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The experimentally obtained (Venkataraman {\em et al}. \cite{latha}) cosine squared relation of electronic conductance in a biphenyl molecule is verified theoretically within a tight-binding framework. Using Green's function formalism we…

Mesoscale and Nanoscale Physics · Physics 2014-04-25 Santanu K. Maiti

The polycrystalline Bi1-xHoxFeO3 (x=0, 0.05, 0.1) compounds were synthesized by conventional solid-state route. Rietveld refinement reveals that all the compounds were stabilized in rhombohedral structure with R3c (IUCr No. 161) space…

Materials Science · Physics 2015-01-06 T. Durga Rao , T. Karthik , Adiraj Srinivas , Saket Asthana

Point defects in Ga- and Al-doped ZnO thin films are studied by means of first principles electronic structure calculations. Candidate defects are identified to explain recently observed differences in electrical and spectroscopical…

Materials Science · Physics 2016-10-06 E. Menéndez-Proupin , P. Palacios , P. Wahnón

We examine the intrinsic physical-chemical properties of the conjugated ladder-type polymer poly(benzimidazobenzophenanthroline) (BBL) in response to electron transfer. We aim at explaining the origin of the anti-ambipolar behavior behind…

Materials Science · Physics 2026-05-29 Maryam Ghotbi , Alejandro Aviles , Perla B. Balbuena

Embedding a magnetic electroactive molecule in a three-terminal junction allows for the fast and local electric field control of magnetic properties desirable in spintronic devices and quantum gates. Here, we provide an example of this…

Conductance measurements of a molecular wire, contacted between an epitaxial molecule-metal bond and the tip of a scanning tunneling microscope, are reported. Controlled retraction of the tip gradually de-hybridizes the molecule from the…

Strongly Correlated Electrons · Physics 2024-02-05 R. Temirov , A. C. Lassise , F. Anders , F. S. Tautz

Reliable organic ferroelectrics for memory applications require extreme endurance under repeated electrical switching. Here we demonstrate exceptional fatigue resistance in highly crystalline 2-methylbenzimidazole (MBI) films grown by…

Materials Science · Physics 2026-03-31 Bibek Tiwari , Yuanyuan Ni , Xiaoshan Xu

Inspired by cotunneling spectroscopy of spin-states in a single OPE5-based molecule, we investigate the prospects for electric control of magnetism in purely organic molecules contacted in a three-terminal geometry. Using the gate…

Mesoscale and Nanoscale Physics · Physics 2012-12-21 J. Fock , M. Leijnse , K. Jennum , A. S. Zyazin , J. Paaske , P. Hedegård , M. Brøndsted Nielsen , H. S. J. van der Zant

We present a theoretical study of the transport characteristics of molecular junctions, where first-row diatomic molecules are attached to (001) gold and platinum electrodes. We find that the conductance of all of these junctions is of the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 J. Ferrer , V. M. Garcia-Suarez

Molecules of bisthiolterthiophene have been adsorbed on the two facing gold electrodes of a mechanically controllable break junction in order to form metal-molecule(s)-metal junctions. Current-voltage (I-V) characteristics have been…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 C. Kergueris , J. -P. Bourgoin , S. Palacin , D. Esteve , C. Urbina , M. Magoga , C. Joachim

This dissertation presents an investigation into the electrical properties of two types of G4-DNA and several DNA-based molecules, targeting them as candidates for molecular wires and devices. Atomic force microscopy (AFM) and electrostatic…

Mesoscale and Nanoscale Physics · Physics 2015-12-08 Gideon I. Livshits

We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunnelling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 Alejandro Ferrón , Santiago A. Rodríguez , Sergio S. Gómez , Jose L. Lado , Joaquín Fernández-Rossier

The potential profile across a biased molecular junction is calculated within the framework of a simple Thomas-Fermi type screening model. In particular, the relationship between this profile and the lateral molecular cross section is…

Chemical Physics · Physics 2007-05-23 Abraham Nitzan , Michael Galperin , Gert-Ludwig Ingold , Hermann Grabert

Magnetic switching of a single molecular magnet (SMM) due to spin-polarized current flowing between ferromagnetic metallic electrodes is investigated theoretically. Magnetic moments of the electrodes are assumed to be collinear and parallel…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 Maciej Misiorny , Józef Barnas

We study the magnetization dynamics of a molecular magnet driven by static and variable magnetic fields within a semiclassical treatment. The underling analyzes is valid in a regime, when the energy is definitely lower than the anisotropy…

Chaotic Dynamics · Physics 2009-07-24 L. Chotorlishvili , P. Schwab , J. Berakdar

The dependence of electron transfer rates and yields in bridged molecular systems on the bridge length, and the dependence of the zero-bias conduction of molecular wires on wire length are discussed. Both phenomena are controlled by…

Chemical Physics · Physics 2007-05-23 Spiros Skourtis , Abraham Nitzan

Donor-$\pi$-acceptor (D-$\pi$-A) functionalization of MOF linkers can enhance visible-light photocatalytic activity, yet the mechanisms responsible for these effects remain unclear. Here we combine EPR spectroscopy, transient…

Among the different types of switchable molecular compounds, sublimable Fe(II) SCO molecules provide a suitable platform to develop smart devices that respond to external stimuli. Here we report the synthesis, crystallographic structure and…

Strong magnetic fields have a large impact on the dynamics of molecules. In addition to the changes of the electronic structure, the nuclei are exposed to the Lorentz force with the magnetic field being screened by the electrons. In this…

Chemical Physics · Physics 2021-07-28 Laurens D. M. Peters , Tanner Culpitt , Laurenz Monzel , Erik I. Tellgren , Trygve Helgaker

Understanding the intermolecular interactions and utilize these interactions to effectively control the transport behavior of single molecule is the key step from single molecule device to molecular circuits1-6. Although many single…

Mesoscale and Nanoscale Physics · Physics 2022-05-26 Xiao Guo , Qing Yang , Wei Yu , Qiuhao Zhu , Yuwen Cai , Wengang Lu , Sheng Meng , Wenjie Liang