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Photothermal spectroscopy and microscopy provides a route to measure the spectral and spatial properties of individual nanoscopic absorbers, independent from scattering, extinction, and emission. The approach relies upon use of two light…

Optics · Physics 2021-04-12 Harrison J. Goldwyn , Stephan Link , David J. Masiello

X-ray echo spectroscopy, a space-domain counterpart of neutron spin echo, is a recently proposed inelastic x-ray scattering (IXS) technique. X-ray echo spectroscopy relies on imaging IXS spectra, and does not require x-ray…

Optics · Physics 2017-08-04 Yuri Shvyd'ko

X-ray refraction and absorption by neon atoms under the influence of an 800 nm laser with an intensity of 10^13 W/cm^2 is investigated. For this purpose, we use an ab initio theory suitable for optical strong-field problems. Its results are…

Atomic Physics · Physics 2013-03-25 Christian Buth , Robin Santra , Linda Young

M\"ossbauer spectroscopy is widely used to study structure and dynamics of matter with remarkably high energy resolution, provided by the narrow nuclear resonance line widths. However, the narrow width implies low count rates, such that…

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

Spectroscopy has played the key role in revealing, and thereby understanding, the structure of atoms and molecules. A central drive in this field is the pursuit of higher precision and accuracy so that ever more subtle effects might be…

We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

Chemical Physics · Physics 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

Nuclear resonant forward scattering (NFS) and nuclear inelastic scattering (NIS) of synchrotron radiation are fairly recent spectroscopic methods for the investigation of complexes containing M\"ossbauer-active transition metal ions. NFS,…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Volker Schünemann , Alfred Xaver Trautwein , Heiner Winkler

Achieving high spatial resolution is the goal of many imaging systems. Designing a high-resolution lens with diffraction-limited performance over a large field of view remains a difficult task in imaging system design. On the other hand,…

A new technique to search for new scalar and tensor interactions at the sub-micrometer scale is presented. The technique relies on small shifts of nuclear gamma lines produced by the coupling between matter and the nuclei in the source or…

High Energy Physics - Phenomenology · Physics 2021-01-04 Giorgio Gratta , David E. Kaplan , Surjeet Rajendran

High energy resolution, hard X-ray spectroscopies are powerful element selective probes of the electronic and local structure of matter, with diverse applications in chemistry, physics, biology and materials science. The routine application…

Instrumentation and Detectors · Physics 2016-11-03 Zoltán Németh , Jakub Szlachetko , Éva G. Bajnóczi , György Vankó

The X-ray signal from active galactic nuclei and black hole X-ray binaries is highly variable on a range of timescales. This variability can be exploited to map the region of interest close to the black hole, which is far too small to…

High Energy Astrophysical Phenomena · Physics 2023-05-24 Adam Ingram

Spectroscopy has an illustrious history delivering serendipitous discoveries and providing a stringent testbed for new physical predictions, including applications from trace materials detection, to understanding the atmospheres of stars…

Atomic Physics · Physics 2015-01-05 Gar-Wing Truong , James D. Anstie , Eric F. May , Thomas M. Stace , Andre N. Luiten

A spectrograph is an optical instrument that disperses photons of different energies into distinct directions and space locations, and images photon spectra on a position-sensitive detector. Spectrographs consist of collimating, angular…

Optics · Physics 2015-06-11 Yuri Shvyd'ko

Absorption spectroscopy is routinely used to characterise chemical and biological samples. For the state-of-the-art in absorption spectroscopy, precision is theoretically limited by shot-noise due to the fundamental Poisson-distribution of…

Photoabsorption of atomic oxygen in the energy region below the $\rm 1s^{-1}$ threshold in x-ray spectroscopy from {\it Chandra} and {\it XMM-Newton} is observed in a variety of x-ray binary spectra. Photoabsorption cross sections…

High Energy Astrophysical Phenomena · Physics 2015-06-16 B. M. McLaughlin , C. P. Ballance , K. P. Bowen , D. J. Gardenghi , W. C. Stolte

Recording of transient absorption microscopy images requires fast detection of minute optical density changes, which is typically achieved with high-repetition-rate laser sources and lock-in detection. Here, we present a highly flexible and…

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

Transient X-ray absorption techniques can measure ultrafast dynamics of the elemental edges in a material or multiple layer junction, giving them immense potential for deconvoluting concurrent processes. However, the interpretation of the…

Materials Science · Physics 2021-06-10 Hanzhe Liu , Isabel M. Klein , Jonathan M. Michelsen , Scott K. Cushing

We have implemented the newly-introduced, coherence-based technique of x-ray near-field speckle (XNFS) at 8-ID-I at the Advanced Photon Source. In the near field regime of high-brilliance synchrotron x-rays scattered from a sample of…

Soft Condensed Matter · Physics 2011-02-16 Xinhui Lu , Simon GJ Mochrie , S. Narayanan , A. R. Sandy , M. Sprung