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In this paper we attempt to understand the role of tin and carbon in magnetic interactions in Mn$_3$SnC. Mn$_3$SnC exhibits a time dependent magnetic configuration and a complex magnetic ground state with both ferromagnetic and…

Materials Science · Physics 2018-10-18 V. N. Gaonkar , E. T. Dias , Arka Bikash Dey , Rajendra Prasad Giri , A. K. Nigam , K. R. Priolkar

The volume expanding magnetostructural transition in Mn$_3$GaC and Mn$_3$SnC has been identified to be due to distortion of Mn$_6$C octahedra. Despite a similar lattice volume as Mn$_3$SnC and similar valence electron contribution to the…

Materials Science · Physics 2019-02-19 E. T. Dias , A. Das , A. Hoser , S. Emura , A. K. Nigam , K. R. Priolkar

In this paper we attempt to understand the different nature of first order magnetic transformation in Mn$_3$SnC as compared to that in Mn$_3$GaC. The transformation in Mn$_3$SnC is close to room temperature (T$_t \approx$ 280K) and is…

Materials Science · Physics 2015-06-30 E. T. Dias , K. R. Priolkar , A. Das , G. Aquilanti , Ö. Çakir , M. Acet , A. K. Nigam

We investigate the magnetic structure of Mn3-xFexSn2 using neutron powder diffraction experiments and electronic structure calculations. These alloys crystallize in the orthorhombic Ni3Sn2 type of structure (Pnma) and comprise two…

Materials Science · Physics 2013-09-03 Q. Recour , V. Ban , Z. Gercsi , T. Mazet , M. Francois , B. Malaman

The structural and magnetic properties of transition metal-doped Mn$_3$SnC are studied with an aim to understand the effect of transition metal atom on magnetostructural properties of the antiperovskite compound. The doped…

Materials Science · Physics 2020-04-03 V. N. Gaonkar , E. T. Dias , A. K. Nigam , K. R. Priolkar

In this paper, we attempt to understand the cause of magnetostructural transformation in Mn-based antiperovskites by calculating EXAFS at the K edges of constituent metal atoms in three antiperovskite compounds, Mn$_3$GaC, Mn$_3$SnC and…

Materials Science · Physics 2020-04-02 Aishwarya Mungale , K. R. Priolkar

Frustrated magnetism in face-centred cubic (fcc) magnetic sublattices remains underexplored but holds considerable potential for exotic magnetic behaviour. Here we report on the crystal structure, magnetic and thermodynamic properties of…

A systematic study using neutron diffraction and magnetic susceptibility are reported on Mn substituted ferrimagnetic inverse spinel Ti$_{1-x}$Mn$_{x}$Co$_2$O$_4$ in the temperature interval 1.6 K $\leq$ $T$ $\leq$ 300 K. Our neutron…

Strongly Correlated Electrons · Physics 2020-03-23 P. Pramanik , D. C. Joshi , M. Reehuis , A. Hoser , J. U. Hoffmann , R. S. Manna , T. Sarkar , S. Thota

Mn$_3$GaC undergoes a ferromagnetic to antiferromagnetic, volume discontinuous cubic-cubic phase transition as a function of temperature, pressure and magnetic field. Through a series of temperature dependent x-ray absorption fine structure…

Materials Science · Physics 2017-10-11 E. T. Dias , K. R. Priolkar , R. Ranjan , A. K. Nigam , S. Emura

Local structural measurements have been performed on hexagonal HoMnO3 in order to ascertain the specific changes in bond distances which accompany magnetic ordering transitions. The transition from paramagnetic to the antiferromagetic…

Strongly Correlated Electrons · Physics 2015-05-14 T. A. Tyson , T. Wu , K. H. Ahn , S. Kim , S. -W. Cheong

Density functional theory is used to study the effect of compressive and tensile biaxial strain on Mn$_{3}$GaN. Mn$_{3}$GaN is a non-collinear antiferromagnetic antiperovskite with a similar structure to that of an ideal cubic oxide…

Materials Science · Physics 2025-01-14 Roman Malyshev , Ingeborg-Helene Svenum , Sverre M. Selbach , Thomas Tybell

Using results of the band structure calculations in the local-spin-density approximation we demonstrate how the crystal distortions affect the magnetic structure of orthorhombically distorted perovskites leading to a non-collinear spin…

Materials Science · Physics 2009-11-10 I. V. Solovyev , N. Hamada , K. Terakura

The crystal and magnetic structures of the nitride antiperovskite Mn$_3$GeN reveals ferrimagnetic order stemming from a distorted kagome-derived lattice of the Mn atoms. Polycrystalline Mn$_3$GeN was synthesized via a solid-state reaction…

We have investigated the crystal, electronic, and magnetic structure of Mn5O8 by means of state of-the-art density functional theory calculations and neutron powder diffraction (NPD) measurements. This compound stabilizes in the monoclinic…

Materials Science · Physics 2016-09-12 M. R. Ashwin Kishore , H. Okamoto , Lokanath Patra , R. Vidya , Anja O. Sjastad , H. Fjellvag , P. Ravindran

Magnetic structures of metastable perovskites ScCrO3, InCrO3 and TlCrO3, stabilized under high-pressure and high-temperature conditions, have been studied by neutron powder diffraction. Similar to the other orthochromites LnCrO3…

Strongly Correlated Electrons · Physics 2021-01-13 Lei Ding , Pascal Manuel , Dmitry D. Khalyavin , Fabio Orlandi , Yu Kumagai , Fumiyasu Oba , Wei Yi , Alexei A. Belik

We study the electronic and magnetic structures of multiferroic CaMn$_7$O$_{12}$ by first-principle calculations, based on the experimentally determined modulated crystal structure. We confirm the presence of a 3$d$ orbital modulation of…

Materials Science · Physics 2015-06-23 Kun Cao , Roger D. Johnson , Natasha Perks , Feliciano Giustino , Paolo G. Radaelli

Room temperature Mn K-edge extended x-ray absorption fine structure (EXAFS) studies were carried out on La$_{1-x}$Sr$_x$MnO$_{3+\delta}$ (x = 0.1 to 0.9) compounds. It is found from the detailed EXAFS analysis that the local structure…

Materials Science · Physics 2009-11-11 R. Bindu , S. K. Pandey , Ashwani Kumar , S. Khalid , A. V. Pimpale

The complex metal oxides Mn2ASbO6 (A=In, Sc) with a corundum-related structure A3BO6 have been prepared as polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties have been investigated using a…

Materials Science · Physics 2011-11-21 S. A. Ivanov , P. Nordblad , R. Mathieu , R. Tellgren , E. Politova , G. André

We have studied the electronic and magnetic states of Co and Mn atoms at the interface of the Co$_\mathrm{2}$Mn$_{\beta}$Si (CMS)/MgO ($\beta$=0.69, 0.99, 1.15 and 1.29) magnetic tunnel junction (MTJ) by means of x-ray magnetic circular…

Strongly Correlated Electrons · Physics 2015-06-11 V. R. Singh , V. K. Verma , K. Ishigami , G. Shibata , A. Fujimori , T. Koide , Y. Miura , M. Shirai , T. Ishikawa , G. f. Li , M. Yamamoto

We investigate the magnetic properties of three Mn$_6$ single molecule magnets by means of inelastic neutron scattering and frequency domain magnetic resonance spectroscopy. The experimental data reveal that small structural distortions of…

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