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We investigate from first-principles the change in transport properties of a two-dimensional azobenzene monolayer sandwiched between two Au electrodes that undergoes molecular switching. We focus on transport differences between a…

Mesoscale and Nanoscale Physics · Physics 2012-08-07 Yan Wang , Hai-Ping Cheng

A new azobenzene-thiophene molecular switch is designed, synthesized and used to form self-assembled monolayers (SAM) on gold. An "on/off" conductance ratio up to 7x1E3 (with an average value of 1.5x1E3) is reported. The "on" conductance…

In molecular nanotechnology, a single molecule is envisioned to act as the basic building block of electronic devices. Such devices may be of special interest for organic photovoltaics, data storage, and smart materials. However, more often…

Materials Science · Physics 2019-05-22 Reinhard J. Maurer , Karsten Reuter

We present a magneto-photoluminescence study of individual vertically stacked InAs/GaAs quantum dot pairs separated by thin tunnel barriers. As an applied electric field tunes the relative energies of the two dots, we observe a strong…

We report the electronic transport properties of a new photo-addressable molecular switch. The switching process relies on a new concept based on linear {\pi}-conjugated dynamic systems, in which the geometry and hence the electronic…

Mesoscale and Nanoscale Physics · Physics 2017-06-13 S. Lenfant , Y. Viero , C. Krzeminski , D. Vuillaume , D. Demeter , I. Dobra , M. Ocafrain , P. Blanchard , J. Roncali , C. van Dyck , J. Cornil

The electronic properties of molecular conductors can be readily varied via physical or chemical pressure as it increases the bandwidth W; this enables crossing the Mott insulator-to-metal phase transition by reducing electronic…

Strongly Correlated Electrons · Physics 2019-11-18 Y. Saito , R. Rösslhuber , A. Löhle , M. Sanz Alonso , M. Wenzel , A. Kawamoto , A. Pustogow , M. Dressel

We investigate the origin of asymmetry in the measured current-voltage (I-V) characteristics of molecules with no inherent spatial asymmetry. We establish that such molecules can exhibit asymmetric I-V characteristics due to unequal…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Avik W. Ghosh , Ferdows Zahid , Prashant S. Damle , Supriyo Datta

Despite its fundamental importance for nano physics and chemistry and potential device applications, the relationship between atomic structure and electronic transport in molecular nanostructures is not well understood. Thus the…

Mesoscale and Nanoscale Physics · Physics 2014-02-04 Alireza Saffarzadeh , Firuz Demir , George Kirczenow

The behavior of polar columnar phases made of bent shaped molecules (B_1Rev and B_1RevTilted) was studied under applied electric field. There are two competing mechanisms of switching in polar B_1RevTilted columnar phase: the collective…

Soft Condensed Matter · Physics 2007-05-23 Ewa Gorecka , Natasa Vaupotic , Damian Pociecha , Mojca Cepic , Josef Mieczkowski

Recent years have shown steady progress in research towards molecular electronics [1,2], where molecules have been investigated as switches [3-5], diodes [6], and electronic mixers [7]. In much of the previous work a Scanning Tunnelling…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. H. M. Smit , Y. Noat , C. Untiedt , N. D. Lang , M. van Hemert , J. M. van Ruitenbeek

The kinetic Monte Carlo simulations are employed to study the proton conductivity for anhydrous heterocyclic based polymers. The proton transport is based on a two-step process called the Grotthuss mechanism. In the referring system the…

Materials Science · Physics 2015-06-23 T. Masłowski , A. Drzewiński , P. Ławniczak , J. Ulner

We obtain here a new relation for the reduced electric quadrupole transition probability B(E2) of a given nucleus in terms of its derivatives with respect to neutron and proton numbers based on a similar local energy relation in the…

Nuclear Theory · Physics 2015-06-19 S. Pattnaik , R. C. Nayak

Time-resolved Faradary rotation experiments have demonstrated coherent transfer of electron spin between CdSe colloidal quantum dots coupled by conjugated molecules. We employ here a Green's function approach, using semi-empirical…

Other Condensed Matter · Physics 2009-11-11 Joshua Schrier , K. Birgitta Whaley

Recently, methanol was identified as a sensitive target system to probe variations of the proton-to-electron mass ratio $\mu$ [Jansen \emph{et al.} Phys. Rev. Lett. \textbf{106}, 100801 (2011)]. The high sensitivity of methanol originates…

Chemical Physics · Physics 2012-03-07 Paul Jansen , Isabelle Kleiner , Li-Hong Xu , Wim Ubachs , Hendrick L. Bethlem

In this work, we have investigated conduction through an artificial molecule comprising two coupled quantum dots. The question addressed is the role of inter-dot coupling on electronic transport. We find that the current through the…

Mesoscale and Nanoscale Physics · Physics 2011-09-22 M. Imran , B. Tariq , M. Tahir , K. Sabeeh

Switching anisotropic molecules from strongly-absorbing to strongly-amplifying through a transparent state is shown to be possible by application of dc or ac control electric fields without the requirement of the population inversion. It is…

Quantum Physics · Physics 2015-06-26 A. K. Popov , V. V. Slabko

The change of conductance of single molecule junctions in response to various external stimuli is the fundamental mechanism for single-molecule electronic devices with multiple functionalities. We propose a concept that the conductance of…

Mesoscale and Nanoscale Physics · Physics 2014-12-04 Chengbo Zhu , Xiaolin Wang

Conjugated molecules are materials which are widely studied and developed for molecular electronic technologies focusing on single molecule devices. In this paper we observed the molecular conductance of single molecule based on n phenyl…

Materials Science · Physics 2015-10-15 Setianto , B. Aradi , Th. Niehaus

Using a first principles approach to electron transport, we calculate the electrical and thermoelectrical transport properties of a series of molecular wires containing benzo-difuran subunits. We demonstrate that the side groups introduce…

Mesoscale and Nanoscale Physics · Physics 2014-05-15 Csaba G. Péterfalvi , Iain Grace , Dávid Zs. Manrique , Colin J. Lambert

Recently, rectifying direction inversion has been observed in dipyrimidinyl-diphenyl (PMPH) diblock molecular wire [J. Am. Chem. Soc. (2005) 127, 10456], and a protonation mechanism was suggested to explain this interesting phenomena. In…

Materials Science · Physics 2008-12-14 Zhenyu Li
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