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The correlation between static magnetoelectric coupling and magnetic structure was investigated in $TbMn_{0.98}Fe_{0.02}O_{3}$ with magnetic field up to 8 T and down to 2 K. Single-crystal neutron diffraction experiments reveal a…

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

We use density-functional theory calculations to explore the magnetic properties of perovskite rare-earth nickelates, $\mathcal{R}$NiO$_3$, by constructing microscopic magnetic models containing all relevant exchange interactions via…

Materials Science · Physics 2021-08-04 Danis I. Badrtdinov , Alexander Hampel , Cyrus E. Dreyer

The crystal structure and the magnetism of BaMn$_2$O$_3$ have been studied by thermodynamic and by diffraction techniques using large single crystals and powders. BaMn$_2$O$_3$ is a realization of a $S = 5/2$ spin ladder as the magnetic…

Strongly Correlated Electrons · Physics 2015-05-20 M. Valldor , O. Heyer , A. C. Komarek , A. Senyshyn , M. Braden , T. Lorenz

The magnetic correlations in double perovskites La2Mn2-xNixO6 (x = 0.5, 0.75, 1.0, 1.25 and 1.5) have been systematically investigated across macroscopic, mesoscopic, and microscopic length scales using temperature-dependent bulk DC…

Materials Science · Physics 2025-10-14 A. K. Bera , K. S. Chikara , B. Saha , S. M. Yusuf , Mohd. Nasir , S. Sen

The magnetic order, spin dynamics, and crystal structure of the multiferroic Sr0.56Ba0.44MnO3 have been investigated using neutron and x-ray scattering. Ferroelectricity develops at TC=305 K with a polarization of 4.2 microC/cm2 associated…

Transition metal compounds with complex crystal structures tend to demonstrate interesting magnetic coupling resulting in unusual magnetic properties. In this work, the structural and magnetic characterization of a single crystal of the…

Materials Science · Physics 2019-10-18 S. J. Ahmed , J. E. Greedan , C. Boyer , M. Niewczas

We model changes of magnetic ordering in Mn-antiperovskite nitrides driven by biaxial lattice strain at zero and at finite temperature. We employ a non-collinear spin-polarised density functional theory to compare the response of the…

Strongly Correlated Electrons · Physics 2017-06-07 J. Zemen , E. Mendive Tapia , Z. Gercsi , R. Banerjee , C. E. Patrick , J. B. Staunton , K. G. Sandeman

We have successfully induced multiferroic behavior in the A-type antiferromagnet SmMnO3 by the substitution of Y at the Sm site. A magnetic transition develops at 24 K for Sm1-xYxMnO3 (x=0.4,0.5) which is not present in the parent compound.…

Strongly Correlated Electrons · Physics 2011-05-17 D. O'Flynn , C. V. Tomy , M. R. Lees , A. Daoud-Aladine , G. Balakrishnan

Coupling between different interactions allows to control physical aspects in multifunctional materials by perturbing any of the degrees of freedom. Here, we aim to probe the correlation among structural, electronic and magnetic observables…

Materials Science · Physics 2025-07-28 S. Majumder , M. Tripathi , D. O. de Souza , A. Sagdeo , L. Olivi , M. N. Singh , S. Pal , R. J. Choudhary , D. M. Phase

Effect of carbon content on magnetostructural transformation in antiperovskites of the type Mn$_3$GaC$_x$ ($x$ = 0.8, 1.0 and 1.05) has been investigated. It is found that, increase in carbon content changes the ground state from…

Materials Science · Physics 2015-06-19 E. T . Dias , K. R. Priolkar , A. K. Nigam

The local atomic disorder and the electronic structure in the environment of manganese atoms in LaMnO_3 has been studied by x-ray absorption spectroscopy, over a temperature range (300K to 870K) covering the orbital ordering transition…

Strongly Correlated Electrons · Physics 2009-11-10 Raquel A. Souza , Narcizo M. Souza-Neto , Aline Y. Ramos , Helio C. N. Tolentino , Eduardo Granado

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

Strongly Correlated Electrons · Physics 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…

We report temperature dependent magnetization and neutron diffraction measurements on the corundum related magnetoelectric antiferromagnet Mn$_{4}$Ta$_{2}$O$_{9}$. Measurements performed on a single crystalline specimen reveal that the…

Strongly Correlated Electrons · Physics 2021-01-20 Soumendra Nath Panja , Pascal Manuel , Sunil Nair

We use resonant and non-resonant X-ray diffraction measurements in combination with first-principles electronic structure calculations and Monte Carlo simulations to study the relationship between crystal structure and multiferroic orders…

Detailed structural measurements were conducted on a new perovskite, ScMnO3, and on orthorhombic LuMnO3. Complementary density functional theory (DFT) calculations were carried out, and predict that ScMnO3 possesses E-phase magnetic order…

Strongly Correlated Electrons · Physics 2015-06-19 T. Yu , T. A. Tyson , H. Y. Chen , A. M. M. Abeykoon , Y. -S. Chen , K. H. Ahn

The local structure about the Mn site in the half doped system La0.5Ca0.5MnO3 was measured in magnetic fields up 10 T to probe the melting of the charge ordered state. Examination of the Mn-O and Mn-Mn correlations reveal three distinct…

Strongly Correlated Electrons · Physics 2009-11-10 T. A. Tyson , M. Deleon , M. Crof , V. G. Harris , C. -C. Kao , J. Kirkland , S. -W. Cheong

The chemical selectivity and great sensitivity of the Extended X-ray Absorption Spectroscopy technique allowed the determination, in the paramagnetic phase, of the structural distortions induced by doping in the spin-Peierls CuGeO$_3$…

This article takes a broad view of the understanding of magnetic bistability and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on three families of relatively simple, low-nuclearity transition metal clusters: spin S…