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We provide a theoretical estimate of the thermoelectric current and voltage over a Phenyldithiol molecule. We also show that the thermoelectric voltage is (1) easy to analyze, (2) insensitive to the detailed coupling to the contacts, (3)…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Paulsson , S. Datta

We explore electron transport properties in molecular wires made of heterocyclic molecules (pyrrole, furan and thiophene) by using the Green's function technique. Parametric calculations are given based on the tight-binding model to…

Mesoscale and Nanoscale Physics · Physics 2009-09-13 Santanu K. Maiti , S. N. Karmakar

Using benzene-diamine and benzene-dithiol molecular junctions as benchmarks, we investigate the widespread analysis of the quantum transport conductance $\mathcal{G}(\epsilon)$ in terms of the projected density of states (PDOS) onto…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Tonatiuh Rangel , Gian-Marco Rignanese , Valerio Olevano

The angle-dependences of the magnetoresistance of two different isotopic substitutions (deuterated and undeuterated) of the layered organic superconductor \kappa-(ET)2Cu(NCS)2 are presented. The angle dependent magnetoresistance…

Strongly Correlated Electrons · Physics 2009-11-10 P. A. Goddard , S. J. Blundell , J. Singleton , R. D. McDonald , A. Ardavan , A. Narduzzo , J. A. Schlueter , A. M. Kini , T. Sasaki

The quantum transport via a donor (D)-bridge (B)-acceptor (A) single molecule is studied using density functional theory in conjunction with the Landauer-B\"{u}ttiker formalism. Asymmetric electrical response for opposite biases is observed…

Mesoscale and Nanoscale Physics · Physics 2008-09-22 Haiying He , Ravindra Pandey , Govind Mallick , Shashi P. Karna

The current work investigates candidate building blocks based on molecular junctions from hydrogen transfer tautomerization in the benzoquinone-like core of an azophenine molecule with QTAIM and the recently-introduced stress tensor…

We report the formation of self-assembled monolayers of a molecular photoswitch (azobenzene-bithiophene derivative, AzBT) on cobalt via a thiol covalent bond. We study the electrical properties of the molecular junctions formed with the tip…

We report a full self-consistent ab initio calculation of the conductance of a diarylethene-based molecular switch with two graphene electrodes. Our result show the contributions of the resonant states of the molecule, of the electrode…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 C. Motta , M. I. Trioni , G. P. Brivio , K. L. Sebastian

The conductance of a single metal-molecule-metal junction depends critically on the conformations of the molecule. In the simple case of a biphenyl, two phenyl rings linked together by a single C-C bond, the conductance is expected to…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Latha Venkataraman , Jennifer E. Klare , Colin Nuckolls , Mark S. Hybertsen , Michael L. Steigerwald

Vibrationally inelastic electron transport through a flexible molecular junction is investigated. The study is based on a mechanistic model for a biphenyl molecule between two metal electrodes. Employing methods from electron-molecule…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Martin Cizek , Michael Thoss , Wolfgang Domcke

The attachment of redox active molecules to transition metal dichalcogenides (TMDs), such as MoS2, constitutes a promising approach for designing electrochemically switchable devices through the control of the material charge/spin transport…

We report the fabrication and electron transport properties of nanoparticles self-assembled networks (NPSAN) of molecular switches (azobenzene derivatives) interconnected by Au nanoparticles, and we demonstrate optically-driven switchable…

Applied Physics · Physics 2018-10-09 Y. Viero , D. Guerin , A. Vladyka , F. Alibart , S. Lenfant , M. Calame , D. Vuillaume

We show that a ferro-electric quantum phase transition can be driven by the dipolar interaction of polar molecules in the presence a micro-wave field. The obtained ferro-electricity crucially depends on the harmonic confinement potential,…

Quantum Gases · Physics 2015-05-13 Chien-Hung Lin , Yi-Ting Hsu , Hao Li , Daw-Wei Wang

We present calculations of spin-dependent electron transport through single organic molecules bridging pairs of iron nanocontacts. We predict the magnetoresistance of these systems to switch from positive to negative with increasing applied…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Hugh Dalgleish , George Kirczenow

Azulene (Az) is a non-alternating, aromatic hydrocarbon composed of a five-membered, electron-rich and a seven-membered, electron-poor ring; an electron distribution that provides intrinsic redox activity. By varying the attachment points…

Mesoscale and Nanoscale Physics · Physics 2017-09-04 Florian Schwarz , Michael Koch , Georg Kastlunger , Heinz Berke , Robert Stadler , Koushik Venkatesan , Emanuel Loertscher

The conductance ${\cal G}$ of an Aharonov-Bohm interferometer (ABI), with a strongly correlated quantum dot on one arm, is expressed in terms of the dot Green function, $G_{dd}$, the magnetic flux $\phi$ and the non-interacting parameters…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Amnon Aharony , Ora Entin-Wohlman

We investigate the electron transfer from a dissociatively adsorbed H2 molecule to a Au(111) surface using the first-principles methods. A fractional electron transfers from a molecule to a substrate, and potential energy increases during…

Materials Science · Physics 2009-11-13 Shigeyuki Takagi , Jun-ichi Hoshino , Hidekazu Tomono , Kazuo Tsumuraya

We probed the charge transfer interaction between the amine-containing molecules: hydrazine, polyaniline and aminobutyl phosphonic acid, and carbon nanotube field effect transistors (CNTFETs). We successfully converted p-type CNTFETs to…

Materials Science · Physics 2015-07-20 Christian Klinke , Jia Chen , Ali Afzali , Phaedon Avouris

We report on inelastic electron tunneling spectroscopy measurements carried out on single molecules incorporated into a mechanically controllable break-junction of Au and Pt electrodes at low temperature. Here we establish a correlation…

Mesoscale and Nanoscale Physics · Physics 2010-11-16 Youngsang Kim , Hyunwook Song , Florian Strigl , Hans-Fridtjof Pernau , Takhee Lee , Elke Scheer

The Q-cycle mechanism plays an important role in the conversion of the redox energy into the energy of the proton electrochemical gradient across the biomembrane. The bifurcated electron transfer reaction, which is built into this…

Biological Physics · Physics 2013-03-19 Anatoly Yu. Smirnov , Franco Nori
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