Physics 2020-12-21 Uwe Scheithauer

X-ray echo spectroscopy, a counterpart of neutron spin-echo, is being introduced here to overcome limitations in spectral resolution and weak signals of the traditional inelastic x-ray scattering (IXS) probes. An image of a point-like x-ray…

Optics · Physics 2016-02-26 Yuri Shvyd'ko

This paper makes a comparison between x-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) in the rare earths. Atomic calculations are given for 2p -> 4f and 2p -> 5d XAS. The latter calculation includes the contraction and…

Materials Science · Physics 2009-10-30 Michel van Veenendaal , Robert Benoist

Operando X-ray absorption spectroscopy (XAS) can probe the electrode-electrolyte interface with single-digit nanometer depth resolution and offers a wealth of insight into the evolution and Coulombic efficiency or degradation of prototype…

M\"ossbauer spectroscopy is widely used to study structure and dynamics of matter with remarkably high energy resolution, provided by the narrow nuclear resonance line widths. However, the narrow width implies low count rates, such that…